Skip to main content

Advertisement

Log in

Saharan dust particles in snow samples of Alps and Apennines during an exceptional event of transboundary air pollution

  • Published:
Environmental Monitoring and Assessment Aims and scope Submit manuscript

Abstract

Southern European countries are often affected in summer by transboundary air pollution from Saharan dust. However, very few studies deal with Saharan dust pollution at high altitudes in winter. In Italy, the exceptional event occurred on February 19, 2014, colored in red the entire mountain range (Alps and Apennines) and allowed to characterize the particulate matter deposited on snow from a morphological and chemical point of view. Snow samples were collected after this event in four areas in the Alps and one in the Apennines. The particulate matter of the melted snow samples was analyzed by scanning electron microscopy with energy dispersive X-ray spectrometry (SEM-EDS) and by inductively coupled plasma mass spectrometry (ICP-MS). These analyses confirmed the presence of Saharan dust particle components in all areas with similar percentages, supported also by the positive correlations between Mg-Ca, Al-Ca, Al-Mg, and Al-K in all samples.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8
Fig. 9

Similar content being viewed by others

References

  • AINEVA (2014) http://www.aineva.it/pubblica/neve81/nv81_rivista_3.pdf.Accessed 2 Feb 2015.

  • Bonazza, A., Brimblecombe, P., Grossi, C. M., & Sabbioni, C. (2007). Carbon in black crusts from the Tower of London. Environmental Science & Technology, 41, 4199–4204.

    Article  CAS  Google Scholar 

  • Bosellini, A. (1998). Geologia delle Dolomiti. Bolzano: Editore Athesia.

    Google Scholar 

  • Choobari, A. O., Zawar-Reza, P., & Sturman, A. (2014). The global distribution of mineral dust and its impacts on the climate system: a review. Atmospheric Research, 138, 152–165.

    Article  CAS  Google Scholar 

  • CNR Report Winter.(2013/2014). Italian Climate Observatory O. Vittori Mt. Cimone GAW459 WMO Global Station.

  • Cusinato, A., & Bertola, S. (2004). Le risorse litiche dell’Altopiano di Folgaria e il loro utilizzo a Riparo Cogola. Studi Trent Sci Nat, 40, 107–123.

    Google Scholar 

  • De Longueville, F., Hountondji, Y. C., Henry, S., & Ozer, P. (2010). What do we know about effects of desert dust on air quality and human health in West Africa compared to other regions? The Science of the Total Environment, 409, 1–8.

    Article  Google Scholar 

  • Di Sarra, A., Di Biagio, C., Meloni, D., Monteleone, F., Pace, G., Pugnaghi, S., & Sferlazzo, D. (2011). Shortwave and longwave radiative effects of the intense Saharan dust event of 25–26 March 2010 at Lampedusa (Mediterranean Sea). Journal of Geophysical Research, 116, D23209.

    Article  Google Scholar 

  • Dimitriou, K., & Kassomenos, P. (2014). Indicators reflecting local and transboundary sources of PM2.5 and PM coarse in Rome—impacts in air quality. Atmospheric Environment, 96, 154–162.

    Article  CAS  Google Scholar 

  • Directive2008/50/EC of the European Parliament and of the Council of 21 May 2008 on ambient air quality and cleaner air for Europe.

  • EEA.(2012). Particulate matter from natural sources and related reporting under the EU Air Quality Directive in 2008 and 2009. EEA Technical Report No 10/2012.

  • Escudero, M., Stein, A. F., Draxler, R. R., Querol, X., Alastuey, A., Castillo, S., & Avila, A. (2011). Source apportionment for African dust outbreaks over the Western Mediterranean using the HYSPLIT model. Atmospheric Environment, 99, 518–527.

    CAS  Google Scholar 

  • EUMETSAT (2016) http://www.eumetsat.int/website/home/index.html. Accessed 30 May 2016.

  • Falasco, E., Ector, L., Ciaccio, E., Hoffmann, L., & Bona, F. (2012). Alpine freshwater ecosystems in a protected area: a source of diatom diversity. Hydrobiologia, 695, 233–251.

    Article  CAS  Google Scholar 

  • Garrison, V. H., Majewski, M. S., Konde, L., Wolf, R. E., Otto, R. D., & Tsuneoka, Y. (2014). Inhalable desert dust, urban emissions and potentially biotoxic metals in urban Saharan-Sahelian air. The Science of the Total Environment, 500-501, 383–394.

    Article  CAS  Google Scholar 

  • Ghedini, N., Ozga, I., Bonazza, A., Dilillo, M., Cachièr, H., & Sabbioni, C. (2011). Atmospheric aerosol monitoring as a strategy for the preventive conservation of urban monumental heritage: the Florence Baptistery. Atmospheric Environment, 45, 5979–5987.

    Article  CAS  Google Scholar 

  • Guerrero-Rascado, J. L., Olmo, F. J., Avilés-Rodriguez, I., Navas-Guzman, F., Pérez-Ramirez, D., Lyamani, H., & AladosArboledas, L. (2009). Extreme Saharan dust event over the southern Iberian Peninsula in September 2007: active and passive remote sensing from surface and satellite. Atmospheric Chemistry and Physics, 9, 8453–8469.

    Article  CAS  Google Scholar 

  • Guinot, B., Cachier, H., & Oikonomou, K. (2007). Geochemical perspectives from a new aerosol chemical mass closure. Atmospheric Chemistry and Physics, 7, 1657–1670.

    Article  CAS  Google Scholar 

  • Handbook on the Implementation of EC Environmental Legislation (2008). Section 3: 167–192. Regional Environmental Center, Umweltbundesamt GmbH.

  • Kocak, M., Theodosi, C., Zarmpas, P., Séguret, M. J. M., Herut, B., Kallos, G., Mihalopoulos, N., Kubilay, N., & Nimmo, M. (2012). Influence of mineral dust transport on the chemical composition and physical properties of the Eastern Mediterranean aerosol. Atmospheric Environment, 57, 266–277.

    Article  CAS  Google Scholar 

  • Kubilay, N., Oguz, T., & Kocak, M. (2005). Ground-based assessment of Total Ozone Mapping Spectrometer (TOMS) data for dust transport over the northeastern Mediterranean. Global Biogeochemical Cycles, 19, GB1022.

    Article  Google Scholar 

  • Kumar, A., Abouchami, W., Galer, S., Garrison, V., Williams, E., & Andreae, M. (2014). A radiogenic isotope tracer study of transatlantic dust transport from Africa to the Caribbean. Atm Env, 82, 130–143.

    Article  CAS  Google Scholar 

  • Lequy, É., Conil, S., & Turpault, M. P. (2012). Impacts of Aeolian dust deposition on European forest sustainability: a review. Forest Ecology and Management, 267, 240–252.

    Article  Google Scholar 

  • Malaguti, A., Mircea, M., La Torretta, T. M. G., Telloli, C., Petralia, E., Stracquadanio, M., & Berico, M. (2015). Chemical composition of fine and coarse aerosol particles in Central Mediterranean in dust and non-dust conditions. Aerosol and Air Quality Research, 15, 410–425.

    Article  CAS  Google Scholar 

  • Mallone, S., Stafoggia, M., Faustini, A., Gobbi, G. P., Marconi, A., & Forastiere, F. (2011). Saharan dust and associations between particulate matter and daily mortality in Rome, Italy. Environmental Health Perspectives, 119, 1409–1414.

    Article  CAS  Google Scholar 

  • Marconi, M., Sferlazzo, D. M., Becagli, S., Bommarito, C., Calzolai, G., Chiari, M., Di Sarra, A., Ghedini, C., Gomez-Amo, J. L., Lucarelli, F., Meloni, D., Monteleone, F., Nava, S., Pace, G., Piacentino, S., Rugi, F., Severi, M., Traversi, R., & Udisti, R. (2013). Saharan dust aerosol over the central Mediterranean Sea: optical columnar measurements vs. aerosol load, chemical composition and marker solubility at ground level. Atmospheric Chemistry and Physics, 14, 2039–20154.

    Article  Google Scholar 

  • Mitsakou, C., Kallos, G., Papantoniou, N., Spyrou, C., Solomos, S., Astitha, M., & Housiadas, C. (2008). Saharan dust levels in Greece and received inhalation doses. Atmospheric Chemistry and Physics, 8, 7181–7192.

    Article  CAS  Google Scholar 

  • Moreno, T., Querol, X., Castillo, S., Alastuey, A., Cuevas, E., Herrmann, L., Mounkaila, M., Elvira, J., & Gibbons, W. (2006). Geochemical variations in aeolian mineral particles from the Sahara-Sahel Dust Corridor. Chemosphere, 65, 261–270.

    Article  CAS  Google Scholar 

  • Nastos, P. T. (2011). Environmental impacts on human health during a Saharan dust episode at Crete Island, Greece. Meteorologische Zeitschrift, 20, 517–529.

    Article  Google Scholar 

  • Nava, S., Becagli, S., Calzolai, G., Chiari, M., Lucarelli, F., Prati, P., Traversi, R., Udisti, R., Valli, G., & Vecchi, R. (2012). Saharan dust impact in central Italy: an overview on three years’ elemental data records. Atm Env, 60, 444–452.

    Article  CAS  Google Scholar 

  • Painter, T. H., McKenzie Skiles, S., Deems, J. S., Bryant, A. C., & Landry, C. C. (2012). Dust radiative forcing in snow of the Upper Colorado River Basin: 1. A 6-year record of energy balance, radiation, and dust concentrations. Water Resources Research, 48, W07521.

  • Perez, N., Pey, J., Querol, X., Alastuey, A., Lopez, J. M., & Viana, M. (2008). Partitioning of major and trace components in PM10-PM2.5-PM1 at an urban site in Southern Europe. Atmospheric Environment, 42, 1677–1691.

    Article  CAS  Google Scholar 

  • Perrino, C., Canepari, S., Catrambrone, M., Dalla Torre, S., Rantica, E., & Sargolini, T. (2009). Influence of natural events on the concentration and composition of atmospheric particulate matter. Atmospheric Environment, 43, 4776–4779.

    Article  Google Scholar 

  • Pettijohn, F. J. (1975). Sedimentary rocks. In Earth data 3rd ed. New York: Harper & Row.

  • Pey, J., Querol, X., Alastuey, A., Forastiere, F., & Stafoggia, M. (2013). African 554 dust outbreaks over the Mediterranean Basin during 2001–2011: PM10 concentrations, phenomenology and trends, and its relation with synoptic and mesoscale meteorology. Atmospheric Chemistry and Physics, 13, 1395–1410.

    Article  Google Scholar 

  • Prospero, J., Collard, F. X., Molinie, J., & Jeannot, A. (2014). Characterising the annual cycle of African dust transport to the Caribbean basin and South America and its impact on the environment and air quality. Global Biogeochemical Cycles, 29, 757–773.

    Article  Google Scholar 

  • Putaud, J. P., Van Dingenen, R., Alastuey, A., Bauer, H., Birmili, W., Cyrys, J., Flentje, H., Fuzzi, S., Gehrig, R., Hansson, H. C., Harrison, R. M., Hermann, H., Hitzenberger, R., Huglin, C., Jones, A. M., Kasper-Giebl, A., Kiss, G., Kousa, A., Kuhlbusch, T. A. J., Loschau, G., Maenhaut, W., Molnar, A., Moreno, T., Pekkanen, J., Perrino, C., Pitz, M., Puxbaum, H., Querol, X., Rodriguez, S., Salma, I., Schwarz, J., Smolik, J., Schneider, J., Spindler, G., Ten Brink, H., Tursic, J., Viana, M., Wiedensohler, A., & Raes, F. (2010). A European aerosol phenomenology—3: physical and chemical characteristics of particulate matter from 60 rural, urban, and kerbside sites across Europe. Atmospheric Environment, 44, 1308–1320.

    Article  CAS  Google Scholar 

  • Querol, X., Alastuey, A., Rodriguez, S., Plana, F., Riuz, C. R., Cots, N., Massagué, G., & Puig, O. (2001). PM10 and PM2.5 source apportionment in the Barcelona Metropolitan area, Catalonia, Spain. Atmospheric Environment, 35, 6407–6419.

    Article  CAS  Google Scholar 

  • Querol, X., Alastuey, A., Pey, J., Cusak, M., Perez, N., Mihalopoulos, N., Theodosi, C., Gerasopoulos, E., Kubilay, N., & Kocak, M. (2009). Variability in regional background aerosols within the Mediterranean. Atmospheric Chemistry and Physics, 9, 4575–4591.

    Article  CAS  Google Scholar 

  • Radhi, M., Box, M. A., Box, G. P., Mitchell, R. M., Cohen, D. D., Stelcer, E., & Keywood, M. D. (2010). Size-resolved mass and chemical properties of dust aerosols from Australia’s Lake Eyre Basin. Atmospheric Environment, 44, 3519–3528.

    Article  CAS  Google Scholar 

  • Remoundaki, E., Papayannis, A., Kassomenos, P., Mantas, E., Kokkalis, P., & Tsezos, M. (2013). Influence of Saharan dust transport events on PM2.5 concentrations and composition over Athens. Water, Air & Soil Pollution, 224, 1373.

    Article  Google Scholar 

  • Reynolds, R. L., Goldstein, H. L., Moskowitz, B. M., Bryant, A. C., McKenzie Skiles, S., Kokaly, R. F., Flagg, C. B., Yauk, K., Berquó, T., Breit, G., Ketterer, M., Fernandez, D., Miller, M. E., & Painter, T. H. (2014). Composition of dust deposited to snow cover in the Wasatch Range (Utah, USA): Controls on radiative properties of snow cover and composition to some dust-source sediments. Aeolian Research, 15, 73–90.

  • Rinaldi, M., Emblico, L., Decesari, S., Fuzzi, S., Facchini, M. C., & Librando, V. (2007). Chemical characterization and source apportionment of size-segregated aerosol collected at an urban site in Sicily. Water, Air & Soil, Pollution, 185, 311–321.

    Article  CAS  Google Scholar 

  • Rudich, Y., Kaufman, Y. J., Dayan, U., Hongbin, Y., & Kleidman, R. G. (2008). Estimation of transboundary transport of pollution aerosols by remote sensing in the eastern Mediterranean. Journal of Geophysical Research, 113, 1–8.

    Article  Google Scholar 

  • Sajani, Z., Bonasoni, S., Cristofanelli, P., Marinoni, A., & Lauriola, P. (2012). Only coarse particles from the Sahara? Epidemiology, 23, 642–643.

    Article  Google Scholar 

  • Telloli, C. (2014). Metal concentrations in snow samples in an Urban Area in the Po Valley. International Journal of Geosciences, 5, 1116–1136.

    Article  Google Scholar 

  • Telloli, C., Fazzini, M., Tassinari, R., Marrocchino, E., & Vaccaro, C. (2013). Monitoring of solid particulate airborne samples from mountain snow in some sites of the Alps, Italy. International Journal of Geosciences, 4, 711–723.

    Article  Google Scholar 

  • Thomas, D. (2011). Arid zone geomorphology: process form and change in drylands (3rd ed.). Oxford: Wiley-Blackwell.

    Book  Google Scholar 

  • Vasić, M. V., Mihailovic, A., Kozmidis-Luburic, U., Nemes, T., Ninkov, J., Zeremski-Skoric, T., & Antic, B. (2012). Metal contamination of short-term snow cover near urban crossroads: correlation analysis of metal content and fine particles distribution. Chemosphere, 86, 585–592.

    Article  Google Scholar 

Download references

Acknowledgements

We would like to thank Renzo Tassinari and Lisa Volpe for the precious help in analyzing samples by ICP-MS and SEM-EDS analysis respectively.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Chiara Telloli.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Telloli, C., Chicca, M., Pepi, S. et al. Saharan dust particles in snow samples of Alps and Apennines during an exceptional event of transboundary air pollution. Environ Monit Assess 190, 37 (2018). https://doi.org/10.1007/s10661-017-6412-6

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1007/s10661-017-6412-6

Keywords

Navigation