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Influences of (LiCe) co-doping on the structure and properties of Na0.15Bi2.85Ti0.7Nb1.3O9 piezoceramics

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Abstract

Aurivillius-type piezoceramics, Na0.15−xLixBi2.85−x CexTi0.7Nb1.3O9 (NBTN-LC100x; x = 0, 0.02, 0.04, 0.06), were fabricated by the solid-state reaction method. The crystal structure, surface microstructure, and electrical properties of NBTN-LC100x ceramics were studied systematically. The XRD revealed that the (LiCe) co-doping induced lattice distortion and the orthogonality of ceramics were weakened. The grain size decreased obviously from 23.1 to 9.1 µm and the Curie temperature (TC) decreased from 877 to 853 °C as the increase of (LiCe) content. As x = 0.04, the NBTN-LC100x (NBTN-LC4) ceramics had the best performance, its TC, tanδ at 500 °C, EC, and Pr were 861 °C, 7.61%, 62 kV/cm, and 3.4 µC/cm2, respectively. The piezoelectric property was enhanced significantly and optimal d33 value was about 20.7 pC/N at x = 0.04 for NBTN-LC100x ceramics. In addition, the NBTN-LC4 ceramics possessed a good thermal stability after annealing at 850 °C for 2 h. The high d33, high TC, low tanδ, good thermal stability of NBTN-LC4 ceramics make it is potential candidate in high-temperature electronic devices.

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Authors and Affiliations

  1. Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of Education, School of Materials Science and Engineering, Tianjin University, Tianjin, 300350, China

    Pengfei Zhang, Weibing Ma, Shenghui Wang, Jingdong Guo, Jingnan Hong, Ruiqing Ba, Xinghui He & Jing Li

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  1. Pengfei Zhang
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  2. Weibing Ma
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  3. Shenghui Wang
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  4. Jingdong Guo
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  5. Jingnan Hong
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  7. Xinghui He
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  8. Jing Li
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Contributions

PZ: completed the experiment and manuscript. WM: completed the revision of the manuscript. SW, JG: provided assistances for data analysis. JH, RB, XH, and JL: provided assistances for drawing and testing.

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Correspondence to Weibing Ma.

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Zhang, P., Ma, W., Wang, S. et al. Influences of (LiCe) co-doping on the structure and properties of Na0.15Bi2.85Ti0.7Nb1.3O9 piezoceramics. J Mater Sci: Mater Electron 32, 8450–8459 (2021). https://doi.org/10.1007/s10854-021-05464-x

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  • DOI: https://doi.org/10.1007/s10854-021-05464-x

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