Abstract
Quantum dot (QD) semiconductor nanocrystals are being considered a competitive contender as the emitting materials of next-generation light-emitting diodes (LEDS) in lighting and display applications. One of ways to improve the performance of a QDs-based device is to develop/modify the layers in the multi-layer structure of the device to have good stability and electrical properties. In this study, urea was selected as a treatment agent for PEDOT: PSS modification as a hole injection layer in QLED. The study found that the performance of a QLEDs with the urea-treated PEDOT:PSS film improved compared to that of a QLEDs with pristine PEDOT:PSS film, and that the performance could further be improved with modifications in the solvent system of PEDOT:PSS with the addition of isopropanol (IPA), resulting in better surface morphology. Consequently, a QLED made of the urea/IPA-treated PEDOT:PSS had a higher performances than those of conventional QLED. Thus, the use of a modified PEDOT:PSS layer in a QLED is very effective in enhancing the injection holes and overall performance of the QLED.
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References
J. Cameron, P J. Skabara Mater. Horizons 7, 1759 (2020)
E. Dauzon, A.E. Mansour, M.R. Niazi, R. Munir, D.-M. Smilgies, X. Sallenave, C. Plesse, F. Goubard, A. Amassian, ACS Appl. Mater. Interfaces 11, 17570 (2019)
A.L. Efros, L.E. Brus, ACS Nano 15, 6192 (2021)
H. Elbohy, B. Bahrami, S. Mabrouk, K.M. Reza, A. Gurung, R. Pathak, M. Liang, Q. Qiao, K. Zhu, Adv. Funct. Mater. 29, 6740 (2018)
Z. Liu, L. Wu, J. Qian, J. Peng, R. Liu, Y. Xu, X. Shi, C. Qi, S. Ye, J. Electron. Mater. 50, 2356 (2021)
F. Louwet, L. Groenendaal, J. Dhaen, J. Manca, J. van Luppen, E. Verdonck, and L. Leenders. Syn. Metals 135–136, 115 (2003)
J. Luo, D. Billep, T. Waechtler, T. Otto, M. Toader, O. Gordan, E. Sheremet, J. Martin, M. Hietschold, D.R.T. Zahn, T. Gessner, J. Mater. Chem. A 1, 7576 (2013)
A.M. Nardes, R.A.J. Janssen, M. Kemerink, Adv. Funct. Mater. 18, 865 (2008)
A.J. Olivares, I. Cosme, M.E. Sanchez-Vergara, S. Mansurova, J.C. Carrillo, H.E. Martinez, A. Itzmoyotl, Polymers 11, 1034 (2019)
H. Shi, C. Liu, Q. Jiang, J. Xu, Adv. Electron. Mater. 1, 17 (2015)
T.C. Nguyen, T.T.T. Can, W.-S. Choi, Sci. Rep. 10, 11075 (2020)
I. Song, N.Y. Park, G.S. Jeong, J.H. Kang, J.H. Seo, J.Y. Choi, Appl. Surf. Sci. 529, 147176 (2020)
T. Zhang, C. Shi, C. Zhao, Z. Wu, J. Chen, Z. Xie, D. Ma, ACS Appl. Mater. Interfaces 10, 8148 (2018)
Y. Wang, M. Wang, P. Wang, W. Zhou, Z. Chen, Q. Gao, M. Shen, J. Zhu, Compos. Comm. 27, 100885 (2021)
Y. Xia, J. Ouyang, J. Mater. Chem. 21, 4927–4936 (2011)
W. Zhang, X. Bi, X. Zhao, Z. Zhao, J. Zhu, S. Dai, Y. Lu, S. Yang, Org. Electron. 15, 3445 (2014)
Y. Zhou, S. Mei, J. Feng, D. Sun, F. Mei, J. Xu, X. Cao, RSC Adv. 10, 26381 (2020)
Acknowledgements
This work was supported by the Basic Science Research Program through the National Research Foundation Korea (NRF-2018R1D1A1B07048441).
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DLN: investigation, data analysis, writing. WSC: conceptualization, review & editing, supervision.
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Nguyen, D.L., Choi, WS. Effect of a urea/IPA-treated PEDOT:PSS hole injection layer in quantum-dot light emitting diodes. J Mater Sci: Mater Electron 34, 1064 (2023). https://doi.org/10.1007/s10854-023-10488-6
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DOI: https://doi.org/10.1007/s10854-023-10488-6