Improved thermal and mechanical properties of aluminium oxide filled epoxy composites by reinforcing milled carbon fiber by partial replacement method

Abstract

The demands for high performance electronic devices have been increasing recently. This continuous demand simultaneously put forward stringent requirements for effective thermal management solutions. In this study, improved thermal and mechanical properties of epoxy composites consisting of milled carbon fiber (MCF) and polyhedral aluminium oxide (Al₂O₃) fillers have been reported. By adding 14.5 wt% MCF and 60 wt% Al₂O₃ particles into epoxy, the maximum thermal conductivity reached were 3.3 and 7.9 times that of neat epoxy respectively. To further improve the composite thermal conductivity, a mixture of the two fillers was utilized. Milled carbon fiber with high aspect ratio enables it to act as heat conducting bridges among 3-D Al₂O₃ irregular particles; contributing considerably to the formation of a more efficient percolating network for heat flow. This resulted in an exceptionally high thermal conductivity with relatively lower filler content. A thermal conductivity of ten times that of neat epoxy was obtained with 42 wt% Al₂O₃ + 8 wt% MCF thus not only break the bottleneck of further improving the thermal conductivity of epoxy composite but also broaden the application of MCF in the field of thermal management solutions.