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Correlation between phase structure and polarization of Mg doped (Ba0.98Li0.02)TiO3 energy storage ceramics

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Abstract

Mg doped (Ba0.98Li0.02)TiO3 energy storage ceramics with antiferroelectric-like double hysteresis loops were prepared using solid-state reaction method. XRD patterns indicated that tetragonal phase structure of the pure (Ba0.98Li0.02)TiO3 ceramic was destroyed and the orthorhombic phase structure appeared with Mg doping. The ratio of orthorhombic/tetragonal phase increased with Mg content increasing, and the value of polarization was in direct proportion to the ratio of orthorhombic/tetragonal phase. The breakdown strength of (Ba0.98Li0.02)(MgxTi1−x)O3 ceramics was improved from 60.97 kV/cm at x = 0 to 103.66 kV/cm at x = 0.04. The optimum energy storage properties of (Ba0.98Li0.02)(MgxTi1−x)O3 ceramics were obtained with energy storage density of 0.76 J/cm3 at 102.5 kV/cm when x = 0.04, which is nearly 2.3 times larger than the pure (Ba0.98Li0.02)TiO3 ceramic, and the energy storage efficiency was improved from 64 to 87%.

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Data availability

The datasets generated during and/or analyzed during the current study are available from the corresponding author on reasonable request.

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Funding

This work was supported by (National Natural Science Foundation of China) [Grant No. (51702024)].

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Authors and Affiliations

  1. School of Materials Science and Engineering, Jiangsu Collaborative Innovation Center of Photovolatic Science and Engineering, Changzhou University, Changzhou, 213164, Jiangsu, China

    Gui-wei Yan, Qing-qing Liu, Bi-jun Fang & Zhi-hui Chen

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  1. Gui-wei Yan
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Contributions

All authors contributed to the study conception and design. Material preparation, data collection and analysis were performed by GY, QL, BF and ZC. The first draft of the manuscript was written by GY and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.

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Correspondence to Bi-jun Fang or Zhi-hui Chen.

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Yan, Gw., Liu, Qq., Fang, Bj. et al. Correlation between phase structure and polarization of Mg doped (Ba0.98Li0.02)TiO3 energy storage ceramics. J Mater Sci: Mater Electron 33, 20981–20991 (2022). https://doi.org/10.1007/s10854-022-08903-5

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