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Manifestation in IR-Luminescence of Cross Relaxation Processes between NV-Centers in Weak Magnetic Fields

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Journal of Applied Spectroscopy Aims and scope

The effect of a magnetic field on the luminescence from an ensemble of NV-centers in diamond was studied experimentally and theoretically. It was found that the intensity of infrared luminescence associated with transitions between singlet levels of NV-centers showed a pronounced increase in a near-zero magnetic field. The influence of the power and polarization of the laser radiation on the amplitude and shape of the revealed local maximum in the IR-luminescence of NV-centers was investigated. An eight-level photophysical model of an NV-center in the presence of an arbitrarily directed magnetic field was constructed and used as a basis to calculate the intensity of the luminescence emitted by an ensemble of NV-centers in both the visible and infrared spectral regions. It was shown that a phenomenological allowance for cross relaxation of NV-centers between each other and with other diamond paramagnetic centers within the framework of this model allows the experimentally observed fluorescence features of an ensemble of NV-centers in the presence of weak magnetic fields to be described.

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Authors and Affiliations

  1. B. I. Stepanov Institute of Physics, National Academy of Sciences of Belarus, Minsk, Belarus

    D. S. Filimonenko, V. M. Yasinskii, A. P. Nizovtsev & S. Ya. Kilin

  2. National Research Nuclear University MEPhI, Moscow, Russia

    A. P. Nizovtsev

  3. Institute for Quantum Optics, Ulm University, Ulm, Germany

    F. Jelezko

Authors
  1. D. S. Filimonenko
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  2. V. M. Yasinskii
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  3. A. P. Nizovtsev
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  4. S. Ya. Kilin
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  5. F. Jelezko
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Correspondence to D. S. Filimonenko.

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Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 88, No. 6, pp. 858–871, November–December, 2021.

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Filimonenko, D.S., Yasinskii, V.M., Nizovtsev, A.P. et al. Manifestation in IR-Luminescence of Cross Relaxation Processes between NV-Centers in Weak Magnetic Fields. J Appl Spectrosc 88, 1131–1143 (2022). https://doi.org/10.1007/s10812-022-01290-z

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  • DOI: https://doi.org/10.1007/s10812-022-01290-z

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