Skip to main content
Log in

Effect of a urea/IPA-treated PEDOT:PSS hole injection layer in quantum-dot light emitting diodes

  • Published:
Journal of Materials Science: Materials in Electronics Aims and scope Submit manuscript

Abstract

Quantum dot (QD) semiconductor nanocrystals are being considered a competitive contender as the emitting materials of next-generation light-emitting diodes (LEDS) in lighting and display applications. One of ways to improve the performance of a QDs-based device is to develop/modify the layers in the multi-layer structure of the device to have good stability and electrical properties. In this study, urea was selected as a treatment agent for PEDOT: PSS modification as a hole injection layer in QLED. The study found that the performance of a QLEDs with the urea-treated PEDOT:PSS film improved compared to that of a QLEDs with pristine PEDOT:PSS film, and that the performance could further be improved with modifications in the solvent system of PEDOT:PSS with the addition of isopropanol (IPA), resulting in better surface morphology. Consequently, a QLED made of the urea/IPA-treated PEDOT:PSS had a higher performances than those of conventional QLED. Thus, the use of a modified PEDOT:PSS layer in a QLED is very effective in enhancing the injection holes and overall performance of the QLED.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5

Similar content being viewed by others

Data availability

Data are available upon request.

References

  1. J. Cameron, P J. Skabara Mater. Horizons 7, 1759 (2020)

    Article  CAS  Google Scholar 

  2. E. Dauzon, A.E. Mansour, M.R. Niazi, R. Munir, D.-M. Smilgies, X. Sallenave, C. Plesse, F. Goubard, A. Amassian, ACS Appl. Mater. Interfaces 11, 17570 (2019)

    Article  CAS  Google Scholar 

  3. A.L. Efros, L.E. Brus, ACS Nano 15, 6192 (2021)

    Article  CAS  Google Scholar 

  4. H. Elbohy, B. Bahrami, S. Mabrouk, K.M. Reza, A. Gurung, R. Pathak, M. Liang, Q. Qiao, K. Zhu, Adv. Funct. Mater. 29, 6740 (2018)

    Google Scholar 

  5. Z. Liu, L. Wu, J. Qian, J. Peng, R. Liu, Y. Xu, X. Shi, C. Qi, S. Ye, J. Electron. Mater. 50, 2356 (2021)

    Article  CAS  Google Scholar 

  6. F. Louwet, L. Groenendaal, J. Dhaen, J. Manca, J. van Luppen, E. Verdonck, and L. Leenders. Syn. Metals 135–136, 115 (2003)

    Article  Google Scholar 

  7. J. Luo, D. Billep, T. Waechtler, T. Otto, M. Toader, O. Gordan, E. Sheremet, J. Martin, M. Hietschold, D.R.T. Zahn, T. Gessner, J. Mater. Chem. A 1, 7576 (2013)

    Article  CAS  Google Scholar 

  8. A.M. Nardes, R.A.J. Janssen, M. Kemerink, Adv. Funct. Mater. 18, 865 (2008)

    Article  CAS  Google Scholar 

  9. A.J. Olivares, I. Cosme, M.E. Sanchez-Vergara, S. Mansurova, J.C. Carrillo, H.E. Martinez, A. Itzmoyotl, Polymers 11, 1034 (2019)

    Article  CAS  Google Scholar 

  10. H. Shi, C. Liu, Q. Jiang, J. Xu, Adv. Electron. Mater. 1, 17 (2015)

    Google Scholar 

  11. T.C. Nguyen, T.T.T. Can, W.-S. Choi, Sci. Rep. 10, 11075 (2020)

    Article  CAS  Google Scholar 

  12. I. Song, N.Y. Park, G.S. Jeong, J.H. Kang, J.H. Seo, J.Y. Choi, Appl. Surf. Sci. 529, 147176 (2020)

    Article  CAS  Google Scholar 

  13. T. Zhang, C. Shi, C. Zhao, Z. Wu, J. Chen, Z. Xie, D. Ma, ACS Appl. Mater. Interfaces 10, 8148 (2018)

    Article  CAS  Google Scholar 

  14. Y. Wang, M. Wang, P. Wang, W. Zhou, Z. Chen, Q. Gao, M. Shen, J. Zhu, Compos. Comm. 27, 100885 (2021)

    Article  Google Scholar 

  15. Y. Xia, J. Ouyang, J. Mater. Chem. 21, 4927–4936 (2011)

    Article  CAS  Google Scholar 

  16. W. Zhang, X. Bi, X. Zhao, Z. Zhao, J. Zhu, S. Dai, Y. Lu, S. Yang, Org. Electron. 15, 3445 (2014)

    Article  CAS  Google Scholar 

  17. Y. Zhou, S. Mei, J. Feng, D. Sun, F. Mei, J. Xu, X. Cao, RSC Adv. 10, 26381 (2020)

    Article  CAS  Google Scholar 

Download references

Acknowledgements

This work was supported by the Basic Science Research Program through the National Research Foundation Korea (NRF-2018R1D1A1B07048441).

Author information

Authors and Affiliations

Authors

Contributions

DLN: investigation, data analysis, writing. WSC: conceptualization, review & editing, supervision.

Corresponding author

Correspondence to Woon-Seop Choi.

Ethics declarations

Competing interests

The authors declare no competing interests.

Additional information

Publisher’s Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Nguyen, D.L., Choi, WS. Effect of a urea/IPA-treated PEDOT:PSS hole injection layer in quantum-dot light emitting diodes. J Mater Sci: Mater Electron 34, 1064 (2023). https://doi.org/10.1007/s10854-023-10488-6

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1007/s10854-023-10488-6

Navigation