Skip to main content

Advertisement

Log in

The effects of irrigation and fertilization on the migration and transformation processes of main chemical components in the soil profile

  • Original Paper
  • Published:
Environmental Geochemistry and Health Aims and scope Submit manuscript

Abstract

Understanding the changes in chemical composition of soil plays an important role in effective control of irrigation and fertilization in agricultural productions, which further protects the groundwater quality and predicts its evolution. Field trials were conducted from 2014 to 2016 to investigate the impacts of irrigation and fertilization on mineral composition transformation in the soil profile. Based on HYDRUS-HP1 and Visual MINTEQ, this paper simulated and computed the migration and transformation of chemical components during the irrigation and fertilization in the vadose zone soil of Jinghuiqu district. The results showed that when the nitrogen fertilizer entered the soil, the urea was hydrolyzed to NH4+ and it was nitrified as NO2, which caused pH value to drop around the first 4 days after irrigation, and rise slightly on the 12th day. Due to the fact that soil belongs to calcareous soil, concentration of CaCO3 and other carbonates (Mg or Na in sodic soils) could buffer the soil pH well above 8.5. Thus, on the 30th day of the post-irrigation the pH reached the same level as it was before irrigation. The change in pH resulted in the main ions reacting, dissolving and precipitating simultaneously in the soil profile. The concentrations of Ca2+, Mg2+ and HCO3 had significant correlations with the increasing ammonia nitrogen hydrolyzed from urea, and this process is accompanied with the saturation index of minerals and the main ion content changing. At the same time, the varying temperature action on pH of the soil was higher in summer than that in winter. Thus, the irrigation, fertilization and temperature had affected pH and main chemical components in the soil.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6

Similar content being viewed by others

References

  • Alekseeva, T., Alekseev, A., Xu, R. K., Zhao, A. Z., & Kalinin, P. (2011). Effect of soil acidification induced by a tea plantation on chemical and mineralogical properties of alfisols in eastern china. Environmental Geochemistry and Health,33(2), 137–148.

    CAS  Google Scholar 

  • Allison, J. D. (1991). Minteqa2/peodwefa2, a geochemical assessment model for environmental systems. Version Users Manual,37(106), 371–383.

    Google Scholar 

  • Appelo, C. A. J., & Postma, D. (2005). Geochemistry, groundwater, and pollution (2nd ed.). Rotterdam: A.A. Balkema.

    Google Scholar 

  • Augusto, L., Turpault, M. P., & Ranger, J. (2000). Impact of forest tree species on feldspar weathering rates. Geoderma,96(3), 215–237.

    Google Scholar 

  • Ayora, C., Taberner, C., Saaltink, M. W., & Carrera, J. (1998). Genesis of dedolomites: A discussion based on reactive transport modeling. Journal of Hydrology,209(1–4), 346–365.

    CAS  Google Scholar 

  • Barakat, M., Cheviron, B., & Angulo-Jaramillo, R. (2016). Influence of the irrigation technique and strategies on the nitrogen cycle and budget: A review. Agricultural Water Management,178, 225–238.

    Google Scholar 

  • Beckurts, H., & Frerichs, H. (2001). The effect of soil pH on utilization of nitrogen fertilizer by spring barley in the year of application and in the following year. Scientia Agriculturae Bohemica,32(2), 85–95.

    Google Scholar 

  • Berner, R. A., Rao, J. L., Chang, S., O’Brien, R., & Keller, C. K. (1998). Seasonal variability of adsorption and exchange equilibria in soil waters. Aquatic Geochemistry,4(2), 273–290.

    CAS  Google Scholar 

  • Bloom, P. R. (2000). Soil pH and pH buffering. In M. E. Sumner, et al. (Eds.), Handbook of soil science (pp. B333–B352). Boca Raton, FL: CRC Press.

    Google Scholar 

  • Charlton, S. R., & Parkhurst, D. L. (2011). Modules based on the geochemical model PHREEQC for use in scripting and programming languages. Computers & Geosciences,37(10), 1653–1663.

    CAS  Google Scholar 

  • Chen, J., Wu, H., Qian, H., & Li, X. (2016). Challenges and prospects of sustainable groundwater management in an agricultural plain along the silk road economic belt, north-west China. International Journal of Water Resources Development,34, 1–15.

    Google Scholar 

  • Clément, J. C., Aquilina, L., Bour, O., Plaine, K., Burt, T. P., & Pinay, G. (2003). Hydrological flowpaths and nitrate removal rates within a riparian floodplain along a fourth-order stream in brittany (France). Hydrological Processes,17(6), 1177–1195.

    Google Scholar 

  • Davis, J. A., Yabusaki, S. B., Steefel, C. I., Zachara, J. M., Curtis, G. P., Redden, G. D., et al. (2004). Assessing conceptual models for subsurface reactive transport of inorganic contaminants. Eos Transactions American Geophysical Union,85(44), 449–455.

    Google Scholar 

  • Dijkshoorn, W., Lampe, J., & Broekhoven, L. V. (1983). The effect of soil pH and chemical form of nitrogen fertilizer on heavy-metal contents in ryegrass. Fertilizer Research,4(1), 63–74.

    CAS  Google Scholar 

  • Durner, W., & Flühler, H. (2006). Soil hydraulic properties. Encyclopedia of hydrological sciences. London: Wiley.

    Google Scholar 

  • Fan, X., Thompson, B., & Wang, L. (1999). Effects of sample size, estimation methods, and model specification on structural equation modeling fit indexes. Structural Equation Modeling A Multidisciplinary Journal,6(1), 56–83.

    Google Scholar 

  • Fenn, L. B., & Wu, E. (1987). Effect of ammonium fertilizer on NH3 loss and Ca, Mg, ammonium and nitrate content in a calcareous soil solution. Biology and Fertility of Soils,5(2), 171–174.

    CAS  Google Scholar 

  • Genuchten, M. T. V. (1980). A closed-form equation for predicting the hydraulic conductivity of unsaturated soils. Soil Science Society of America Journal,44(44), 892–898.

    Google Scholar 

  • Gheysari, M., Mirlatifi, S. M., Homaee, M., Asadi, M. E., & Hoogenboom, G. (2009). Nitrate leaching in a silage maize field under different irrigation and nitrogen fertilizer rates. Agricultural Water Management,96(6), 946–954.

    Google Scholar 

  • Guo, S., Jiang, R., Qu, H., Wanf, Y., Misselbrook, T., Gunina, A., et al. (2019). Fate and transport of urea-N in a rain-fed ridge-furrow crop system with plastic mulch. Soil & Tillage Research,186, 214–223.

    Google Scholar 

  • Gustafsson, J. P. (2012). Visual minteq 3.0 user guide. Department of Land & Water Resources Engineering.

  • Henriksen, A., & Selmer-Olsen, A. R. (1970). Automatic methods for determining nitrate and nitrite in water and soil extracts. Analyst,95(1130), 514–518.

    CAS  Google Scholar 

  • Hilten, R. N., Lawrence, T. M., & Tollner, E. W. (2008). Modeling stormwater runoff from green roofs with HYDRUS-1D. Journal of Hydrology,358(3), 288–293.

    Google Scholar 

  • Hinsinger, P., Plassard, C., Tang, C., & Jaillard, B. (2003). Origins of root-mediated pH changes in the rhizosphere and their responses to environmental constraints: A review. Plant and Soil,248(1–2), 43–59.

    CAS  Google Scholar 

  • Jacques, D., Šimůnek, J., Mallants, D., & Genuchten, M. T. V. (2006). Operator-splitting errors in coupled reactive transport codes for transient variably saturated flow and contaminant transport in layered soil profiles. Journal of Contaminant Hydrology,88(3), 197–218.

    CAS  Google Scholar 

  • Jacques, D., Šimůnek, J., Mallants, D., & Genuchten, M. T. V. (2008). Modelling coupled water flow, solute transport and geochemical reactions affecting heavy metal migration in a podzol soil. Geoderma,145(3), 449–461.

    CAS  Google Scholar 

  • Jacques, D., Simunek, J., Mallants, D., & Van Genuchten, R. (2010). Simulating water flow, heat and solute transport and biogeochemistry in variably-saturated porous media using HP1. Egu General Assembly,74(12), 4623.

    Google Scholar 

  • Jacques, D., Smith, C., Simunek, J., & Smiles, D. (2012). Inverse optimization of hydraulic, solute transport, and cation exchange parameters using HP1 and UCODE to simulate cation exchange. Journal of Contaminant Hydrology,142–143, 109–125.

    Google Scholar 

  • Jalali, M. (2007). Assessment of the chemical components of Famenin groundwater, western Iran. Environmental Geochemistry and Health,29(5), 357–374.

    CAS  Google Scholar 

  • Jansen, B., Nierop, K. G. J., & Verstraten, J. M. (2002). Influence of pH and metal/carbon ratios on soluble organic complexation of Fe(ii), Fe(iii) and Al(iii) in soil solutions determined by diffusive gradients in thin films. Analytica Chimica Acta,454(2), 259–270.

    CAS  Google Scholar 

  • Jarvis, S. C., & Hatch, D. J. (1994). Potential for denitrification at depth below long-term grass swards. Soil Biology & Biochemistry,26(12), 1629–1636.

    CAS  Google Scholar 

  • Kohler, M., Curtis, G. P., Kent, D. B., & Davis, J. A. (1996). Experimental investigation and modeling of uranium (vi) transport under variable chemical conditions. Water Resources Research,32(12), 3539–3551.

    CAS  Google Scholar 

  • Langmuir, D. (1997). Aqueous environmental geochemistry. Upper Saddle River, New Jersry: Prentice-Hall, Inc.

    Google Scholar 

  • Lindsay, W. L. (1979). Chemical equilibria in soils. Clays and Clay Minerals,28(4), 319-319.

    Google Scholar 

  • Liu, X., Šimůnek, J., Li, L., & He, J. (2013). Identification of sulfate sources in groundwater using isotope analysis and modeling of flood irrigation with waters of different quality in the Jinghuiqu district of china. Environmental Earth Sciences,69(5), 1589–1600.

    Google Scholar 

  • Liu, X. H., Gao, W. D., Sun, S. J., Hu, A. Y., He, Y., & He, S. S. (2019). Responses of soil water dynamic processes and groundwater recharge to irrigation intensity and antecedent moisture in the vadose zone. Hydrological Processes,33(5), 849–863.

    Google Scholar 

  • Liu, X. H., & Wang, R. (2016). Research on impact process of irrigation amount on moisture migration and retention in vadose zone. Agricultural Research in the Arid Areas,34(5), 262–268. (in Chinese with English abstract).

    Google Scholar 

  • Lottermoser, B. G. (2012). Effect of long-term irrigation with sewage effluent on the metal content of soils, Berlin, Germany. Environmental Geochemistry and Health,34(1), 67–76.

    CAS  Google Scholar 

  • Ludwig, B., Beese, F., & Michel, K. (2010). Modelling cation transport and pH buffering during unsaturated flow through intact subsoils. European Journal of Soil Science,56(5), 635–645.

    Google Scholar 

  • Martin, C., Aquilina, L., Gascuel-Odoux, C., Molénat, J., Faucheux, M., & Ruiz, L. (2004). Seasonal and interannual variations of nitrate and chloride in stream waters related to spatial and temporal patterns of groundwater concentrations in agricultural catchments. Hydrological Processes,18(7), 1237–1254.

    Google Scholar 

  • Matijevic, L., Romic, D., & Romic, M. (2014). Soil organic matter and salinity affect copper bioavailability in root zone and uptake by Vicia faba L. plants. Environmental Geochemistry and Health,36(5), 883–896.

    CAS  Google Scholar 

  • Meeussen, J. C. L., Scheidegger, André, Hiemstra, T., Van Riemsdijk, W. H., & Borkovec, M. (1996). Predicting multicomponent adsorption and transport of fluoride at variable pH in a goethite–silica sand system. Environmental Science and Technology,30(2), 481–488.

    CAS  Google Scholar 

  • Michel, K., Herrmann, S., & Ludwig, B. (2010). Modelling chemical and biological reactions during unsaturated flow in silty arable soils. Geoderma,156(3–4), 293–301.

    CAS  Google Scholar 

  • Muthén, B. (1984). A general structural equation model with dichotomous, ordered categorical, and continuous latent variable indicators. Psychometrika,49(1), 115–132.

    Google Scholar 

  • Oren, A., & Steinberger, Y. (2008). Coping with artifacts induced by CaCO3–CO2–H2O equilibria in substrate utilization profiling of calcareous soils. Soil Biology & Biochemistry,40(10), 2569–2577.

    CAS  Google Scholar 

  • Öztürk, H. S., & Özkan, İ. (2004). Effects of evaporation and different flow regimes on solute distribution in soil. Transport in Porous Media,56(3), 245–255.

    Google Scholar 

  • Parkhurst, D. L. (1995). User guide to PHREEQC-A computer program for speciation, reaction path, advective-transport, and inverse geochemical calculations. Center for Integrated Data Analytics Wisconsin Science Center.

  • Parkhurst, D. L., & Appelo, C. A. J. (1999). User’s guide to PHREEQC-A computer program for speciation, batch-reaction, one-dimensional transport, and inverse geochemical calculations (p. 99). U.S. Geological Survey Water Resources Investigations Report.

  • Parshotam, H., Gericke, G., Ngila, J. C., & Mishra, S. (2016). A study of seasonal effects on metal-nom interactions and the impact of CaCO3 precipitation potentials using visual MINTEQ, in raw and cooling water. Water SA,42(1), 171–175.

    CAS  Google Scholar 

  • Pauln, N., & Su, N. (2010). Soil pH buffering capacity: A descriptive function and its application to some acidic tropical soils. Soil Research,48(3), 201–207.

    Google Scholar 

  • Penman, H. L. (1948). Natural evaporation from open water, bare soil and grass. Proceedings of the Royal Society of London,193(1032), 120–145.

    CAS  Google Scholar 

  • Phillip, P. L. (1984). The Berthelot or indophenol reaction and its use in the analytical chemistry of nitrogen. A review. Analyst,109(5), 549–568.

    Google Scholar 

  • Refsgaard, J. C., Thorsen, M., Jensen, J. B., Kleeschulte, S., & Hansen, S. (1999). Large scale modelling of groundwater contamination from nitrate leaching. Journal of Hydrology,221(3), 117–140.

    CAS  Google Scholar 

  • Ruan, J., Ma, L., & Shi, Y. (2006). Aluminium in tea plantations: Mobility in soils and plants, and the influence of nitrogen fertilization. Environmental Geochemistry and Health,28(6), 519–528.

    CAS  Google Scholar 

  • Simunek, J., He, C., Pv ang, L., & Bradford, S. A. (2006). Colloid-facilitated solute transport in variably saturated porous media. Vadose Zone Journal,5(3), 1035.

    CAS  Google Scholar 

  • Šimůnek, J., Jacques, D., Van Genuchten, R., & Mallants, D. (2010). Multicomponent geochemical transport modeling using HYDRUS-1D and HP1. Jawra Journal of the American Water Resources Association,42(6), 1537–1547.

    Google Scholar 

  • Simunek, J., Saito, H., Sakai, M., & Genuchten, T. M. (2009). The HYDRUS-1D software package for simulating the one-dimensional movement of water, heat, and multiple solutes in variably-saturated media (p. 68). Department of Environmental Sciences University of California Riverside.

  • Šimůnek, J., & Valocchi, A. J. (2002). Geochemical transport (3rd ed.). In J. H. Dane & G. C. Topp (Eds.), Methods of Soil Analysis, Part 1, Physical Methods, SSSA, Madison, Wisconsin, Chapter 6.9 (pp. 1511–1536).

  • Slattery, W. J., & Ronnfeldt, G. R. (1992). Seasonal variation of pH, aluminium, and manganese in acid soils from north-eastern victoria. Australian Journal of Experimental Agriculture,32(8), 1105–1112.

    CAS  Google Scholar 

  • Slessarev, E. W., Lin, Y., Bingham, N. L., Johnson, J. E., Dai, Y., Schimel, J. P., et al. (2016). Water balance creates a threshold in soil pH at the global scale. Nature,540, 567–569.

    CAS  Google Scholar 

  • Sparling, G. P., & West, A. W. (1990). A comparison of gas chromatography and differential respirometer methods to measure soil respiration and to estimate the soil microbial biomass. Pedobiologia,34, 103–112.

    CAS  Google Scholar 

  • Suntari, R., Retnowati, R., Soemarno, S., & Munir, M. (2013). Study on the release of N-available (NH4 + and NO3 ) of urea-humate. International Journal of Agriculture & Forestry,3(6), 209–219.

    Google Scholar 

  • Tafteh, A., & Sepaskhah, A. R. (2012). Application of HYDRUS-1D model for simulating water and nitrate leaching from continuous and alternate furrow irrigated rapeseed and maize fields. Agricultural Water Management,113(10), 19–29.

    Google Scholar 

  • Tavakkoli, A. R., & Oweis, T. Y. (2004). The role of supplemental irrigation and nitrogen in producing bread wheat in the highlands of Iran. Agricultural Water Management,65(3), 225–236.

    Google Scholar 

  • Vogeler, I., Scotter, D. R., Green, S. R., & Clothier, B. E. (1997). Solute movement through undisturbed soil columns under pasture during unsaturated flow. Soil Research,35(5), 1153–1163.

    CAS  Google Scholar 

  • Wang, H., Ju, X., Wei, Y., Li, B., Zhao, L., & Hu, K. (2011). Simulation of bromide and nitrate leaching under heavy rainfall and high-intensity irrigation rates in North China plain. Agricultural Water Management,97(10), 1646–1654.

    Google Scholar 

  • Wang, X., Liu, S., Zhang, S., Li, H., Ma, B., et al. (2018). Localized ammonium and phosphorus fertilization can improve cotton lint yield by decreasing rhizosphere soil pH and salinity. Filed Crops Research,217, 75–81.

    Google Scholar 

  • Wissmeier, L., & Barry, D. A. (2009). Effect of mineral reactions on the hydraulic properties of unsaturated soils: Model development and application. Advances in Water Resources,32(8), 1241–1254.

    CAS  Google Scholar 

  • Yang, Y., Wang, Z., Hu, Y., & Zeng, Z. (2017). Irrigation frequency alters the abundance and community structure of ammonia-oxidizing archaea and bacteria in a northern Chinese upland soil. European Journal of Soil Biology,83, 34–42.

    CAS  Google Scholar 

  • Yu, H., He, Z. W., Kong, B., Weng, Z. Y., & Shi, Z. M. (2016). The spatial relationship between human activities and C, N, P, S in soil based on landscape geochemical interpretation. Environmental Geochemistry and Health,38, 381–398.

    CAS  Google Scholar 

  • Zhang, J., Cai, Z., Yang, W., Zhu, T., Yu, Y., Yan, X., et al. (2012). Long-term field fertilization affects soil nitrogen transformations in a rice-wheat-rotation cropping system. Journal of Plant Nutrition and Soil Science,175(6), 939–946.

    CAS  Google Scholar 

  • Zhang, Y., Jiang, J., & Chen, M. (2008). Minteq modeling for evaluating the leaching behavior of heavy metals in MSWI fly ash. Journal of Environmental Science,20(11), 1398–1402.

    CAS  Google Scholar 

Download references

Acknowledgements

This research was supported by the National Natural Science Foundation of China (41273104, 41877179 and 41472222), the Natural Basic Research Program of Shaanxi Province (2012K12-03-06), the Central University Special Fund (310829163405), the urban construction technique project of Xi’an (SJW2017-11) and by the Fund Project of Shaanxi Key Laboratory of Land Consolidation.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Xiuhua Liu.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Hu, A., Yu, Z., Liu, X. et al. The effects of irrigation and fertilization on the migration and transformation processes of main chemical components in the soil profile. Environ Geochem Health 41, 2631–2648 (2019). https://doi.org/10.1007/s10653-019-00298-3

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10653-019-00298-3

Keywords

Navigation