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Excellent thermal stability and low dielectric loss of (1 − x)BaTiO3 –xBi(Li0.5Nb0.5)O3 solid solutions in a broad temperature range applied in X8R

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Abstract

(1 − x)BaTiO3–xBi(Li0.5Nb0.5)O3 [(1 − x)BT–xBLN, 0 ≤ x ≤ 0.1] lead-free ceramics were prepared via a conventional solid state reaction method. Raman spectra and X-ray diffraction results confirmed the phase transformation from tetragonal to pseudo cubic symmetry at 0 ≤ x ≤ 0.02. With adding Bi(Li0.5Nb0.5)O3, the thermal stability of permittivity and dielectric loss of ceramics were improved. Especially, 0.9BT–0.1BLN ceramics exhibited good dielectric properties with small Δε/ε25 °C values (≤ ± 15%) in a wide temperature range of −61–160 °C, high relative permittivity (~1500–1750) and low dielectric loss (tan δ ≤ 0.02) from −60 to 200 °C, which indicates that BT–BLN is candidate for X8R devices.

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Acknowledgements

This work was supported by Natural Science Foundation of China (Nos. 11664008, 11364012 and 11464009), Natural Science Foundation of Guangxi (Nos. 2015GXNSFDA139033 and 2014GXNSFAA118326), Research Start-up Funds Doctor of Guilin University of Technology (Nos. 002401003281 and 002401003282), and Project of Outstanding Young Teachers’ Training in Higher Education Institutions of Guangxi.

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Authors and Affiliations

  1. Guangxi Ministry-Province Jointly-Constructed Cultivation Base for State Key Laboratory of Processing for Non-ferrous Metal and Featured Materials, Guangxi Key Laboratory in Universities of Clean Metallurgy and Comprehensive Utilization for Non-ferrous Metals Resources, Collaborative Innovation Center for Exploration of Hidden Nonferrous Metal Deposits and Development of New Materials in Guangxi, School of Materials Science and Engineering, Guilin University of Technology, Guilin, 541004, China

    Xiuli Chen, Xiaoxia Li, Guisheng Huang, Gaofeng Liu, Xiao Yan & Huanfu Zhou

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  1. Xiuli Chen
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  2. Xiaoxia Li
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  3. Guisheng Huang
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  4. Gaofeng Liu
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  5. Xiao Yan
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  6. Huanfu Zhou
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Correspondence to Xiuli Chen or Huanfu Zhou.

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Chen, X., Li, X., Huang, G. et al. Excellent thermal stability and low dielectric loss of (1 − x)BaTiO3 –xBi(Li0.5Nb0.5)O3 solid solutions in a broad temperature range applied in X8R. J Mater Sci: Mater Electron 28, 17278–17282 (2017). https://doi.org/10.1007/s10854-017-7659-y

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  • DOI: https://doi.org/10.1007/s10854-017-7659-y

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