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Triple Cascade Arrangement for Purifying Regenerated Uranium Hexafluoride from 232,234,236U

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Aspects of the lowering of the 232,234,236U concentration in regenerated uranium hexafluoride are considered. A three-cascade purification scheme including dilution with waste uranium or natural raw material at an intermediate stage is proposed. A computational experiment was performed to determine the parameters of purification of regenerated uranium hexafluoride of each isotope 232,234,236U. It is shown that the overall product formed after dilution with natural raw materials and enrichment in a third cascade satisfies the ASTM C996-20 specifications for enriched commercial uranium hexafluoride.

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References

  1. V. V. Vodolazskikh, V. A. Kozlov, V. I. Mazin, et al., Patent RF No. 2282904, “Method of isotopic reduction of regenerated uranium,” subm. Aug. 27, 2006, Byull. Izobret. Polezn. Modeli, No. 24, 549–550 (2006).

  2. A. A. Orlov, A. V. Kravchenko, E. S. Titov, and A. Ya. Lebedev, “Review of promising methods of uranium recycling in the nuclear fuel cycle,” Usp. Vyssh. Uchebn. Zaved. Fizika, 58, No. 2/2, 35–40 (2015).

    Google Scholar 

  3. V. I. Mazin, V. V. Vodolazskikh, V. A. Zhurin, et al., Patent RF No. 2497210, “Method of isotopic reduction of regenerated uranium,” subm. Oct. 27, 2013, Byull. Izobret. Polezn. Modeli, No. 30, 714–715 (2013).

  4. V. A. Palkin, “Separation of uranium isotopes in a cascade with intermediate selection,” Perspekt. Mater., No. 8, 11–14 (2010).

  5. A. Yu. Smirnov and G. A. Sulaberidze, “Enrichment of regenerated uranium with simultaneous dilution of 232–236U with natural raw and waste uranium,” At. Energiya, 117, No. 1, 36–41 (2014); Atomic Energy, 117, No. 1, 44–51 (2014).

  6. A. Yu. Smirnov, G. A. Sulaberidze, A. A. Dudnikov, and V. A. Nevinitsa, “Enrichment of regenerated uranium in a gas centrifuge cascade with simultaneous dilution of 232–236U by waste and low-enrichment uranium,” At. Energiya, 125, No. 5, 287–290 (2017); Atomic Energy, 125, No. 5, 353–357 (2017).

  7. A. Yu. Smirnov, V. E. Gusev, G. A. Sulaberidze, and V. A. Nevinitsa, “A method to enrich reprocessed uranium with various initial contents of even-numbered isotopes,” AIP Conf. Proc., 2101, 020006 (2019).

    Article  Google Scholar 

  8. Management of High Enriched Uranium for Peaceful Purposes. Status and Trends, IAEA, Vienna (2005).

    Google Scholar 

  9. V. A. Palkin, “Multistream cascades for separation of multicomponent isotopic mixtures,” At. Energiya, 119, No. 2, 101–105 (2015); Atomic Energy, 119, No. 2, 125–131 (2015).

  10. V. A. Palkin, N. A. Sbitnev, and E. S. Frolov, “Calculation of the optimal parameters of a cascade for separating a multicomponent mixture of isotopes,” At. Energiya, 92, No. 2, 130–133 (2002); Atomic Energy, 92, No. 2, 141–146 (2002).

  11. R. Hooke and T. A. Jeeves,”Direct search solution of numerical and statistical problems,” J. Ass. Comput. Mach., No. 8, 212–229 (1961).

  12. A. A. Sazykin, “Thermodynamic approach to isotope separation,” in: Isotopes: Properties, Production, and Application, V. Yu. Baranov (ed.), IzdAT, Moscow (2000), pp. 72–108.

    Google Scholar 

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Correspondence to V. A. Palkin.

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Translated from Atomnaya Énergiya, Vol. 132, No. 6, pp. 346–352, June, 2022.

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Palkin, V.A. Triple Cascade Arrangement for Purifying Regenerated Uranium Hexafluoride from 232,234,236U. At Energy 132, 364–370 (2022). https://doi.org/10.1007/s10512-023-00961-0

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  • DOI: https://doi.org/10.1007/s10512-023-00961-0

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