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Studies of Ceria and Zirconia Promotion of Nickel Catalyst for Carbon Dioxide Reforming of Methane

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Abstract

The CO2 reforming reactions of methane were carried out using three types of Ni/δ-Al2O3s and the effects of the addition of CeO2 were examined. In this study, the addition of a high weight percentage of CeO2 focused on reducing the amount of deposited carbon. It was revealed that a high Al2O3 surface area was necessary for the effective reduction of the deposited carbon by the addition of 50% CeO2 with the lowest conversion decrease. The addition of CeO2 and ZrO2 (Ni/Al2O3(A)-CeO2(45)-ZrO2(5)) further decreased the deposited carbon to 0.14 mmol per 1 mol of produced CO at 1073 K.

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Acknowledgements

The authors thank Mr. Tomoyuki Takiyama and Ms. Aki Mouri for helping the experiments.

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Authors and Affiliations

  1. Graduate School of Science and Engineering for Research, University of Toyama, Gofuku, Toyama, 930-8555, Japan

    Tsutomu Osawa & Kiyotaka Tamagawa

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  1. Tsutomu Osawa
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  2. Kiyotaka Tamagawa
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Correspondence to Tsutomu Osawa.

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Osawa, T., Tamagawa, K. Studies of Ceria and Zirconia Promotion of Nickel Catalyst for Carbon Dioxide Reforming of Methane. Catal Lett 149, 1579–1588 (2019). https://doi.org/10.1007/s10562-019-02750-6

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  • DOI: https://doi.org/10.1007/s10562-019-02750-6

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