Abstract
In this paper, we report a top-gate amorphous In–Al–Zn–O (a-IAZO) thin film transistor (TFT) based on dip-coated poly(methyl methacrylate) (PMMA) dielectric layer and investigate PMMA thickness influence on a-IAZO TFT performance. A thinner PMMA gate dielectric can cumulate more charges per unit area and induce more electron carriers, resulting in increasing of on-state current of TFT. Moreover, it is found that a TFT with the thinner PMMA gate dielectric contains less trap states at a-IAZO/PMMA interface due to decreased surface roughness with thinner PMMA dielectric, which is essential for reducing the capture of electron carriers in the process of electron transport. Therefore, the on/off current ratio (Ion/off), saturated mobility (μsat) and subthreshold gate swing (SS) of device improved with the PMMA thickness decreased from 610 to 280 nm. Furthermore, experimental results show that the PMMA thickness plays an important role on controlling the threshold voltage (Vth) and adjusting the operating mode of device, thus influencing on the power dissipation. Overall, the TFT with a 390-nm-thick PMMA dielectric layer exhibits the adequate operating mode (enhancement mode) and the high electrical performance (a high μsat of 21.42 cm2/Vs, a small SS of 0.46 V/decade, a close-to-zero Vth of 0.12 V, and Ion/off of more than104).
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K. Normura, H. Ohta, A. Takagi, M. Hirano, H. Hosono, Room-temperature fabrication of transparent flexible thin-film transistors using amorphous oxide semiconductors. Nature 432, 488–492 (2004)
S. Yang, D.-H. Cho, M.K. Ryu, S.-H.K. Park, C.-S. Hwang, J. Jang, J.K. Jeong, High-performance Al–Sn–Zn–In–O thin-film transistors: impact of passivation layer on device stability. IEEE Electron Device Lett. 31, 144–146 (2010)
J.H. Jeon, Y.H. Hwang, B.S. Bae, H.L. Kwon, H.J. Kang, Addition of aluminum to solution processed conductive indium tin oxide thin film for an oxide thin film transistor. Appl. Phys. Lett. (2010). https://doi.org/10.1063/1.3442482
D.C. Paine, B. Yaglioglu, Z. Beiley, S. Lee, Amorphous IZO-based transparent thin film transistors. Thin Solid Films 516, 5894–5898 (2008)
W. Lim, Y.L. Wang, F. Ren, D.P. Norton, I.I. Kravchenko, J.M. Zavada, S.J. Pearton, Indium zinc oxide thin films deposited by sputtering at room temperature. Appl. Surf. Sci. 254, 2878–2881 (2008)
J.I. Song, J.S. Park, H. Kim, Y.W. Heo, J.H. Lee, J.J. Kim, Transparent amorphous indium zinc oxide thin-film transistors fabricated at room temperature. Appl. Phys. Lett. (2007). https://doi.org/10.1063/1.2430917
W.W. Xia, G.D. Xia, G.S. Tu, X. Dong, S. Wang, R. Liu, Sol-gel processed high-k aluminum oxide dielectric films for fully solution-processed low-voltage thin-film transistors. Ceram. Int. 44, 9125–9131 (2018)
J.Y. Kwon, J.S. Jung, K.S. Son, K.H. Lee, J.S. Park, T.S. Kim, J.S. Park, R. Choi, J.K. Jeong, B. Koo, S.Y. Lee, The impact of gate dielectric materials on the light-induced bias instability in Hf-In-Zn-O thin film transistor. Appl. Phys. Lett. (2010). https://doi.org/10.1063/1.3513400
G. Jiang, A. Liu, G.X. Liu, C.D. Zhu, Y. Meng, B. Shin, E. Fortunato, R. Martins, F. Shan, Solution-processed high-k magnesium oxide dielectrics for low-voltage oxide thin-film transistors. Appl. Phys. Lett. 97, 183503-1–183503-3 (2010)
C.X. Fan, A. Liu, Y. Meng, Z.D. Guo, G.X. Liu, F.K. Shan, Solution-processed SrOx-gated oxide thin-film transistors and inverters. IEEE Trans. Electron Devices 64, 4137–4143 (2017)
J. Kim, S. Choi, J.-W. Jo, S.K. Park, Y.-H. Kim, Solution-processed lanthanum-doped Al2O3 gate dielectrics for high-mobility metal-oxide thin-film transistors. Thin Solid Films 660, 814–818 (2018)
J.B. Kim, C. Fuentes-Hernandez, B. Kippelen, High-performance InGaZnO thin-film transistors with high-k amorphous Ba0.5Sr0.5TiO3 gate insulator. Appl. Phys. Lett. (2008). https://doi.org/10.1063/1.3054335
M.R. Shijeesh, A.C. Saritha, M.K. Jayaraj, Investigations on the reasons for degradation of zinc tin oxide thin film transistor on exposure to air. Mat. Sci. Semicon. Proc. 74, 116–121 (2018)
S.I.L. Kim, J.-S. Park, C.J. Kim, J.C. Park, I. Song, Y.S. Park, High reliable and manufacturable gallium indium zinc oxide thin-film transistors using the double layers as an active layer. J. Electrochem. Soc. 156, H184–H187 (2009)
A. Facchetti, M.H. Yoon, T.J. Marks, Gate dielectrics for organic field-effect transistors: new opportunities for organic electronics. Adv. Mater. 17, 1705–1725 (2005)
J.-A. Cheng, C.-S. Chuang, M.-N. Chang, Y.-C. Tsai, H.-P. Shieh, Controlable carrier density of pentacene field-effect transistors using polyacrylates as gate dielectrics. Org. Electron. 9, 1069–1075 (2008)
H. Faber, M. Burkhardt, A. Jedaa, D. Kalblein, H. Klauk, M. Halik, Low-temperature solution-processed memory transistors based on zinc oxide nanoparticles. Adv. Mater. 21, 3099–3104 (2009)
S. Bang, S. Lee, S. Jeon, S. Kwon, W. Jeong, H. Kim, I. Shin, H.J. Chang, H.-H. Park, H. Jeon, Al2O3 buffer in a ZnO thin film transistor with poly-4-vinylphenol dielectric. Semicond. Sci. Technol. (2009). https://doi.org/10.1088/0268-1242/24/2/025008
H.F. Pu, G.F. Li, J.H. Feng, B.Y. Liu, Q. Zhang, Amorphous indium zinc oxide thin film transistors with poly-4-vinylphenol gate dielectric layers. Semicond. Sci. Technol. (2011). https://doi.org/10.1088/0268-1242/26/9/095004
I. Karteri, S. Karatas, A.A. Al-Ghamdi, F. Yakuphanoglu, The electrical characteristics of thin film transistors with graphene oxide and organic insulators. Synth. Met. 199, 241–245 (2015)
C.J. Chiu, Z.W. Pei, S.P. Chang, S.J. Chang, Influence of weight ratio of poly(4-vinylphenol) insulator on electronic properties of InGaZnO thin-film transistors. J. Nanomater. 2012, 1–7 (2012)
H.-C. Lai, B.-J. Tzeng, Z. Pei, C.-M. Chen, C.-J. Huang, Ultra-flexible amorphous indium-gallium-zinc oxide (a-IGZO) thin film transistor. SID Symp. Dig. Tech. Pap. 43, 764–767 (2012)
S.-W. Jung, J.-S. Choi, J.H. Park, J.B. Koo, C.W. Park, B.S. Na, J.-Y. Oh, S.C. Lim, S.S. Lee, H.Y. Chu, Oxide semiconductor-based flexible organic/inorganic hybrid thin-film transistors fabricated on polydimethylsiloxane elastomer. J. Nanosci. Nanotechnol. 16, 2752–2755 (2016)
Y.H. Zhang, M.Z. Xia, L.H. Li, D.X. Long, Review of flexible and transparent thin-film transistors based on zinc oxide and related materials. Chin. Phys. B 26, 1–17 (2017)
N.B. Ukah, J. Granstrom, R.R. Sanganna Gari, G.M. King, S. Guha, Low-operating voltage and stable organic field-effect transistors with poly(methyl methacrylate) gate dielectric solution deposited from a high dipole moment solvent. Appl. Phys. Lett. (2011). https://doi.org/10.1063/1.3669696
M. Harris, H.A. Macleod, S. Ogura, E. Pelletier, B. Vidal, The relationship between optical inhomogeneity and film structure. Thin Solid Films 57, 173–178 (1979)
T.-S. Huang, Y.-K. Su, P.-C. Wang, Study of organic thin film transistor with polymethylmethacrylate as a dielectric layer. Appl. Phys. Lett. (2007). https://doi.org/10.1063/1.2775333
V.K. Singh, B. Mazhari, Impact of scaling of dielectric thickness on mobility in top-contact pentacene organic thin film transistors. J. Appl. Phys. (2012). https://doi.org/10.1063/1.3681809
G.W. Hyung, J. Park, J.-X. Wang, H.W. Lee, Z.-H. Li, J.-R. Koo, S.J. Kwon, E.-S. Cho, W.Y. Kim, Y.K. Kim, Amorphous indium gallium zinc oxide thin-film transistors with a low-temperature polymeric gate dielectric on a flexible substrate. Jpn. J. Appl. Phys. (2013). https://doi.org/10.7567/JJAP.52.071102
W. Ye, J.P. Deng, X.F. Wang, L. Cui, Effect of thickness of Bi1.5Zn1.0Nb1.5O7 gate insulator on performance of ZnO based thin film transistors. Appl. Surf. Sci. 390, 831–837 (2016)
X.W. Ding, J.H. Zhang, W.M. Shi, H. Ding, H. Zhang, J. Li, X.Y. Jiang, Z.L. Zhang, C.Y. Fu, Effect of gate insulator thickness on device performance of InGaZnO thin-film transistors. Mat. Sci. Semicon. Proc. 29, 326–330 (2015)
A.H. Chen, H.T. Cao, H.Z. Zhang, L.Y. Liang, Z.M. Liu, Z. Yu, Q. Wan, Influence of the channel layer thickness on electrical properties of indium zinc oxide thin-film transistor. Microelectron. Eng. 87, 2019–2023 (2010)
Acknowledgements
This research was supported by National Natural Science Foundation of China (Grant number 61504031), Science and Technology Foundation of GuiZhou Province, China [Grant number LH(2014)7389], Youth’s growth Foundation of Education Department of GuiZhou Province, China [Grant number (2016)155], Special and Key Laboratory of Guizhou Provincial Higher Education for Photoelectric information Analysis and Processing, China [Grant number KY(2016)003]. We thank Prof. Q. Zhang for valuable suggestions and he guidance for this research.
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Yue, L., Meng, F., Ren, D. et al. Top-gate In–Al–Zn–O thin film transistor based on organic poly(methyl methacrylate) dielectric layer. J Mater Sci: Mater Electron 30, 11976–11983 (2019). https://doi.org/10.1007/s10854-019-01548-x
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DOI: https://doi.org/10.1007/s10854-019-01548-x