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Improved energy-storage performance of (1–x)[(Bi0.5Na0.5)0.94Ba0.06]0.98La0.02TiO3–xBi(Mg0.5Zr0.5)O3 ceramics

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Abstract

Lead-free ceramic capacitors have attracted growing demand for energy-storage. Here, (1 − x)[(Bi0.5Na0.5)0.94Ba0.06]0.98La0.02TiO3–xBi(Mg0.5Zr0.5)O3 ((1 − x)BNBLT–xBMZ, x = 0–0.3) ceramics were synthesized via citrate combustion technology. The nanoscale domains are observed and slim hysteresis loops are realized as addition of BMZ. The recoverable energy-storage density (Wre of 2.6 J/cm3) and efficiency (η of 81%) are obtained in 0.8BNBLT-0.2BMZ sample under 160 kV/cm. The energy-storage performances of 0.8BNBLT-0.2BMZ sample show excellent frequency stability (Wre varies 4% and η varies 2.5% at 5 Hz to 100 Hz). More importantly, Wre increases from 1.02 to 1.36 J/cm3 with increasing temperature from 20 to 120 ºC, and η increases from 80 to 97% at 100 kV/cm, which demonstrates that it is the promising candidate for high temperature energy-storage devices.

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The datasets generated and analysed during the current study are available from the corresponding author on reasonable request.

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Authors and Affiliations

  1. School of Mechatronics and Information Engineering, Chongqing College of Humanities, Science and Technology, Chongqing, 401524, China

    Hua Qiang, Xiaoyang Wang & Lingyun Deng

  2. School of Materials and Energy, Southwest University, Chongqing, 400715, China

    Zunping Xu

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  1. Hua Qiang
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  2. Xiaoyang Wang
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  3. Lingyun Deng
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  4. Zunping Xu
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Contributions

The corresponding author ZX is responsible for ensuring that the descriptions are accurate and agreed by all authors. The role(s) of all authors is listed as follows, HQ: Resource and writing original draft, XW: Experiment and Investigation, LD: Investigation and resource, ZX: Review & editing.

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Correspondence to Zunping Xu.

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Qiang, H., Wang, X., Deng, L. et al. Improved energy-storage performance of (1–x)[(Bi0.5Na0.5)0.94Ba0.06]0.98La0.02TiO3–xBi(Mg0.5Zr0.5)O3 ceramics. J Mater Sci: Mater Electron 34, 108 (2023). https://doi.org/10.1007/s10854-022-09610-x

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  • DOI: https://doi.org/10.1007/s10854-022-09610-x

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