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Robust deposition of conductive polymer on waste textile assisted by vapor polymerization for flexible zinc-ion hybrid capacitor

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Abstract

Flexible energy storage devices have been applied more and more in recent years, such as wearable electronic products, folding mobile phones, and so on. In this study, through the use of waste face mask (WFM) unique three-layer structure, designed a zinc-ion hybrid capacitor (ZHC), the outer layer of WFM through the vapor phase polymerization method on the surface of WFM uniformly covered with a layer of polypyrrole (PPy), to enhance the conductivity of the material and improve the surface topography. The loading of PPy is then increased by electrodeposition and dopants are introduced to further improve its electrochemical properties. It improves the problem that the conductivity of the active material becomes poor with increasing polymerization time and cannot continue to grow so that the electrochemical and mechanical properties of the electrode can be effectively strengthened. The other pole also through the way of electrodeposition on the surface of Zn deposition. ZHC is assembled using ZnSO4/gelatin as the electrolyte and WFM inner layer as the separator. The assembled ZHC has excellent electrochemical performance, with a mass-specific capacity of 121.5 mAh g−1 at 0.1 A g−1 and an energy density of 97.6 Wh kg−1 at 0.1 A g−1. In addition, the capacity retention rate remains 77.1% after 10,000 charge-discharge cycles. The assembled ZHC allows a small fan or digital watch to function properly. These results indicate that the prepared ZHC can be widely used in reality.

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Funding

This work was supported by the National Natural Science Foundation of China (No. 22265007, 52263016); the Natural Science Foundation of Guangxi Province (No. 2022GXNSFAA035597, 2023GXNSFAA026162); the Project of Department of Science and Technology of Guilin (2020010906).

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  1. Mingyang Lan and Zhanhui Fan have contributed equally to this work.

Authors and Affiliations

  1. Guangxi Colleges and Universities Key Laboratory of Natural and Biomedical Polymer Materials, College of Materials Science and Engineering, Guilin University of Technology, Guilin, 541004, China

    Mingyang Lan, Zhanhui Fan, Chao Yang & Limin Zang

  2. Department of Machine Intelligence and Systems Engineering, Faculty of Systems Science and Technology, Akita Prefectural University, Yurihonjo, 015-0055, Japan

    Jianhui Qiu

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  1. Mingyang Lan
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Contributions

ML: Data curation, Investigation, Writing—original draft. ZF: Data curation, Investigation, Writing—original draft. CY: Resources, Investigation, Validation, Writing—review. JQ: Supervision, Validation. LZ: Conceptualization, Supervision, Investigation, Writing-review, Supervision, Methodology.

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Correspondence to Chao Yang or Limin Zang.

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Lan, M., Fan, Z., Yang, C. et al. Robust deposition of conductive polymer on waste textile assisted by vapor polymerization for flexible zinc-ion hybrid capacitor. J Mater Sci: Mater Electron 34, 1502 (2023). https://doi.org/10.1007/s10854-023-10913-w

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