Abstract
Two novel Wells–Dawson based coordination polymers, [Co2(btb)4(H2O)][H2X2W18O62]·nH2O (X = P for 1 and As for 2; n = 3 for 1 and 6 for 2) (btb = 1,4-bis(1,2,4-triazol-1-y1)butane), have been successfully isolated under hydrothermal conditions. Single crystal X-ray diffraction analyses reveal that isostructural compounds 1 and 2 exhibit 2D metal–organic layers, which are further linked by four-dentate [X2W18O62]6− anions to form an unusual (4,4,6)-connected self-penetrating 3D framework with the Schläfli symbol of {3·5·64}{32·52·66·73·82}{52·64}. To the best of our knowledge, this kind of topological structure has not been reported yet. The electrochemical and photocatalytic properties of compounds 1 and 2 have been investigated.
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Acknowledgments
Financial supports of this research by the National Natural Science Foundation of China (No.21171025 and 21101015), New Century Excellent Talents in University (NCET-09-0853), Natural Science Foundation (201102003) and Doctoral Initiation Project (No. 20111147) of Liaoning Province.
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Wang, XL., Zhao, D. & Tian, AX. Two Novel 3D Wells–Dawson Based Coordination Polymers with Unusual Topological Structure Extended by 1,4-Bis(1,2,4-triazol-1-yl)butane. J Clust Sci 24, 259–271 (2013). https://doi.org/10.1007/s10876-012-0548-x
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DOI: https://doi.org/10.1007/s10876-012-0548-x