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Thermally stable Ba0.8Ca0.2TiO3–Bi(Mg0.5Zr0.5)O3 solid solution with low dielectric loss in a broad temperature usage range

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Abstract

Lead-free (1−x)Ba0.8Ca0.2TiO3–xBi(Mg0.5Zr0.5)O3 [(1−x)BCT–xBMZ, 0 ≤ x ≤ 0.3] ceramics were fabricated via a conventional solid-state reaction method. The structure and dielectric properties of BCT–BMZ ceramics were systematically investigated. X-ray diffraction patterns and Raman spectra show that a systematically structural change form a tetragonal to pseudo-cubic phase occurred at about x = 0.06–0.08. As x values increased to 0.3, the temperature stability of permittivity of ceramics was markedly increased (Δε/ε 27 °C ≤ ±15 %) and low dielectric loss (≤2 %) was obtained over a wide temperature range from 27 to 290 °C at 1 kHz. These results indicate that (1−x)BCT–xBMZ ceramics are promising candidates for thermally stabile devices.

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Acknowledgments

This work was supported by Natural Science Foundation of China (Nos. 11364012 and 11464009), Natural Science Foundation of Guangxi (Nos. 2013GXNSFAA019291, 2014GXNSFAA118326, and 2014GXNSFAA118312), Project of Guangxi Scientific Research and Technical Development (No. 1348020-11).

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Authors and Affiliations

  1. Key Laboratory of New Processing Technology for Nonferrous Metals and Materials, Ministry of Education, School of Materials Science and Engineering, Guilin University of Technology, Guilin, 541004, China

    Guisheng Huang, Xiuli Chen, Dandan Ma, GaoFeng Liu & Huanfu Zhou

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  1. Guisheng Huang
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  2. Xiuli Chen
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  3. Dandan Ma
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  4. GaoFeng Liu
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  5. Huanfu Zhou
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Correspondence to Xiuli Chen.

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Huang, G., Chen, X., Ma, D. et al. Thermally stable Ba0.8Ca0.2TiO3–Bi(Mg0.5Zr0.5)O3 solid solution with low dielectric loss in a broad temperature usage range. J Mater Sci: Mater Electron 27, 6552–6557 (2016). https://doi.org/10.1007/s10854-016-4599-x

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  • DOI: https://doi.org/10.1007/s10854-016-4599-x

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