Skip to main content
Log in

Synthesis of carbon nanotubes using a novel catalyst derived from hydrotalcite-like Co–Al layered double hydroxide precursor

  • Published:
Catalysis Letters Aims and scope Submit manuscript

Abstract

In the present letter, for the first time, the efficacy of hydrotalcite-like layered double hydroxides (LDHs) materials as alternative and novel catalyst precursors for the synthesis of carbon nanotubes (CNTs) via catalytic chemical vapor deposition (CCVD) of acetylene was reported. Nanometer-sized cobalt particles were prepared by calcination of a single molecular LDH precursor containing cobalt (II) and aluminum (III) and following by a process of reduction. Multi-walled CNTs with uniform diameters were obtained using the as-synthesized catalyst in the reaction.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • S. Iijima (1991) Nature 354 56 Occurrence Handle10.1038/354056a0 Occurrence Handle1:CAS:528:DyaK38Xmt1Ojtg%3D%3D

    Article  CAS  Google Scholar 

  • R.H. Baughman A.A. Zakhidov W.A. Heer (2002) Science 297 787 Occurrence Handle10.1126/science.1060928 Occurrence Handle1:CAS:528:DC%2BD38XlvVyhsrw%3D

    Article  CAS  Google Scholar 

  • A. Thess R. Lee P. Nikolaev H. Dai P. Petit J. Robert C Xu Y.H. Lee S.G. Kim D.T. Colbert G. Scuseria D. Tomanek J.E. Fisher R.E. Smalley (1996) Science 273 483 Occurrence Handle1:CAS:528:DyaK28Xks1Wmurc%3D

    CAS  Google Scholar 

  • B. Kitiyanan W.E. Alvarez J.H. Harwell D.E. Resasco (2000) Chem. Phys. Lett. 317 497 Occurrence Handle10.1016/S0009-2614(99)01379-2 Occurrence Handle1:CAS:528:DC%2BD3cXhtFagsrY%3D

    Article  CAS  Google Scholar 

  • A.M. Benito Y. Maniette E. Munoz (1998) Carbon 36 681 Occurrence Handle10.1016/S0008-6223(98)00039-6 Occurrence Handle1:CAS:528:DyaK1cXkvVKrtrc%3D

    Article  CAS  Google Scholar 

  • J.P. Pinheiro M.C. Schouler P. Gadelle M. Mermoux E. Dooryhee (2000) Carbon 38 1469 Occurrence Handle10.1016/S0008-6223(00)00002-6 Occurrence Handle1:CAS:528:DC%2BD3cXktlOisrY%3D

    Article  CAS  Google Scholar 

  • J.F. Colomer C. Stephan S. Lefrant G.V. Tendeloo I. Willems Z. Konya A. Fonseca C. Laurent J.B. Nagy (2000) Chem. Phys. Lett. 317 83 Occurrence Handle10.1016/S0009-2614(99)01338-X Occurrence Handle1:CAS:528:DC%2BD3cXotlymsA%3D%3D

    Article  CAS  Google Scholar 

  • P. Piedigrosso Z. Konya J.F. Collomer A. Fonseca G.V. Tendeloo J.B. Nagy (2000) Phys. Chem. Chem. Phys 2 163 Occurrence Handle10.1039/a905622j Occurrence Handle1:CAS:528:DyaK1MXotVKgtb0%3D

    Article  CAS  Google Scholar 

  • F. Cavani F. Trifiro A. Vaccarj (1991) Catal. Today 11 173 Occurrence Handle10.1016/0920-5861(91)80068-K Occurrence Handle1:CAS:528:DyaK38XkslSmtQ%3D%3D

    Article  CAS  Google Scholar 

  • A. de Roy C. Forano K. EI Malki J.P. Besse (1992) Expanded Clays and Other Microporous Solids M.L. Occelli H. Robson (Eds) Synthesis of Microporous Materials Van Nostrand Reinhold New York

    Google Scholar 

  • Y. Huh J.Y. Lee J. Cheon Y.K. Hong J.Y. Koo T.J. Lee C.J. Lee (2003) J. Mater. Chem. 13 2297 Occurrence Handle10.1039/b304582j Occurrence Handle1:CAS:528:DC%2BD3sXmsFWhsr0%3D

    Article  CAS  Google Scholar 

  • Dresselhaus M.S. Dresselhaus G. Pimenta M.A. and Eklund P.C.in:, (ed.) pelletier M.J. (Oxford, Blackwell Science, 1999), ch. 9

  • M. Sveningsson R.E. Morjan O.A. Nerushev Y. Sato J. Bäckström E.E.B. Campbell F. Rohmund (2001) Appl. Phys. A 73 409 Occurrence Handle10.1007/s003390100923 Occurrence Handle1:CAS:528:DC%2BD3MXnvFSltL4%3D

    Article  CAS  Google Scholar 

  • M. Endo Y.A. Kim Y. Fukai T. Hayashi M. Terrones H. Terrones M.S. Dresselhaus (2001) Appl. Phys. Lett. 79 IssueID10 1531 Occurrence Handle10.1063/1.1400774 Occurrence Handle1:CAS:528:DC%2BD3MXmsFagurg%3D

    Article  CAS  Google Scholar 

  • F. Li J. Liu D.G. Evans X. Duan (2004) Chem. Mater. 16 1597 Occurrence Handle10.1021/cm035248c Occurrence Handle1:CAS:528:DC%2BD2cXit1Sqt74%3D

    Article  CAS  Google Scholar 

  • J. Pérez-Ramírez G. Mul F. Kapteijn J.A. Moulijn (2001) J. Mater. Chem. 11 821 Occurrence Handle10.1039/b009320n

    Article  Google Scholar 

  • J.J. Liu F. Li D.G. Evans X. Duan (2003) Chem. Commun. 4 542 Occurrence Handle10.1039/b212233b Occurrence Handle1:CAS:528:DC%2BD3sXhtVOns7w%3D

    Article  CAS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Rights and permissions

Reprints and permissions

About this article

Cite this article

Li, F., Tan, Q., Evans, D.G. et al. Synthesis of carbon nanotubes using a novel catalyst derived from hydrotalcite-like Co–Al layered double hydroxide precursor. Catal Lett 99, 151–156 (2005). https://doi.org/10.1007/s10562-005-2107-7

Download citation

  • Received:

  • Accepted:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10562-005-2107-7

Keywords

Navigation