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A facile one-pot method to prepare nitrogen and fluorine co-doped three-dimensional graphene-like materials for supercapacitors

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Abstract

Nitrogen and fluorine co-doped three-dimensional(3D) graphene-like material, MP-700, is successfully prepared using a one-pot method by directly pyrolyzing melamine and PTFE in N2 flow. This 3D graphene-like material has a high specific surface area (1309 m2 g−1) and the N and F contents are is 19.03 and 0.41 at.%, respectively. Furthermore, it shows the high specific capacitance of 230 F g−1 at 0.5 A g−1; and exhibits long-term stability. After 10,000 cycles, the capacitance retention rate is 86.3% at 20 A g−1, which has a good prospect in the electrode materials of supercapacitors.

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Acknowledgements

We gratefully acknowledge the financially supported by the National Science Foundation of China (51761006, 51671062, 51801041), the National Key Research and Development Program of China (2018YFB1502103), the National Science Foundation of Guangxi Province (2018JJA160046, AD17195073, 2017AD23029, 2017JJB150085) and Guangxi Bagui Scholar Foundation.

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  1. Guangxi Key Laboratory of Information Material, Guangxi Collaborative Innovation Center of Structure and Property for New Energy and Materials, School of Material Science and Engineering, Guilin University of Electronic Technology, Guilin, 541004, People’s Republic of China

    Diancheng Duan, Fang Hu, Jiaojun Ma, Hongliang Peng, Kexiang Zhang, Pengru Huang, Hailiang Chu, Xiangcheng Lin, Shujun Qiu, Siyue Wei, Fen Xu & Lixian Sun

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  1. Diancheng Duan
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Correspondence to Hongliang Peng or Lixian Sun.

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Duan, D., Hu, F., Ma, J. et al. A facile one-pot method to prepare nitrogen and fluorine co-doped three-dimensional graphene-like materials for supercapacitors. J Mater Sci: Mater Electron 30, 19505–19512 (2019). https://doi.org/10.1007/s10854-019-02316-7

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