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Low temperature sintered of Ba3MgNb2O9 ceramics with high quality factor via B-site oxide precursor method

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Abstract

B-site oxide precursor method was utilized to synthesize Ba3MgNb2O9 ceramics. The effects of sintering temperature on phase composition of Ba3MgNb2O9 ceramics was evaluated by the X-ray diffraction. Experimental results indicated that all prepared Ba3MgNb2O9 ceramics exhibited 1:2 ordered hexagonal structure. The second phase Ba5Nb4O15 can emerge in all ceramics due to the decrease of activation energy of reaction, leading to the splitting of Eg(O) vibration mode in the Raman spectra. In addition, lattice parameters of 1:2 ordered phase were obtained from the refinement of XRD patterns. The maximum value of c/a ratio occurred at 1475 °C, meanwhile the ceramics showed the highest 1:2 ordered degree and excellent Q × f. It was also found that the uniform grain-size distribution of Ba3MgNb2O9 powder were important factors for preparing dense Ba3MgNb2O9 ceramics. Moreover, B-site oxide precursor method can not only effectively lower the densification temperature from 1650 to 1475 °C, but also increase the quality factor (Q × f) by about 90.8%, i.e., from 55,277 to 105,467 GHz.

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Acknowledgement

This work is supported by the Department of Education’s Production-Study-Research combined innovation Funding-“Blue fire plan (Huizhou)” (No. CXZJHZ201733), and Natural Science Foundation of Shandong Province (ZR2018LE003).

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Authors and Affiliations

  1. College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, People’s Republic of China

    He Wang, Renli Fu & Yunan Liu

  2. College of Microtechnology & Nanotechnology, Qingdao University, Qingdao, 266071, People’s Republic of China

    Xuhai Liu

  3. Key Laboratory of Processing and Testing Technology of Glass & Functional Ceramics of Shandong Province, School of Materials Science and Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan, People’s Republic of China

    Yue Xu

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  1. He Wang
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  2. Renli Fu
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Correspondence to Renli Fu.

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Wang, H., Fu, R., Liu, X. et al. Low temperature sintered of Ba3MgNb2O9 ceramics with high quality factor via B-site oxide precursor method. J Mater Sci: Mater Electron 31, 20245–20254 (2020). https://doi.org/10.1007/s10854-020-04544-8

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  • DOI: https://doi.org/10.1007/s10854-020-04544-8

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