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Pb(II) Coordination Polymer Based on Mixed Ligands: Syntheses, Structures, Photoluminescence, and Photocatalysis

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Abstract

A new coordination polymer [Pb(ttbt)(1,4-bdoa)]n·2nH2O (1) (1,4-H2bdoa = benzene-1,4-dioxyacetic acid and ttbt = 10,11,12,13-tetrahydro-4,5,9,14-tetraaza-benzo[b]triphenylene) has been obtained under hydrothermal conditions. The structure of polymer 1 has been determined by single-crystal X-ray diffraction analysis and further characterized by elemental analysis, infrared spectra (IR), powder X-ray diffraction (PXRD) and diffuse-reflectance UV–vis spectrum. Polymer 1 displays a one-dimensional chain structure, which is further extended into a two-dimensional layer structure through π-π stacking interactions and hydrogen-bonding interactions. The photoluminescence behavior of polymer 1 was also discussed in paper. Meanwhile, polymer 1 represents good performance for the photocatalytic degradation of organic dyes under UV irradiation.

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Acknowledgments

This work is supported by the Program for New Century Excellent Talents in University (NCET-10-0176) of China, the National Natural Science Foundation of China (No. 21407064) and Postgraduate Research and Innovation Project of Jiangsu University (No. CXZZ11_0555).

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Authors and Affiliations

  1. School of Material Science and Engineering, Jiangsu University, Zhenjiang, 212013, People’s Republic of China

    Xiu-Ying Li & Qing-Feng Guan

  2. Key Laboratory of Preparation and Applications of Environmental Friendly Materials (Jilin Normal University), Chinese Ministry of Education, Siping, 136000, People’s Republic of China

    Xiu-Ying Li & Guang-Bo Che

  3. School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212013, People’s Republic of China

    Lin Gao, Chun-Bo Liu, Guang-Bo Che & Yong-Sheng Yan

  4. Jilin Entry-Exit Inspection and Quarantine Bureau, Hunchun, People’s Republic of China

    Yue-Qi Niu

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  1. Xiu-Ying Li
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  2. Lin Gao
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  4. Chun-Bo Liu
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Correspondence to Guang-Bo Che or Yong-Sheng Yan.

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Li, XY., Gao, L., Niu, YQ. et al. Pb(II) Coordination Polymer Based on Mixed Ligands: Syntheses, Structures, Photoluminescence, and Photocatalysis. J Inorg Organomet Polym 25, 886–891 (2015). https://doi.org/10.1007/s10904-015-0182-9

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  • DOI: https://doi.org/10.1007/s10904-015-0182-9

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