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Boosting CO Hydrogenation Performance of Facile Organics Modified Iron Oxide/Reduced Graphene Oxide Catalysts

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Abstract

Organics including terephthalic acid and glucose are added to selectively adsorb on iron oxide or graphene oxide, which can further modify the structure properties and metal-support interaction of iron oxide/reduced graphene oxide catalysts. The proper metal-support interaction is favorable for the reduction and carburization of iron oxide to form more active sites for CO hydrogenation. Thus, higher CO conversion and heavier hydrocarbons are achieved over organics modified catalysts. This simple, eco-friendly and economic viable method opens a new avenue from molecular level for the design of highly active supported catalysts.

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Acknowledgements

This research is supported by the National Natural Science Foundation of China (Grant Nos. 21902001, U1832165 and U1632273), Anhui Provincial Natural Science Foundation (Grant No.2008085QB85) and Key Research and Development Program of Anhui Provincial (Grant Nos. 202004a05020015, 006233172019). We also thank Synfuels China Co., Ltd.

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Authors and Affiliations

  1. School of Chemistry and Chemical Engineering, Anhui University, Hefei, 230601, Anhui, China

    Yuxue Wei, Zhiyuan Fu, Lisheng Guo, Mengdie Cai, Song Sun & Chenghua Zhang

  2. State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan, 030001, PR China

    Dan Luo, Linlin Yan, Caiping Ma & Chenghua Zhang

  3. National Energy Center for Coal To Liquids, Synfuels CHINA Co., Ltd., Huairou District, Beijing, 101400, PR China

    Dan Luo, Linlin Yan, Caiping Ma & Chenghua Zhang

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  1. Yuxue Wei
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  2. Dan Luo
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  3. Linlin Yan
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  4. Caiping Ma
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  5. Zhiyuan Fu
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  8. Song Sun
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  9. Chenghua Zhang
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Correspondence to Song Sun or Chenghua Zhang.

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Wei, Y., Luo, D., Yan, L. et al. Boosting CO Hydrogenation Performance of Facile Organics Modified Iron Oxide/Reduced Graphene Oxide Catalysts. Catal Lett 152, 1835–1843 (2022). https://doi.org/10.1007/s10562-021-03768-5

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  • DOI: https://doi.org/10.1007/s10562-021-03768-5

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