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Carbon quantum dots: organic–inorganic perovskite composites for optoelectronic applications

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Abstract

In this study, we focus on carbon quantum dots (CQDs) derived from L-Lysine using a microwave-assisted technique, which offers a rapid and straightforward route to generate CQDs smaller than 10 nm on average. We present a method for procuring dry CQDs powder, capable of dissolving in various solvents. To examine the influence of CQDs on the properties of organic–inorganic perovskite and the potential impact of DMA solvent on CQDs, we investigated the optical and electrical characteristics of both pure CQDs and CQDs combined with MAPbBr3 films within a temperature range from 89 to 293 K. Our findings reveal the presence of a positive temperature coefficient of resistivity in the temperature range of 90–290 K. Subsequently, we discuss the plausible mechanism responsible for charge carrier transport in these types of composites.

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Data availability

The datasets generated during and/or analyzed during the current study are available from the corresponding author on reasonable request.

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Funding

The authors did not receive support from any organization for the submitted work.

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Authors and Affiliations

  1. Ioffe Institute, 26 Politekhnicheskaya, St. Petersburg, Russian Federation, 194021

    Grigorii V. Nenashev, Petr A. Aleshin, Igor P. Shcherbakov, Vasily N. Petrov & Andrey N. Aleshin

  2. Saint Petersburg Electrotechnical University «LETI», ul. Professora Popova 5, St. Petersburg, Russian Federation, 197022

    Roman S. Kryukov, Maria S. Istomina & Vyacheslav A. Moshnikov

  3. Almazov National Medical Research Centre, 2 Akkuratova Street, St. Petersburg, Russian Federation, 197341

    Maria S. Istomina

Authors
  1. Grigorii V. Nenashev
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  2. Roman S. Kryukov
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  4. Petr A. Aleshin
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  5. Igor P. Shcherbakov
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  6. Vasily N. Petrov
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  7. Vyacheslav A. Moshnikov
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  8. Andrey N. Aleshin
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Contributions

All authors contributed to the study conception and design. Material preparation, data collection and analysis were performed by GVN, RSK, MSI and PAA. The first draft of the manuscript was written by GVN, RSK, ANA and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.

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Correspondence to Grigorii V. Nenashev.

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Nenashev, G.V., Kryukov, R.S., Istomina, M.S. et al. Carbon quantum dots: organic–inorganic perovskite composites for optoelectronic applications. J Mater Sci: Mater Electron 34, 2114 (2023). https://doi.org/10.1007/s10854-023-11566-5

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  • DOI: https://doi.org/10.1007/s10854-023-11566-5

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