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Experimental Investigation on the Solubility of 3,3,3-Trifluoropropene in [hmim][TfO] and [omim][TfO] ILs from 303.15 K to 343.15 K

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Abstract

The working pairs composed of hydrofluoroolefins (HFOs) and ionic liquids (ILs) have exhibited promising potential in the absorption refrigeration systems (ARS). In order to exploit the possibility of 3,3,3-trifluoropropene/ILs as the pairs used in the ARS, the experimental determination on the solubility of 3,3,3-trifluoropropene in 1-hexyl-3-methyl-imidazolium trifluoromethanesulfonate ([hmim][TfO]) and 1-octyl-3-methyl-imidazolium trifluoromethanesulfonate ([omim][TfO]) ILs was conducted. The present measurements were carried out based on the isochoric saturation method at the temperature range from 303.15 K to 343.15 K. The experimental solubility data were correlated through the non-random two-liquid (NRTL) model, universal quasi-chemical (UNIQUAC) model and Krichevsky-Kasarnovsky (K-K) model, respectively. In addition, the influence of the alkyl chain length for different ILs on the solubility of R1243zf and the dissolving capacities of different HFOs in [hmim][TfO] were compared. The Henry’s constants and mixing thermodynamic properties (enthalpy, entropy and Gibbs Energy) of R1243zf in [hmim][TfO] and [omim][TfO] were calculated and discussed. Furthermore, the coefficients of performance of different R1243zf/IL working pairs in single-effect ARS were compared.

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Funding

This work was supported by the National Key Research and Development Program of China (Grant No. 2022YFE0210200) and National Natural Science Foundation of China (No. 51936009).

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Authors and Affiliations

  1. Key Laboratory of Thermo-Fluid Science and Engineering, Ministry of Education, School of Energy and Power Engineering, Xi’an Jiaotong University, Xi’an, 710049, China

    Xiucan Jia, Long Ma & Xiaopo Wang

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  1. Xiucan Jia
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  2. Long Ma
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  3. Xiaopo Wang
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Contributions

XJ contributed to measuring the solubilities, writing draft version. LM contributed to the correlation of the models and analysis. XW contributed to reviewing and editing the whole manuscript.

Corresponding author

Correspondence to Xiaopo Wang.

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Jia, X., Ma, L. & Wang, X. Experimental Investigation on the Solubility of 3,3,3-Trifluoropropene in [hmim][TfO] and [omim][TfO] ILs from 303.15 K to 343.15 K. Int J Thermophys 44, 92 (2023). https://doi.org/10.1007/s10765-023-03200-7

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