Abstract
This study aimed at developing a good co-firing compatibility between the completely self-developed low-εr and middle-εr LTCC materials. To evaluate the co-firing results, the sintering dynamics, shrinkage behavior, chemical compatibility, three-dimensional contour, and microstructure of the co-fired composites were analyzed qualitatively and quantitatively. The results showed that the CaTiO3-TiO2 ceramic mixed with 50 wt% glass additives tended to have a good co-firing compatibility with low-εr composite, especially when the particle size of the CaTiO3–TiO2 ceramic was controlled at 3.04 µm. The composite co-fired with low-εr material at 875 °C for 20 min presented the best co-firing matching characteristic with an ideal chemical compatibility and the smallest height difference (64.73 µm) along the diameter of the samples. Besides, the sintering dynamics process of the hetero-laminates was simulated for a better understanding of the co-firing process. The simulated schematic was adopted to interpret the co-firing behavior of the hetero-laminates and the crucial factors in achieving a good co-firing compatibility.
Similar content being viewed by others
References
M.T. Sebastian, H. Jantunen, Int. Mater. Rev. 53, 2 (2013)
H. Xiang, C. Li, H. Jantunen et al., ACS Sustain. Chem. Eng. 6, 5 (2018)
A. Hajian, D. Müftüoglu, T. Konegger et al., Composites B 157, 14–23 (2019)
J.J. Bian, Y.R. Xie, J. Eur. Ceram. Soc.. 38, 7 (2018)
N. Joseph, J. Varghese, T. Siponkoski et al., ACS Sustain. Chem. Eng. 4, 10 (2016)
F. Liu, X. Huang, J. Qu et al., J. Non-Cryst. Solids 481, 261–275 (2018)
I.J. Induja, M.R. Varma, M.T. Sebastian, J. Mater. Sci.: Mater. Electron. 28, 19 (2017)
A. Sasidharanpillai, C.H. Kim, C.H. Lee et al., ACS Sustain. Chem. Eng. 6, 5 (2018)
M.T. Sebastian, H. Wang, H. Jantunen, Curr. Opin. Solid State Mater. Sci. 20, 3 (2016)
Y.J. Choi, J.H. Park, W.J. Ko et al., J. Am. Ceram. Soc. 89, 2 (2006)
Y. Higuchi, Y. Sugimoto, J. Harada et al., J. Eur. Ceram. Soc. 27, 8–9 (2007)
W.B. Lim, Y.S. Cho, Y.J. Seo, Al, J. Eur. Ceram. Soc. 29, 4 (2009)
L. Ren, X. Luo, L. Hu et al., J. Eur. Ceram. Soc. 37, 2 (2017)
L. Ren, H. Zhou, X. Li et al., J. Alloys Compds. 646, 780–786 (2015)
L. Ren, X. Luo, Y. Xia et al., Int. J. Appl. Ceram. Technol. 16, 1 (2019)
H. Ren, S. Jiang, M. Dang et al., J. Alloys Compds. 740, 1188–1196 (2018)
M.K. Zitani, T. Ebadzadeh, S. Banijamali et al., J. Non-Cryst. Solids. 487, 65–71 (2018)
G. Chen, Z. Liu, M. Ma et al., Ceram. Int. 44, 11030–11038 (2018)
J. Hao, F.Z. Yao, Q. Yuan et al., J. Am. Ceram. Soc. 103, 1 (2019)
M. Liu, H. Zhou, X. Xu et al., J. Mater. Sci.: Mater. Electron. 24, 10 (2013)
X. Luo, L. Ren, Y. Xia et al., Ceram. Int. 43, 9 (2017)
D. Zhou, L.-X. Pang, D.-W. Wang et al., J.Mater. Chem. C 5, 38 (2017)
Y. Li, Y. Xie, R. Xie et al., J. Alloys Compds. 737, 255–262 (2018)
M.T. Sebastian, R. Ubic, H. Jantunen, Int. Mater. Rev. 60, 7 (2015)
L. Ren, X. Luo, H. Zhou, J. Am. Ceram. Soc. 101, 9 (2018)
Acknowledgements
This research was financed by the Key R&D project of Shandong Province (Public welfare projects, 2017GGX20126), the Project of Shandong Province Higher Educational Science and Technology Program (J17KA021) and the Young Teacher Development Support Plan of Shandong University of Technology (201418).
Author information
Authors and Affiliations
Corresponding author
Ethics declarations
Conflict of interest
The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
Additional information
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
About this article
Cite this article
Ren, L., Zhang, M. & Zhou, H. Co-firing compatibility of LTCC hetero-laminates with low and middle permittivity. J Mater Sci: Mater Electron 31, 12282–12291 (2020). https://doi.org/10.1007/s10854-020-03773-1
Received:
Revised:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10854-020-03773-1