Analysis on the influence of forest soil characteristics on radioactive Cs infiltration and evaluation of residual radioactive Cs on surfaces
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We investigated the depth profiles of radioactive Cs, ignition loss, and cation exchange capacity (CEC) in five types of forest soils sampled using scraper plates. We then simulated the monitored depth profiles in a compartment model, taking ignition loss as a parameter based on experimental results showing a positive correlation between ignition loss and the CEC. The calculated values were comparable with the monitored values, though some discrepancy was observed in the middle of the soil layer. Based on decontamination data on the surface dose rate and surface contamination concentration, we newly defined a surface residual index (SRI) to evaluate the residual radioactive Cs on surfaces. The SRI value tended to gradually decrease in forests and unpaved roads and was much smaller in forests and on unpaved roads than on paved roads. The radioactive Cs was assumed to have already infiltrated underground 18 months after the nuclear power plant accident, and the sinking was assumed to be ongoing. The SRI values measured on paved roads suggested that radioactive Cs remained on the surfaces, though a gradual infiltration was observed towards the end of the monitoring term. The SRI value is thought to be effective in grasping the rough condition of residual radioactive Cs quickly at sites of decontamination activity in the field. The SRI value may be serviceable for actual contamination works after further research is done to elucidate points such as the relation between the SRI and the infiltration of radioactive Cs in various types of objects.
KeywordsEffect of forest decontamination Infiltration of radioactive Cs Ignition loss Compartment model Residual radioactive substances Types of radiation
Mr. Sei Kato, director of the Fukushima Office for Environmental Restoration, Ministry of the Environment, kindly provided the data and information on the current state of decontamination works. Mr. Keiichi Kawase, Mr. Masanori Watanabe, and Mr. Yuto Terakawa of the Japan Atomic Energy Agency and Mr. Koichi Mitsuo of the Tokyo Electric Power Company provided the technical support for the field studies. Mr. Hitoshi Kondo, Mr. Tatsunari Kometani, Mr. Hendra Adhi Pramata, Mr. Yongqiang Cui, and Mr. Adriraga Pramata from my laboratory helped me collect samples in the field.
This research was conducted with the financial support from KAKENHI 15H04068 (Representative: Yoko Shimada).
- FA (Forestry Agency) (2016). The result of distribution survey of radioactive substances in forest (Fiscal year 2015). http://www.rinya.maff.go.jp/j/kaihatu/jittaihaaku/zentai.html (in Japanese). Accessed 24 Aug 2017.
- JAEA (Japan Atomic Energy Agency) (2016a). Calculation system for decontamination effect. http://nsec.jaea.go.jp/josen (in Japanese). Accessed 24 Aug 2017.
- JAEA (Japan Atomic Energy Agency) (2016b). Monitoring of air dose rate on and around the road by car-borne survey. Report on distribution of radioactive substances released by Fukushima nuclear accident. http://fukushima.jaea.go.jp/initiatives/cat03/pdf08/Part1-1.pdf. Accessed 24 Aug 2017.
- JCAC (Japan Chemical Analysis Center) (2016). Environment radiation database. http://search.kankyo-hoshano.go.jp/servlet/search.top?pageSID=19275246. Accessed 24 Aug 2017.
- JFTA (Japan Forest Technology Association) (2001). Encyclopedia of forest and forestry, p. 628.Google Scholar
- JRIA (Japan Radioisotope Association) (2011). Radioisotope pocket data book. 11th edition, pp. 63–64.Google Scholar
- Miyoshi, Y., Haruki, M., & Ogiwara, H. (2010). The chemical characteristics of soil on typical stands in Nopporo National Forest. Boreal Forest Research, 58, 67–70 (in Japanese).Google Scholar
- MOE (Ministry of the Environment) (2013a). Guideline for decontamination (ver.2). pp. 1-16–1-17 (in Japanese).Google Scholar
- MOE (Ministry of the Environment) (2013b). Guideline for decontamination (ver.2). pp. 2-116–2-125 (in Japanese).Google Scholar
- MOE (Ministry of the Environment) (2013c). Guideline for decontamination (ver.2). p. 2–56 and p. 2-107 (in Japanese).Google Scholar
- MOE (Ministry of the Environment) (2014). Comprehensive and basic materials concerning influences for health or other things by radiation (in Japanese). http://www.env.go.jp/chemi/rhm/h27kisoshiryo/attach/201606mat1-01-20.pdf. Accessed 28 Aug 2017.
- Muramoto, J., Goto, I., & Ninaki, M. (1992). Rapid analysis of exchangeable cations and cation exchange capacity (CEC) of soils by a shaking extraction method. Journal of Soil Science and Plant Nutrition, 63, 210–215.Google Scholar
- NISA (Nuclear and Industrial Safety Agency) (2011a). The evaluation of the reactor core No. 1, 2 and 3 concerning Fukushima nuclear power plant accident. http://www.meti.go.jp/earthquake/nuclear/pdf/20110606-1nisa.pdf (in Japanese). Accessed 28 Aug 2017.
- NISA (Nuclear and Industrial Safety Agency) (2011b). The error of data for released radioactive substances. http://warp.ndl.go.jp/info:ndljp/pid/6086248/www.meti.go.jp/press/2011/10/20111020001/20111020001.pdf (in Japanese). Accessed 28 Aug 2017.
- Ogawa, K., Kuwana, T., Ushio, A., Shimizu, K., Maki, H., Yoshikura, J., & Watanabe, K. (2004). The influence on yield of rice and wheat by 50-year use of compost and three elements of fertilizer. Kinki Chugoku Shikoku Agricultural Research, 5, 3–9 (in Japanese).Google Scholar
- Shimokawa, K., Takada, H., Watanabe, N., Mori, H., Haha, N., Yasuda, Y., & Ose, Y. (1980). Correlation between cation-exchange capacity and ignition loss, clay fraction or heavy metal content in bottom sediments from the Nagara River. Journal of Water Pollution Research, 3(4), 181–186 (in Japanese).CrossRefGoogle Scholar
- Yamaguchi, N. (2011). Adsorption mechanism of radiocesium on soil. Journal of the Japanese Society of Soil Physics, 126, 11–21 (in Japanese).Google Scholar
- Yamaguchi, N., Takata, Y., Hayashi, K., Ishikawa, S., Kuramata, M., Eguchi, S., Yoshikawa, S., Sakaguchi, A., Asada, K., Wagai, R., Makino, T., Akahane, I., & Hiradate, S. (2012). Behavior of radiocaesium in soil-plant systems and its controlling factor. Bulletin of National Institute for Agro-Environmental Sciences, 31, 75–129 (in Japanese).Google Scholar