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Aircraft measurements of SO2, NOx, CO, and O3 over the coastal and offshore area of Yellow Sea of China

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Abstract

In order to investigate long-range transport of the air pollution in the East Asia, air pollutants, including SO2, NOx, CO, and O3, were observed by aircraft measurement over the coastal and offshore area of Yellow Sea of China in April 2011. NOx and SO2 seemed to become moderate in recent years, and the concentrations during the whole observations ranged from 0.49 to 9.57 ppb and from 0.10 to 16.02 ppb, respectively. The high concentrations of CO were measured with an average value of 0.98 ppm. The measured O3 average concentration was 76.25 ppb, which showed a higher level comparing with the results from some previous studies. Most of the results for the concentration values generally followed the typical characteristic of vertical and spatial distribution, which were “low altitude > high altitude” and “land/coastal > sea,” respectively. Transport of polluted air mass from the continent to the aircraft measurement area was confirmed in some days during the observation by the meteorological analysis, while the measurement results supposed to represent the background level of the pollutants in rest days. Additionally, some small-scale air pollution plumes were observed. Significant positive correlations between NOx and SO2 indicated that these two species originated from the same region. On the other hand, good positive correlations between NOx and O3 found during 2-day flight suggested that the O3 formation was probably under “NOx-limited” regime in these days.

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References

  • Bey, I., Jacob, D. J., Logn, J. A., & Yantosca, R. M. (2001). Asian chemical outflow to the Pacific in spring: origins, pathways, and budgets. Journal of Geophysical Research, 106, 23097–23144.

    Article  CAS  Google Scholar 

  • Chan, C. K., & Yao, X. (2008). Air pollution in mega cities in China. Atmospheric Environment, 42, 1–42.

    Article  CAS  Google Scholar 

  • China statistical communique on environment 2006, Ministry of Environment Protection of China, (http://zls.mep.gov.cn/hjtj/qghjtjgb/201310/t20131018_261850.htm) (in Chinese).

  • China statistical communique on environment 2011, Ministry of Environment Protection of China, (http://zls.mep.gov.cn/hjtj/qghjtjgb/200709/t20070924_109497.htm) (in Chinese).

  • Fang, M., Chan, C. K., & Yao, X. (2009). Managing air quality in a rapidly developing nation: China. Atmospheric Environment, 43, 79–86.

    Article  CAS  Google Scholar 

  • Fuelberg, H. E., Kiley, C. M., Hannan, J. R., Westberg, D. J., Avery, M. A., & Newell, R. E. (2003). Meteorological conditions and transport pathways during the transport and chemical evolution over the Pacific (TRACE-P) experiment. Journal of Geophysical Research, 108(D20), 8782. doi:10.1029/2002JD003092.

    Article  Google Scholar 

  • Geng, F., Zhang, Q., Tie, X., Huang, M., Ma, X., Deng, Z., Yu, Q., Quan, J., & Zhao, C. (2009). Aircraft measurements of O3, NOx, CO, VOCs, and SO2 in the Yangtze River Delta region. Atmospheric Environment, 43, 584–593.

    Article  CAS  Google Scholar 

  • Hatakeyama, S., Murano, K., Bandow, H., Mukai, H., & Akimoto, H. (1995a). High concentration of SO2 observed over the sea of Japan. Terrestrial, Atmospheric and Oceanic Sciences, 6, 403–408.

    Google Scholar 

  • Hatakeyama, S., Murano, K., Bandow, H., Sakamaki, F., Yamato, M., Tanaka, S., & Akimoto, H. (1995b). 91 PEACAMPOT aircraft observation of ozone, NOx, and SO2 over the East China Sea, the Yellow Sea, and the sea of Japan. Journal of Geophysical Research, 100, 23143–23151.

    Article  CAS  Google Scholar 

  • Hatakeyama, S., Murano, K., Mukai, H., Sakamaki, F., Bandow, H., Watanabe, I., Yamato, M., Tanaka, S., & Akimoto, H. (1997). SO2 and sulfate aerosols over the seas between Japan and the Asian continent. Journal of Aerosol Research, Japan, 12, 91–95 in Japanese.

    CAS  Google Scholar 

  • Hatakeyama, S., Murano, K., Sakamaki, F., Mukai, H., Bandow, H., & Komazaki, Y. (2001). Transport of atmospheric pollutants from East Asia. Water, Air, & Soil Pollution, 130, 373–378.

    Article  Google Scholar 

  • Hatakeyama, S., Takami, A., Sakamaki, F., Mukai, H., Sugimoto, N., Shimizu, A., & Bandow, H. (2004). Aerial measurement of air pollutants and aerosols during march 20–22, (2001), over the East China Sea. Journal of Geophysical Research, 109, D13304. doi:10.1029/2003JD004271.

    Article  Google Scholar 

  • Hatakeyama, S., Takami, A., Wang, W., & Tang, D. (2005). Aerial observation of air pollutants and aerosols over Bo Hai, China. Atmospheric Environment, 39, 5893–5898.

    Article  CAS  Google Scholar 

  • Hoell, J. M., Davis, D. D., Liu, S., Newell, R. E., Akimoto, H., & Bendura, R. J. (1997). The pacific exploratory mission-west phase B: February – march 1994. Journal of Geophysical Research, 102, 28223–28239.

    Article  CAS  Google Scholar 

  • Hoell, J. M., Davis, D. D., Liu, S., Newell, R., Shipham, M., Akimoto, H., McNeal, R. J., Bendura, R. J., & Drewry, J. W. (1996). The Pacific exploratory mission-west a (PEM-west a): September–October, 1991. Journal of Geophysical Research, 101, 1641–1653.

    Article  CAS  Google Scholar 

  • Inomata, Y., Iwasaka, Y., Osada, K., Hayashi, M., Mori, I., Kido, M., Hara, K., & Sakai, T. (2006). Vertical distributions of particles and sulfur gases (volatile sulfur compounds and SO2) over East Asia: comparison with two aircraft-borne measurements under the Asian continental outflow in spring and winter. Atmospheric Environment, 40, 430–444.

    Article  CAS  Google Scholar 

  • Intergovernmental Panel on Climate Control (IPCC), Climate Change (2001). In J. T. Houghton et al. (Eds.), The scientific basis. New York: Cambridge Univ. Press.

    Google Scholar 

  • Jacob, D. J., Crawford, J. H., Kleb, M. M., Connors, R. J. B., Raper, J. L., Sachse, G. W., Gille, J. C., Emmons, L., & Heald, C. L. (2002). The transport and chemical evolution over the Pacific (TRACE-P) mission: design, execution, and overview of results. Journal of Geophysical Research, 108(D20), 9000. doi:10.1029/2002JD003276.

    Article  Google Scholar 

  • Lei, W., Zhang, R., Tie, X., & Hess, P. (2004). Chemical characterization of ozone formation in the Houston–Galveston area. Journal of Geophysical Research, 109. doi:10.1029/2003JD004219.

  • Maeda, J., Bandow, H., Watanabe, I., Komazaki, Y., Murano, K., & Hatakeyama, S. (2001). Airborne peroxyacetyl nitrate (PAN) and total nitrogen oxides (NOy) measurements on IGAC project in 1997 and 1999. Journal of Japan Society for Atmospheric Environment, 36, 22–28.

    CAS  Google Scholar 

  • Sillman, S. (1995). The use of NOy, H2O2, and HNO3 as indicators for ozone–NOx hydrocarbon sensitivity in urban locations. Journal of Geophysical Research, 100, 14175–14188.

    Article  Google Scholar 

  • Tang, J., Xu, X., Ba, J., & Wang, S. (2010). Trends of the precipitation acidity over China during 1992–2006. Chinese Science Bulletin, 55(17), 1800–1807.

    Article  CAS  Google Scholar 

  • Taubman, B. F., Hains, J. C., Thompson, A. M., Marufu, L. T., Doddridge, B. G., Stehr, J. W., Piety, C. A., & Dickerson, R. R. (2006). Aircraft vertical profiles of trace gas and aerosol pollution over themid-Atlantic U.S.: statistics and meteorological cluster analysis. Journal of Geophysical Research: Atmospheres, 111(D10). doi:10.1029/2005JD006196.

  • Wang, S., & Hao, J. (2012). Air quality management in China: issues, challenges, and options. Journal of Environmental Sciences, 24(1), 2–13.

    Article  CAS  Google Scholar 

  • Wang, G., Kawamura, K., Hatakeyama, S., Takami, A., Li, H., & Wang, W. (2007). Aircraft measurement of organic aerosols over China. Environmental Science and Technology, 41, 3115–3120.

    Article  CAS  Google Scholar 

  • Wang, W., Liu, H., Yue, X., Li, H., Chen, J., Ren, L., Tang, D., Hatakeyama, S., & Takami, A. (2006). Study on acidity and acidic buffering capacity of particulate matter over Chinese eastern coastal areas in spring. Journal of Geophysical Research, 111, D18207. doi:10.1029/2005JD006753.

    Article  Google Scholar 

  • Wang, W., Ma, J., Hatakeyama, S., Liu, X., Chen, Y., Takami, A., Ren, L., & Geng, C. (2008). Aircraft measurements of vertical ultrafine particles profiles over northern China coastal areas during dust storms in 2006. Atmospheric Environment, 42, 5715–5720.

    Article  CAS  Google Scholar 

  • Watanabe, I., Nakanishi, M., Tomita, J., Hatakeyam, S., Murano, K., Mukai, H., & Bandow, H. (1998). Atmospheric peroxyacyl nitrates in urban/remote sites and the lower troposphere around Japan. Environmental Pollution, 102(S1), 253–261.

    Article  CAS  Google Scholar 

  • Zhang, R., Lei, W., Tie, X., & Hess, P. (2004). Industrial emissions cause extreme diurnal urban ozone variability. Proceedings of the National Academy of Sciences of the United States of America, 101, 6346–6350.

    Article  CAS  Google Scholar 

  • Zhang, Q., Streets, D., Carmichael, G., He, K., Huo, H., Kannari, A., Klimont, Z., Park, I., Reddy, S., & Fu, J. (2009). Asian emissions in 2006 for the NASA INTEX-B mission. Atmospheric Chemistry and Physics, 9, 5131–5153.

    Article  CAS  Google Scholar 

  • Zhang, Q., Streets, D. G., He, K., Wang, Y., Richter, A., Burrows, J. P., Uno, I., Jang, C. J., Chen, D., Yao, Z., & Lei, Y. (2007). NOx emission trends for China 1995-2004: the view from the ground and the view from space. Journal of Geophysical Research, 112, D22306. doi:10.1029/2007JD008684.

    Article  Google Scholar 

Download references

Acknowledgments

This investigation was supported by China Ministry of Environmental Protection’s Special Funds for Scientific Research on Public Welfare (Grant Nos. 201309016 and 201009002), Natural Science Foundation of China (Grant Nos. 41105090 and 20707001).

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Correspondence to Xinhua Wang.

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Yang, X., Wang, X., Yang, W. et al. Aircraft measurements of SO2, NOx, CO, and O3 over the coastal and offshore area of Yellow Sea of China. Environ Monit Assess 188, 527 (2016). https://doi.org/10.1007/s10661-016-5533-7

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