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Low-temperature firing and microwave dielectric properties of LBS glass-added Li2ZnTi3O8 ceramics with TiO2

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Abstract

Temperature stable Li2ZnTi3O8 dielectric ceramics with Li2O–B2O3–SiO2 (LBS) glass additive and TiO2 dopant have been prepared by the conventional solid-state ceramic route. The sintering temperature of Li2ZnTi3O8 ceramics can be reduced from 1,050 to 875 °C by doping LBS glass additive. The 1 wt% LBS-added Li2ZnTi3O8 sintered at 875 °C/4 h has ε r  = 23.9, Q × f = 40,503 GHz, and τ f  = −13.4 ppm/°C. Adding appropriate amount of TiO2 can effectively adjust the temperature coefficient of resonant frequency (τ f ) and improve the dielectric properties. Typically, the Li2ZnTi3O8 + 1 wt% LBS + 3.5 wt% TiO2 sintered at 875 °C shows excellent dielectric properties of εr = 26, Q × f = 44,023 GHz, τ f  = −4.4 ppm/°C. Compatibility with Ag electrode indicates this material may be applied to low temperature co-fired ceramic devices.

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Acknowledgments

This work was supported by the National Undergraduate’s Innovation Experiment Program (101059529), Ministry of Education of the People’s Republic of China.

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Authors and Affiliations

  1. School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin, 541004, China

    Mei-zhen Hou, Guo-hua Chen, Yan Bao, Yun Yang & Chang-lai Yuan

  2. Guangxi Key Laboratory of Information Materials, Guilin University of Electronic Technology, Guilin, 541004, China

    Guo-hua Chen & Chang-lai Yuan

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  1. Mei-zhen Hou
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  2. Guo-hua Chen
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  3. Yan Bao
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  4. Yun Yang
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Correspondence to Guo-hua Chen.

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Hou, Mz., Chen, Gh., Bao, Y. et al. Low-temperature firing and microwave dielectric properties of LBS glass-added Li2ZnTi3O8 ceramics with TiO2 . J Mater Sci: Mater Electron 23, 1722–1727 (2012). https://doi.org/10.1007/s10854-012-0653-5

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