Skip to main content

Advertisement

Log in

The real part of AC conductance in amorphous nanocomposites ferromagnetic alloy–dielectric

  • Published:
Journal of Materials Science Aims and scope Submit manuscript

Abstract

Results of AC conductivity of the granular nanocomposites consisting of amorphous ferromagnetic alloy nanoparticles (Fe0.45Co0.45Zr0.10) embedded into amorphous dielectric matrix (Al2O3) are presented and analyzed here. Conductivity measurements were made for the samples of different metal-to-dielectric ratio x (25 < x < 65 at.%) in the frequency range of 0.1–1000 kHz at temperature of 80–340 K. Real part of AC conductance at low frequencies (f ≤ 5 kHz) have shown temperature dependencies σreal(T) corresponding to Mott hopping regime at x below the percolation threshold and metallic one beyond the percolation threshold. It was shown that σreal(T) dependencies satisfactorily follow the known relations of 3D percolate models with critical indexes t ≈ 1.6, q ≈ 0.9, and s = 0.62. The numerical estimations of the density of localized states N(EF) displayed a tendency to be decreased with x increase and the electron wave-function localization length a was about 11 nm.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Subscribe and save

Springer+
from $39.99 /Month
  • Starting from 10 chapters or articles per month
  • Access and download chapters and articles from more than 300k books and 2,500 journals
  • Cancel anytime
View plans

Buy Now

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4

Similar content being viewed by others

References

  1. Salz D, Wark M, Baalmann A, Simon U, Jaeger N (2002) Phys Chem Chem Phys 4:2438

    Article  CAS  Google Scholar 

  2. Stauffer D, Aharony A (1992) Introduction to percolation theory. Taylor and Francis, London

    Google Scholar 

  3. Boltcher CJF, Bordewijk P (1978) Theory of electric polarization, vol I & II, 2nd edn. Elsevier, New York

    Google Scholar 

  4. McCrum NG, Readond BE, Williams G (1967) Anelastic and dielectric effects in polymeric solids. Wiley, New York

    Google Scholar 

  5. Wong J, Angell CA (1976) Glasses: structure by spectroscopy. Marcel Dekker, New York

    Google Scholar 

  6. Mott NF, Davis EA (1971) Electronic processes in non crystalline materials, 2nd edn. Oxford University, New York

    Google Scholar 

  7. Pollak M, Geballe TH (1961) Phys Rev 122:1742

    Article  CAS  Google Scholar 

  8. Li W, Sun Y, Sullivan CR (2005) IEEE Trans Magn 41:3283

    Article  CAS  Google Scholar 

  9. Sullivan CR, Prabhakaran S, Dhagat P, Sun Y (2003) Trans Magn Soc Jpn 3:126

    Article  CAS  Google Scholar 

  10. Dhagat P, Prabhakaran S, Sullivan CR (2004) IEEE Trans Magn 40:2008

    Article  CAS  Google Scholar 

  11. Saad AM, Mazanik AV, Kalinin YuE, Fedotova JA, Fedotov AK, Wrotek S, Sitnikov AV, Svito IA (2004) Rev Adv Mater Sci 8:34

    Google Scholar 

  12. Dieny B, Speriosu VS, Metin S et al (1991) J Appl Phys 60:4774

    Article  Google Scholar 

  13. Wang ZJ, Mitsudo S, Watanable J (1997) J Magn Magn Mater 176:127

    Article  CAS  Google Scholar 

  14. Jonker B et al (2000) Phys Rev B 62:8180

    Article  CAS  Google Scholar 

  15. Kobayashi N, Ohnuma S, Masumoto T, Fujimori H (2001) J Appl Phys 90:4159

    Article  CAS  Google Scholar 

  16. Grunberg P (2001) J Phys Condens Matter 13:7691

    Article  CAS  Google Scholar 

  17. Schmidt G, Molenkamp LW (2002) Semicond Sci Technol 17:310

    Article  CAS  Google Scholar 

  18. Nishimura N, Hirai T, Koganei A et al (2002) J Appl Phys 91:5246

    Article  CAS  Google Scholar 

  19. Almokhtar M, Mibu K, Shinjo T (2002) Phys Rev B 66:134401

    Article  Google Scholar 

  20. Zaharko O, Oppeneer PM et al (2002) Phys Rev B 66:134406

    Article  Google Scholar 

  21. Kalaev VA, Kalinin YuE, Necaev VN, Sitnikov AV (2003) Bull Voronezh State Tech Univ Mater Sci 13:38

    Google Scholar 

  22. Saad AM, Fedotov AK, Fedotova JA, Svito IA, Andrievsky BV, Kalinin YuE, Fedotova VV, Malyunina-Bronskaya V, Patryn AA, Mazanik AV, Sitnikov AV (2006) Phys Status Solidi C 3:1283

    Article  CAS  Google Scholar 

  23. Saad AM, Fedotov AK, Svito IA, Mazanik AV, Andrievski BV, Patryn AA, Kalinin YuE, Sitnikov AV (2006) Prog Solid State Chem 14:139

    Article  Google Scholar 

  24. Saad AM, Fedotov AK, Svito IA, Fedotova JA, Andrievsky BV, Kalinin YuE, Patryn AA, Fedotova VV, Malyutina-Bronskaya V, Mazanik AV, Sitnikov AV (2006) J Alloys Compd 423:176

    Article  CAS  Google Scholar 

  25. Huang JCA, Hsu CY (2004) Appl Phys Lett 24:85

    Google Scholar 

  26. MacDonald JR (2005) Solid State Ionics 176:1961

    Article  CAS  Google Scholar 

  27. Fedotova J, Kalinin Yu, Fedotov A, Sitnikov A, Svito I, Zalesskij A, Jablonska A (2005) Hyperfine Interact 165:127

    Article  Google Scholar 

  28. Grimmet G (1999) Percolation. Springer-Verlag, Berlin, p 444

    Book  Google Scholar 

  29. Kalinin YuE, Remizov AN, Sitnikov AV (2004) Phys Solid State 46:2146

    Article  CAS  Google Scholar 

  30. Efros AL, Shklovski BI (1976) Phys Status Solidi B 76:475

    Article  CAS  Google Scholar 

  31. Saad AM, Andrievsky B, Fedotov A, Fedotova J, Figielski T, Kalinin Yu, Malyutina-Bronskaya V, Mazanik A, Patryn A, Sitnikov A, Svito IA (2005) In: Podor B, Horvath ZsJ, Basa P (eds) Proceedings of the 1st international workshop on semiconductor nanocrystals (SEMINANO), Budapest, Hungary, 10–12 Sept 2005, p 321

  32. Mott NF, Devis EA (1979) Electron processes in noncrystalline materials. Clarendon Press, Oxford

    Google Scholar 

  33. Yasuda К, Yoshida A, Arizumi T (1977) Phys Status Solidi A 41:k181

    Article  CAS  Google Scholar 

  34. Austin IG, Mott NF (1969) Adv Phys 18:41

    Article  CAS  Google Scholar 

Download references

Acknowledgement

The author wishes to thank Belarusian State University especially Prof. A. Fedotov for allowing him to do this work during his devoted summer vacations for the last several years and also Prof. Yu. Kalinin from Voronezh State Technical University for presentation of the samples.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to A. M. Saad.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Saad, A.M. The real part of AC conductance in amorphous nanocomposites ferromagnetic alloy–dielectric. J Mater Sci 44, 2513–2519 (2009). https://doi.org/10.1007/s10853-009-3325-y

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10853-009-3325-y

Keywords