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Achieving high energy-storage density in K0.5Na0.5NbO3 optimized Bi0.25Na0.25Ba0.15Sr0.35TiO3 relaxor ferroelectric ceramics

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Abstract

Lead-free ceramics with high energy-storage density and dielectric stability are attracted considerable attention to address low-driven energy storage electronic fields. Here, the Bi0.25Na0.25Ba0.15Sr0.35TiO3 + K0.5Na0.5NbO3 (BNBST + Kx, x = 0, 2, 4, 6, 8, 10) ceramics were constructed to systematically investigate. All BNBST + Kx ceramics exhibited single pseudocubic perovskite structure with high bulk density. High energy storage density Wtotal = 2.3 J/cm3, recoverable energy storage density Wrec = 1.91 J/cm3 and efficiency η = 84% under 117 kV/cm were achieved at x = 4, and the value of 1.91 J/cm3 was superior compared with most Wrec in lead-free bulk ceramics under a relatively low electric field (< 150 kV/cm), while the dielectric temperature stability was boosted to meet wider working window. Moreover, the BNBST + K4 ceramics displayed satisfactory frequency (1–100 Hz), anti-fatigue (1–104 cycle times) and temperature (20–200 °C) dependent energy storage stability, which might be a powerful contender for low-voltage driven ceramic capacitors of high energy-storage density.

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The datasets generated during and/or analyzed during the current work are available from the corresponding author on reasonable request.

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Funding

This work was supported by Graduate Innovation Fund of Jiangxi Province (YC2022-S884).

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Author notes

  1. Wen Zhu and Yizhao Zhou have contributed equally to this work.

Authors and Affiliations

  1. Advanced Ceramic Materials Research Institute, School of Materials Science and Engineering, Jingdezhen Ceramic University, Jingdezhen, 333403, China

    Wen Zhu, Yizhao Zhou & Xiangping Zhang

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  1. Wen Zhu
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Contributions

WZ and YZ: project administration, conceptualization, methodology, writing, contributed equally to the manuscript. XZ: methodology and manuscript revision, assist in data handling.

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Correspondence to Wen Zhu.

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Zhu, W., Zhou, Y. & Zhang, X. Achieving high energy-storage density in K0.5Na0.5NbO3 optimized Bi0.25Na0.25Ba0.15Sr0.35TiO3 relaxor ferroelectric ceramics. J Mater Sci: Mater Electron 34, 1700 (2023). https://doi.org/10.1007/s10854-023-11161-8

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