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Dielectric and energy storage properties of Ba0.85Ca0.15Zr0.1Ti0.90O3 ceramics with BaO–Na2O–Nb2O5–WO3–P2O5 glass addition

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Abstract

Lead-free Ba0.85Ca0.15Zr0.10Ti0.90O3 (BCZT) ceramic with different BaO–Na2O–Nb2O5–WO3–P2O5 (BNNWP) glass contents, forming (1–x)BCZT–xBNNWP lead-free ceramics (abbreviated as BCZTx; x = 0, 2, 4, 6, and 8wt%) were synthesized using the conventional solid-state processing route. The XRD investigation shows the coexistence of tetragonal and orthorhombic phases in BCZT pure. Likewise, only the tetragonal phase was detected in BCZTx (x = 2–8 wt%) ceramics. The SEM findings indicate that the average grain size decreases as the amount of BNNWP glass additives increases. In addition, BCZT ceramics modified with glass additions showed narrower hysteresis loops and a large electric field. The BCZT4 showed the highest recovered energy density of 0.52 J/cm3 at 135 kV/cm with an energy storage efficiency of 62.4%, which is increased by 6.6 compared to BCZT0 (0.075 J/cm3). The energy density was also calculated using the Landau–Ginzburg–Devonshire (LGD) theory.

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Acknowledgements

The authors gratefully acknowledge the financial support of CNRST, OCP foundation, and the European Union’s Horizon H2020-MSCA-RISE research and innovation actions, ENGIMA and MELON.

Funding

CNRST Morocco, OCP foundation.

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Authors and Affiliations

  1. IMAD-Lab, Cadi Ayyad University, Avenue Abdelkrim El Khattabi, P.B. 549, 40000, Marrakesh, Morocco

    A. Ihyadn, S. Merselmiz, D. Mezzane, A. Alimoussa & M. Amjoud

  2. Condensed Matter Physics Laboratory, University of Picardie Jules Verne, Amiens, France

    D. Mezzane, A. Lahmar, Igor A. Luk’yanchuk & M. El Marssi

  3. Laboratoire Des Sciences Et Métiers de L’ingénieur (LSMI), ENSAM Meknès, Université Moulay Ismail, Meknès, Morocco

    L. Bih

  4. Department of Building Materials, Kyiv National University of Construction and Architecture, Kyiv, 03680, Ukraine

    Igor A. Luk’yanchuk

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All authors certify that they have participated sufficiently in the work to take public responsibility for the content. Furthermore, each author certifies that this work will not be submitted to other journal or published in any other publication before. AI: Investigation, Writing—Original Draft, visualization, and conceptualization; SM: Writing—Review & Editing; DM: Conceptualization, validation, resources, and supervision; LB: Conceptualization, resources, and supervision; AL: Writing—Review and Editing; AA: Software and supervision; MA and IAL: Reviewing and Editing; MEM: Formal analysis and Resources.

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Ihyadn, A., Merselmiz, S., Mezzane, D. et al. Dielectric and energy storage properties of Ba0.85Ca0.15Zr0.1Ti0.90O3 ceramics with BaO–Na2O–Nb2O5–WO3–P2O5 glass addition. J Mater Sci: Mater Electron 34, 1051 (2023). https://doi.org/10.1007/s10854-023-10483-x

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