Abstract
MgNb2O6- x wt% Ti2Nb10O29 (x = 0, 2, 4, 6, 8, 10) microwave dielectric ceramics with near zero temperature coefficient of resonance frequency τf were prepared by the solid-state reaction technique. The effects of Ti2Nb10O29 incorporation on the microstructure and dielectric properties of MgNb2O6 were investigated to probe the formation and sintering behavior of each phase. The results show that the appropriate Ti2Nb10O29 addition can promote the sintering of MgNb2O6 and improve the density of the ceramics. The quality factor Q × f was decreased with the increasing of Ti2Nb10O29, but, at the same time, the dielectric constant εr and the temperature coefficient of resonance frequency τf were improved, which is consistent with the theoretical calculation. When the addition amount x is equal to 4, the ceramic sample has the best microwave dielectric properties after sintering at 1280 °C for 4 h: εr = 21.72, Q × f = 76,850 GHz, τf = -9.6 × 10–6/°C.
Similar content being viewed by others
Data availability
The datasets generated during and/or analyzed during the current study are available from the corresponding author on reasonable request.
References
O. Hitoshi, J Ceram Soc Jpn. 113(1323), 703–711 (2005)
H Yang, Q Zhang, J Wang, Y You and W Huang, J Chin Chem Soc-Taip. 31,965–973+980(2003)
Lee, H. Jong, Kim, I. Tae, Hong and K. Sun, Jpn J Appl Phys. 36, L1318-L1320(1997).
Anatolii, Belous, Oleg, Ovchar, Bostjan, Jancar and Jana, J Eur Ceram Soc. 27, 2933–2936(2007).
C. Liang, Huang, K. Hau and Chiang, Mat Sci Eng A-Struct. 474, 243–246 (2008)
C. Hsing, H. Su, C. Fang, T. Seng, C. Liang, Huang, Jpn J Appl Phys. 44, 8043–8043 (2005)
Z.Q. Tian, L. Lin, J Mater Sci. 20, 867–871 (2009)
D. Pukazhselvan, N.B. Selvaraj, I. Bdikin, R.S.S. Saravanan, S.K. Jakka, M.J. Soares, D.P. Fagg, Appl Surf Sci. 424, 127–131 (2017)
C.M. Cheng, Y.C. Chen, C.F. Yang, C.C. Chan, J Electroceram. 18, 155–160 (2007)
S. Yu, B. Tang, S. Zhang, X. Zhou, Mater Lett. 80, 124–126 (2012)
C.H. Wu, Y.D. Hu, S.X. Bao, G. Wang, P.B. Jiang, J. Chen, Z.Z. Duan, W.H. Deng, Rsc Adv. 10, 29835–29842 (2020)
S.H. Wu, G.Q. Wang, Y.S. Zhao, Hao, J Eur Ceram Soc. 23, 2565–2568 (2003)
W. M. Gamal, A. A. H. El-Bassuony, R. S. Hafez and H. K. Abdelsalam, JOM. (2022).
A.A.H. El-Bassuony, W.M. Gamal, H.K. Abdelsalam, J Mater Sci-Mater El. 33, 16219–16235 (2022)
B.W. Hakki, P.D. Coleman, IEEE Trans. Microw. Theory Tech. 8, 402–410 (1996)
Y. Zhang, X. Jiang, S. Ding, T. Song, J Mater Sci-Mater El. 32, 12661–12670 (2021)
C.L. Pan, C.H. Shen, P.C. Chen, T.C. Tan, J Alloy Compd. 503, 365–369 (2010)
Y.Z. Hao, H. Yang, G.H. Chen, Q.L. Zhang, J Alloy Compd. 552, 173–179 (2013)
M. Du, R.L. Opila, J Appl Phys. 85, 1496–1502 (1999)
S.S.N. Murthy, A. Paikaray, N. Arya, J Chem Phys. 102, 8213–8220 (1995)
Z.W. Zhang, L. Fang, H.C. Xiang, M.Y. Xu, Y. Tang, H.L. Jantunen, C.C. Li, Ceram Int. 45, 10163–10169 (2019)
S.J. Penn, N.M. Alford, A. Templeton, X.R. Wang, M.S. Xu, M. Reece, K. Schrapel, J Am Ceram Soc. 80, 1885–1888 (1997)
I.M. Reaney, D. Iddles, J Am Ceram Soc. 89, 2063–2072 (2006)
L.Z. Zhang, H.X. Lin, X.Y. Zhao, X.G. Yao, S.H. Jiang, F. He, B.T. Li, L. Luo, J Alloy Compd. 649, 254–260 (2015)
Acknowledgements
This work is supported by the National Natural Science Foundation of China (No. 51767010)
Funding
This article was funded by National Natural Science Foundation of China, 51767010, Zongyang Shen.
Author information
Authors and Affiliations
Contributions
JH—Conceptualization, methodology, writing—original draft. YL—project administration. KL—resources, data curation. YS—visualization, writing—review and editing. ZS—data curation. ZW—conceptualization, validation.
Corresponding author
Ethics declarations
Conflict of interest
The authors declare that they have no conflict of interest.
Additional information
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Huang, J., Li, Y., Li, K. et al. Effect of adding Ti2Nb10O29 on the dielectric properties of MgNb2O6 microwave dielectric ceramics. J Mater Sci: Mater Electron 33, 27014–27021 (2022). https://doi.org/10.1007/s10854-022-09365-5
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10854-022-09365-5