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Effect of configurational entropy on dielectric properties of high-entropy perovskite oxides (Ce0.5,K0.5)x[(Bi0.5,Na0.5)0.25Ba0.25Sr0.25Ca0.25]1−xTiO3

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Abstract

A new kind of high-entropy perovskite oxides (Ce,K)x[(Bi,Na)BaSrCa]1−xTiO3 (x-CKBNBSCTO) were synthesized by using a traditional solid-state reaction method and the dependence of the properties of samples on the content x was also explored. Microstructure analyses found that the most homogeneous particles were obtained when x reached 0.2. The highest dielectric properties can be detected when each element is equal, and the highest dielectric constant and the lowest dielectric loss are captured with the values of 535 and 0.04, respectively. Also, the energy storage is explored, showing a high energy storage efficiency of 85% when x is 0.08.

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Data availability

We confirm that material described in the manuscript, including all relevant raw data, will be freely available to any researcher wishing to use them for non-commercial purposes, without breaching participant confidentiality. The datasets generated during and/or analyzed during the current study are available from the corresponding author on reasonable request.

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Acknowledgements

This work was supported by National Natural Science Foundation of China (No. 51972048) and the Natural Science Foundation of Hebei Province (No. E2018501042).

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Authors and Affiliations

  1. School of Materials Science and Engineering, Northeastern University, Shenyang, 110819, China

    Junjie Zhou, Pengfei Li, Xiaoyan Zhang & Jinhua Yan

  2. School of Resources and Materials, Northeastern University at Qinhuangdao, Qinhuangdao, 066004, China

    Pengfei Li & Xiaoyan Zhang

  3. College of Metallurgy and Energy, North China of Science and Technology, Tangshan, 063210, China

    Xiwei Qi

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  1. Junjie Zhou
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Contributions

All authors contributed to the study conception and design. Material preparation, data collection and analysis were performed by JZ, the first draft of the manuscript was written by JZ and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.

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Correspondence to Pengfei Li or Xiwei Qi.

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Zhou, J., Li, P., Zhang, X. et al. Effect of configurational entropy on dielectric properties of high-entropy perovskite oxides (Ce0.5,K0.5)x[(Bi0.5,Na0.5)0.25Ba0.25Sr0.25Ca0.25]1−xTiO3. J Mater Sci: Mater Electron 33, 20721–20730 (2022). https://doi.org/10.1007/s10854-022-08882-7

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