Skip to main content

Advertisement

Log in

New Metal Emission Patterns in Road Traffic Environments

  • Published:
Environmental Monitoring and Assessment Aims and scope Submit manuscript

Abstract

The increased awareness of traffic as a major diffuse metal emission source emphasizes the need for more detailed information on the various traffic-related sources and how and where the metals are dispersed. In this study, metal emission patterns in the road traffic environment were examined from the perspective of different surrounding factors, e.g. the importance of intersections, deceleration, vehicle speed and traffic density. A total of 148 topsoil samples from 18 south Swedish roads were analysed (using GFAAS) for traffic-emitted metals, i.e. Cd, Cr, Cu, Ni, Pb, Sb and Zn. The roadside topsoil metal concentrations were used to examine correlations between metals and surrounding factors. The studied metals were divided into three groups corresponding to different emission sources: metals from decelerating activities (Cu, Sb and Zn), metals as historical residues from the combustion of petrol (Pb and Cd), and non-source-specific metals (Cr and Ni). It was found that Cu and Sb, despite their rather short history as traffic-emitted metals, have increased more than eightfold in roadside soils compared to background levels. The major source of road traffic related Cu and Sb is brake linings. The significant increase of Cu and Sb in roadside topsoil stresses the need for metal transport studies as well as effect studies of these metals. Metals emitted due to decelerating activities were not correlated to elevated concentrations near road junctions. Emission patterns of traffic-related metals alongside roads are crucial in order to be able to evaluate the optimal localization of storm water treatment ponds.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • Ayres, R. U. and Rod, S. R.: 1986, ‘Patterns of pollution in the Hudson-Raritan basin’, Environment 28, 14–43.

    Google Scholar 

  • Bäckström, M., Karlsson, S. and Allard, B.: 2004, ‘Metal leachability and anthropogenic signal in roadside soils estimated from sequential extraction and stable lead isotopes’, Environ. Monit. Assess. 90, 135–160.

    Article  Google Scholar 

  • Bergbäck, B. and Sörme, L.: 1998, ‘Metallflöden via trafik i Stockholm’, Report, SNV 4952, Swedish Environmental Protection Agency, Stockholm (in Swedish).

  • Bergbäck, B., Johansson, K. and Mohlander, U.: 2001, ‘Urban metal flows —a case study of Stockholm’, Water Air Soil Pollut. Focus 1, 3–24.

    Article  Google Scholar 

  • Cadle, S., Mulawa, P., Hunsanger, E., Nelson, K., Ragazzi, R., Barrett, R., Gallanger, G., Lawson, D., Knapp, K. and Snow, R.: 1999, ‘Composition of light-duty motor vehicle exhaust particulate matter in the Denver, Colorado area’, Environ. Sci. Technol. 33, 2328–2339.

    Article  CAS  Google Scholar 

  • Cal-Prieto, M. J., Carlosena, A., Andrade, J. M., Martinez, M. L., Muniategui, S., Lopez-Mahia, P. and Prada, D.: 2001, ‘Antimony as a tracer of the anthropogenic influence on soils and estuarine sediments’, Water Air Soil Pollut. 129, 333–348.

    Article  CAS  Google Scholar 

  • Carlosena, A., Andrade, J. M. and Prada, D.: 1998, ‘Searching for heavy metals grouping roadside soils as a function of motorized traffic influence’, Talanta 47, 753–767.

    Article  CAS  Google Scholar 

  • Davis, A.P., Shokouhian, M. and Ni, S.: 2001, ‘Loading estimates of lead, copper, cadmium, and zinc in urban runoff from specific sources’, Chemospere 44, 997–1009.

    Article  CAS  Google Scholar 

  • De Miguel, E., Llamas, J. F., Chacon, E. and Mazadiego, L. F.: 1999, ‘Sources and pathways of trace elements in urban environments: A multi-elemental qualitative approach’, Sci. Total Environ. 235, 355–357.

    Article  Google Scholar 

  • EEA: 2004, ‘EMEP/CORINAIR Emission Inventory Guidebook’, Technical Report, 30, European Environmental Agency, Copenhagen.

  • Gustafsson, M.: 2001, ‘Icke-avgasrelaterade partiklar i vägmiljön’, Report, VTI meddelande 910, Swedish National Road Administration, Linköping (in Swedish).

  • Kemp, K.: 2002, ‘Trends and sources for heavy metals in urban atmosphere’, Nucl. Instrum. Meth. Phys. Res. Sect. B-Beam Interact. Mater. Atoms 189, 227–232.

    Article  CAS  Google Scholar 

  • Legret, M. and Pagotto, C.: 1999, ‘Evaluation of pollutant loadings in the runoff waters from a major rural highway’, Sci. Total Environ. 235, 143–150.

    Article  CAS  Google Scholar 

  • Li, X. D., Poon, C. S. and Liu, P. S.: 2001, ‘Heavy metal contamination of urban soils and street dusts in Hong Kong’, Appl. Geochem. 16, 1361–1368.

    Article  CAS  Google Scholar 

  • Lindgren, Å.: 1996, ‘Asphalt wear and pollution transport’, Sci. Total Environ. 189–190, 281–286.

    Google Scholar 

  • Lindgren, Å.: 1998, ‘Road construction materials as a source of pollutants’, Doctoral Thesis, Department of Environmental Engineering, Luleå University of Technology, Luleå.

  • Malmqvist, P.-A.: 1983, ‘Urban stormwater pollutant sources —an analysis of inflows and outflows of nitrogen, phosphorus, lead, zinc and copper in urban areas’, Doctoral Thesis, Department of Sanitary Engineering, Chalmers University of Technology, Göteborg.

  • Månsson, N. and Carlsson, E.: 2002, ‘Antimony emissions of concern for the crystal glass industry’, Glasteknisk tidskrift 57, 50–53.

    Google Scholar 

  • Monaci, F., Moni, F., Lanciotti, E., Grechi, D. and Bargagli, R.: 2000, ‘Biomonitoring of airborne metals in urban environments: New tracers of vehicle emission, in place of lead’, Environ. Pollut. 107, 321–327.

    Article  CAS  Google Scholar 

  • Ozaki, H., Watanabe, I. and Kuno, K.: 2004, ‘As, Sb and Hg distribution and pollution sources in the roadside soil and dust around Kamikochi, Chubu Sangaku National Park, Japan’, Geochem. J. 38, 473–484.

    CAS  Google Scholar 

  • Palm, P.: 2002, ‘Material flow analyses in technosphere and biosphere —metals, natural resources and chemical products’, Doctoral Thesis, Department of Civil and Environmental Engineering, Royal Institute of Technology, Stockholm.

  • Peltola, P. and Åstrom, M.: 2003, ‘Urban geochemistry: A multimedia and multielement survey of a small town in northern Europe’, Environ. Geochem. Health 25, 397–419.

    Article  CAS  Google Scholar 

  • Saint' Pierre, T. D., Dias, L. F., Maia, S. M. and Curtius, A. J.: 2004, ‘Determination of Cd, Cu, Fe, Pb and Tl in gasoline as emulsion by electrothermal vaporization inductively coupled plasma mass spectrometry with analyte addition and isotope dilution calibration techniques’, Spectroc. Acta Pt. B-Atom. Spectr. 59, 551–558.

    Article  Google Scholar 

  • San Miguel, G., Fowler, G. D. and Sollars, C. J.: 2002, ‘The leaching of inorganic species from activated carbons produced from waste tyre rubber’, Water Res. 36, 1939–1946.

    Article  CAS  Google Scholar 

  • Sederholm, B.: 2001, ‘Klassificering av korrosiviteten hos olika bromiljöer genom mätning av korrosionshastigheten hos kolstål och zink’, Report, 2001:1, Swedish Corrosion Institute, Stockholm (In Swedish).

  • SEPA: 1999, ‘Contaminated sites’, Report, 4918, Swedish Environmental Protection Agency, Stockholm (in Swedish).

  • Sörme, L., Bergbäck, B. and Lohm, U.: 2001, ‘Goods in the anthroposphere as a metal emission source ’, Water Air Soil Pollut. Focus 1, 213–227.

    Google Scholar 

  • Stellpflug, J.: 2002, ‘Ausgebremst —Test Bremsbeläge’, Öko-test —Richtig Gut Leben 72.

  • Sternbeck, J., Sjödin, A. and Andreasson, K.: 2002, ‘Metal emissions from road traffic and the influence of resuspension —results from two tunnel studies’, Atmos. Environ. 36, 4735–4744.

    Article  CAS  Google Scholar 

  • von Uexkull, O., Skerfving, S., Doyle, R. and Braungart, M.: 2005, ‘Antimony in brake pads —a carcinogenic component?’, J. Clean Prod. 13, 19–31.

    Article  Google Scholar 

  • Weckwerth, G.: 2001, ‘Verification of traffic emitted aerosol components in the ambient air of Cologne (Germany)’, Atmos. Environ. 35, 5525–5536.

    Article  CAS  Google Scholar 

  • Westerlund, K. -G.: 2001, ‘Metal emissions from Stockholm traffic —Wear of brake linings’, Reports from SLB-analys, 2:2001, Environment and Health Protection Administration in Stockholm, Stockholm.

  • Yeung, Z. L. L., Kwok, R. C. W. and Yu, K. N.: 2003, ‘Determination of multi-element profiles of street dust using energy dispersive X-ray fluorescence (EDXRF)’, Appl. Radiat. Isot. 58, 339–346.

    Article  CAS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to David Hjortenkrans.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Hjortenkrans, D., Bergbäck, B. & Häggerud, A. New Metal Emission Patterns in Road Traffic Environments. Environ Monit Assess 117, 85–98 (2006). https://doi.org/10.1007/s10661-006-7706-2

Download citation

  • Received:

  • Accepted:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10661-006-7706-2

Keywords

Navigation