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Lightweight poly(m-phenylene isophthalamide)/CF/GO@Fe3O4 composites for enhanced shielding of electromagnetic pollution

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Abstract

In this work, ferroferric oxide (Fe3O4) microspheres with a diameter of ~ 150 nm were in situ grown on the surface of graphene oxide (GO) to obtain GO@Fe3O4 hybrids. Then, novel PMIA/CF/GO@Fe3O4 electromagnetic shielding composites have been developed with a simple and efficient paper-making method using poly(m-phenylene isophthalamide) (PMIA) fibers as matrix and carbon fiber (CF) and GO@Fe3O4 as fillers. Due to the introduction of GO@Fe3O4 and a large number of voids into the materials, the obtained PMIA/CF/GO@Fe3O4 composites exhibit good magnetic sensitivity and low density. Besides, the obtained PMIA/CF/GO@Fe3O4 composites with 10 wt% GO@Fe3O4 loading shows outstanding EMI-shielding effectiveness (EMI SE) of 42.55–46.98 dB at 8–12 GHz, and as the content of GO@Fe3O4 increases to 30 wt%, the EMI SE increases to 55.22 to 60.23 dB. The EMI SE of the PMIA/CF/GO@Fe3O4 composites is far more than the target value (20 dB) required by practical application. Thus, it provides a path to obtain a new class of high-performance and lightweight PMIA-based composites for enhanced shielding of electromagnetic pollution.

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Acknowledgements

The authors wish to thank for the Opening Project of Material Corrosion and Protection Key Laboratory of Sichuan province (2019CL04) and Sichuan University Students Innovation and Entrepreneurship Training Programs (S202010622036).

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Author notes

  1. Hongbo Hou and Zejun Pu have contributed equally to this work.

Authors and Affiliations

  1. College of Materials Science and Engineering, Material Corrosion and Protection Key Laboratory of Sichuan Province, Sichuan University of Science & Engineering, Zigong, 643000, China

    Hongbo Hou, Zejun Pu, Xueyu Liu, Xianyong Li, Xiaohang He, Jingyue Liu & Jiachun Zhong

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  1. Hongbo Hou
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  2. Zejun Pu
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  3. Xueyu Liu
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  4. Xianyong Li
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  7. Jiachun Zhong
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HH and ZP contributed equally to this work, and they are the co-first author. Besides, all the authors approved the final version of the manuscript.

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Correspondence to Zejun Pu.

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Hou, H., Pu, Z., Liu, X. et al. Lightweight poly(m-phenylene isophthalamide)/CF/GO@Fe3O4 composites for enhanced shielding of electromagnetic pollution. J Mater Sci: Mater Electron 32, 21441–21449 (2021). https://doi.org/10.1007/s10854-021-06652-5

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