Abstract
A series of rare earth zeolites Ln–ZSM-5 (Ln = La, Ce, Pr, Nd) were synthesized directly via a one-step hydrothermal method. The obtained zeolites were used as support and applied in low-temperature CO oxidation. The influence of various factors such as rare earth types, rare earth contents, particle sizes of molecular sieve, and silica alumina ratios, etc., on the catalytic activity of CO oxidation were investigated in detail. The results showed that low silica small size Ce–ZSM-5 (1 % Ce content) had the highest activity. The results also showed that Ce–ZSM-5 zeolite prepared by one-step direct synthesis was more suitable as catalytic support than ZSM-5 or Ce/ZSM-5 zeolite, prepared by impregnation of ZSM-5 with Ce.
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Acknowledgments
The financial support of The National Basic Research Program of China (2013CB933201), West Light Foundation of The Chinese Academy of Sciences, Science and Technology Program of Gansu Province (1204GKCA063), Science and Technology Program of Lanzhou City (2012-2-103) is gratefully acknowledged.
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Han, W., Tang, Z., Zhang, P. et al. Study of One Step Synthesis of Rare Earth Zeolite (Ln–ZSM-5) and Application for Low Temperature CO Catalytic Oxidation. Catal Surv Asia 17, 147–155 (2013). https://doi.org/10.1007/s10563-013-9156-5
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DOI: https://doi.org/10.1007/s10563-013-9156-5