Abstract
The main purpose for this study is to observe the seasonal and monthly variations for arsenic (As) in total suspended particulates (TSP) concentration and dry deposition at five characteristic sampling sites during the years 2009 and 2010 in central Taiwan. The results show that the highest and lowest monthly average As concentrations in TSP occurred in January and May at Bei-shi (suburban/coastal) and Quan-xing (industrial) sampling sites. In addition, the results show that the highest and lowest monthly average As dry deposition occurred in October and May at Chang-hua (downtown) and Gao-mei (wetland) sampling sites. This study reflected that the mean highest As concentrations in TSP and mean highest As dry deposition occurred at Quan-xing (industrial). However, the mean lowest As concentrations in TSP and mean lowest As dry deposition also occurred at Gao-mei (wetland). Regarding seasonal variation, the results show that the As average seasonal concentration order in TSP was winter > spring > fall > summer, respectively, at Chang-hua (downtown) and He-mei (residential) sampling sites. Finally, the order of As average seasonal dry deposition was fall > winter > spring > summer, respectively, at Chang-hua (downtown), He-mei (residential), and Gao-mei (wetland) sampling sites.
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References
Chu, C. C., Fang, G. C., Chen, J. C., & Lin, I. C. (2008). Ambient air dry deposition and ionic species analysis by using various deposition collectors in Shalu, central Taiwan. Atmospheric Research, 88, 212–223.
Duker, A. A., Carranza, E. J. M., & Hale, M. (2005). Arsenic geochemistry and health. Environment International, 31, 631–641.
Fang, G. C., Basu, N., Nam, D. H., & Yang, I. L. (2009). Characterization of ambient air particulates and particulate mercury at Sha-Lu, central Taiwan. Environmental Forensics, 10, 277–285.
Farinha, M. M., Slejkovec, Z., Vanelteren, J. T., Wolterbeek, H. Th., & Freitas, M. C. (2004). Arsenic speciation in lichens and in coarse and fine airborne particulate matter by HPLC–UV–HG–AFS. Journal of Atmospheric Chemistry, 49, 343–353.
Harrison, R. M., Smith, D. J. T., Pio, C. A., & Castro, L. M. (1997). Comparative receptor modeling study of airborne particulate pollutants in Birmingham (United Kingdom), Coimbra (Portugal) and Lahore (Pakistan). Atmospheric Environment, 31, 3309–3321.
Hayes, R. B. (1997). The carcinogenicity of metals in humans. Cancer Causes and Control, 8, 371–385.
Holsen, T. M., Noll, K. E., Fang, G. C., Lee, W. J., & Lin, J. M. (1993). Dry deposition and particle size distributions measured during the Lake Michigan urban air toxics study. Environmental Science & Technology, 7, 1327–1333.
Huang, X., Olmez, I., Aras, N. K., & Gordon, G. E. (1994). Emissions of trace elements from motor vehicles: Potential marker elements and source composition profile. Atmospheric Environment, 28, 1385–1391.
Künzli, N., Mudway, I. S., Götschi, T., Shi, T., Kelly, F. J., Cook, S., et al. (2006). Comparison of oxidative properties, light absorbance, and total and elemental mass concentration of ambient PM2.5 collected at 20 European sites. Environmental Health Perspectives, 5, 114.
Lin, J. M., Fang, G. C., Holsen, T. M., & Noll, K. E. (1993). Dry deposition of atmospheric particles. Atmospheric Environment, 27, 1131–1138.
Milford, J. B., & Davidson, C. I. (1985). The size of particulate trace elements in the atmosphere: A review. Journal of the Air Pollution Control Association, 35, 1249–1260.
Oliveira, V., Gomez-Ariza J. L., & Sanchez-Rodas, D. (2005). Extraction procedures for chemical speciation of arsenic in atmospheric total suspended particles. Analytical and Bioanalytical Chemistry, 382, 335–340.
Roy, P., & Saha, A. (2002). Metabolism and toxicity of arsenic: A human carcinogen. Current Science, 82, 38–45.
Sanchez dela Campa, A. M., de la Rosa, J. D., Sanchez-Rodas, D., Oliveira, V., Alastuey, A., Querol, X., et al. (2008). Arsenic speciation study of PM2.5 in an urban area near a copper smelter. Atmospheric Environment, 42, 6487–6495.
Sanchez-Rodas, D., Sanchez dela Campa, A. M., de la Rosa, J. D., Oliveira, V., Gomez Ariza, J. L., Querol, X., et al. (2007). Arsenic speciation of atmospheric particulate matter (PM10) in an industrialized urban site in southwestern Spain. Chemosphere, 66, 1485–1493.
Serbula, S. M., Antonijevic, M. M., Milosevic, N. M., Milic, S. M., & Ilic, A. A. (2010). Concentrations of particulate matter and arsenic in Bor (Serbia). Journal of Hazardous Materials, 181, 23–51.
Thomaidis, N. S., Bakeas, E. B., & Siskos, P. A. (2003). Characterization of lead, cadmium, arsenic and nickel in PM2.5 particles in the Athens atmosphere, Greece. Chemosphere, 52, 959–966.
Tsai, Y. I., Kuo, S. C., & Lin, Y. H. (2003). Temporal characteristics of inhalable mercury and arsenic aerosols in the urban atmosphere in southern Taiwan. Atmospheric Environment, 37, 3401–3411.
Vassilakos, Ch., Veros, D., Michopoulos, J., Maggos, T., & O’Connor, C. M. (2007). Estimation of selected heavy metals and arsenic in PM10 aerosols in the ambient air of the Greater Athens Area, Greece. Journal of Hazardous Materials, 140, 389–398.
WHO (World Health Organization) (2000). Air quality guidelines for Europe (2nd ed.). Copenhagen: WHO Regional Publications, Regional Office for Europe.
Wu, Y., Hao, J. M., Fu, L. X., Hu, J. N., Wang, Z. S., & Tang, U. W. (2003). Chemical characteristics of airborne particulate matter near major roads and at background locations in Macao, China. Science of the Total Environment, 317, 159–172.
Xie, R., Seip, H. M., Wibetoe, G., Nori, S., & McLeod, C. W. (2006). Heavy coal combustion as the dominant source of particulate pollution in Taiyuan, China, corroborated by high concentrations of arsenic and selenium in PM10. Science of the Total Environment, 370, 409–415.
Zheng, J., Tan, M. G., Shibata, Y., Tanaka, A., Li, Y., & Zhang, G. L. (2004). Characteristics of lead isotope ratios and elemental concentrations in PM10 fraction of airborne particulate matter in Shanghai after the phase-out of leaded gasoline. Atmospheric Environment, 38, 1191–1200.
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Fang, GC., Huang, YL. & Huang, JH. Atmospheric arsenic (As) study at five characteristic sampling sites in Taiwan. Environ Monit Assess 184, 729–740 (2012). https://doi.org/10.1007/s10661-011-1997-7
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DOI: https://doi.org/10.1007/s10661-011-1997-7