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Development of Mössbauer diffractometer by using nuclear resonant scattering at SPring-8 BL11XU

Hyperfine Interactions volume 237, Article number: 157 (2016) Cite this article

Abstract

A Mössbauer diffractometer has been developed by using 57Fe nuclear resonant scattering apparatus at SPring-8 BL11XU in order to obtain a crystal-site-selective Mössbauer spectrum. A 𝜃-2𝜃 goniometer was newly installed between the nuclear monochromator and a detector. From a single crystal Fe3 O 4 mounted on the goniometer, the 111, 222, and 220 reflected γ-rays were used to collect the diffraction spectra at room temperature. The intensity ratio of the two subspectra, corresponding to A- and B-site Fe ions, changes notably according to the reflection index. The diffraction spectrum is composed of a major absorption spectrum and a minor emission spectrum. The former is given by the γ-ray due to the electron scattering and nuclear absorption, whereas the latter is given by the γ-ray due to the nuclear resonant scattering. Interference effects between these two γ-rays are also seen as line broadenings, asymmetric line shapes, and slope of the base lines. These features can be successfully expressed by a Fano function. We consider that the emission spectrum due to the nuclear resonant scattering represents crystal-site-selective Mössbauer spectrum.

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Authors and Affiliations

  1. Department of Science and Engineering, Teikyo University, Utsunomiya, 320-8551, Japan

    Shin Nakamura

  2. National Institutes for Quantum and Radiological Science and Technology, 1-1-1 Kouto, Sayo-cho, Sayo-gun, Hyogo, 679-5148, Japan

    Takaya Mitsui

  3. Okayama University, 1-1-1, Tsushima-Naka, Kita-ku, Okayama, 700-8530, Japan

    Kosuke Fujiwara & Naoshi Ikeda

  4. Research Reactor Institute, Kyoto University, 2-1010 Asashironishi, Kumatori-cho, Sennan-gun, Osaka, 590-0494, Japan

    Yasuhiro Kobayashi

  5. Kyoto Sangyo University, Motoyama, Kamigamo, Kita-ku, Kyoto, 603-8555, Japan

    Susumu Shimomura

Authors
  1. Shin Nakamura
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  2. Takaya Mitsui
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  3. Kosuke Fujiwara
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  4. Naoshi Ikeda
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  5. Yasuhiro Kobayashi
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  6. Susumu Shimomura
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Corresponding author

Correspondence to Shin Nakamura.

Additional information

This article is part of the Topical Collection on Proceedings of the International Conference on Hyperfine Interactions and their Applications (HYPERFINE 2016), Leuven, Belgium, 3–8 July 2016

Edited by Kristiaan Temst, Stefaan Cottenier, Lino M. C. Pereira and André Vantomme

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Nakamura, S., Mitsui, T., Fujiwara, K. et al. Development of Mössbauer diffractometer by using nuclear resonant scattering at SPring-8 BL11XU. Hyperfine Interact 237, 157 (2016). https://doi.org/10.1007/s10751-016-1370-x

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  • DOI: https://doi.org/10.1007/s10751-016-1370-x

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