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230U Yield Measurement on 3,4He-Irradiated ThO2 Targets

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Atomic Energy Aims and scope

The 230U yield in the direct reactions 232Th(3He, 5n)230U and 232Th(4He, 6n)230U on thick ThO2 targets irradiated by 65 and 55 MeV nuclei 3,4He was measured and compared with calculations. The experimental yield of 230U in the reaction 232Th(3He, 5n)230U is approximately 10 times higher than the value computed using the constants from TENDL-2019. The experimental yield of 230U in the reaction 232Th(4He, 6n)230U the same, to within t5he limits of error, as the computed value. Comparing the experimental and computed yield in the reaction 232Th(4He, 6n)230U with the cross section obtained by the ALICA program (USA) showed that the computed cross section is incorrect and the prognoses for 230U production based on it are unsubstantiated. It is concluded that the reactions 232Th(3He, 5n)230U and 232Th(4He, 6n)230U are inefficient for 230U production in the U-150 cyclotron at the NRC Kurchatov Institute in amounts required for clinical applications.

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References

  1. A. Morgenstern, C. Apostolidis, F. Bruchertseifer, et al., “Cross-sections of the reaction 232Th(p, 3n)230Pa for production of 230U for targeted alpha therapy,” Appl. Rad. Isot., 66, 1275–1280 (2008).

    Article  Google Scholar 

  2. C. Duchemin, A. Guertin, F. Haddad, et al., “232Th(d, 4n)230Pa cross-section measurements at ARRONAX facility for the production of 230U,” Nucl. Med. Biolog., 41, 19–22 (2014).

    Article  Google Scholar 

  3. A. Morgenstern, K. Abbas, F. Simonelli, et al., “Measurement and modeling of the cross sections for the reaction 232Th(3He, 3n)230U,” Phys. Rev. C, 87, 064602 (2013).

    Article  ADS  Google Scholar 

  4. A. Morgenstern, O. Lebeda, J. Stursa, et al., “Production of 230U/226Th for targeted alpha therapy via proton irradiation of 231Pa,” Anal. Chem., 80, 8763 (2008).

    Article  Google Scholar 

  5. A. Morgenstern, O. Lebeda, J. Stursa, et al., “Cross sections of the reaction 231Pa(d, 3n)230U for the production of 230U/226Th for targeted α-therapy,” Phys. Rev. C, 80, 054612 (2009).

    Article  ADS  Google Scholar 

  6. E. Browne and J. Tuli, “Nuclear data sheets for A = 230,” Nucl. Data Sheets, 113, 2113 (2012).

    Article  ADS  Google Scholar 

  7. A. Morgenstern, C. Apostolidis, R. Molinet, et al., Patent No. US 7794691 B2, “Radionuclides for medical use,” publ. Sep. 14, 2010.

  8. A. Koning, and D. Rochman, “Modern nuclear data evaluation with the TALYS code system,” Nucl. Data Sheets, 113, 2841–2934 (2012).

    Article  ADS  Google Scholar 

  9. J. Ziegler, M. Ziegler, and J. Biersack, “SRIM – the stopping and range of ions in matter,” Nucl. Instrum. Meth., 268, 1818–1823 (2010).

    Article  Google Scholar 

  10. S. Singh, A. Jain, and J. Tuli, “Nuclear data sheets for A = 222,” Nucl. Data Sheets, 112, 2851 (2011).

    Article  ADS  Google Scholar 

  11. E. Browne and J. Tuli , “Nuclear data sheets for A = 231,” Nucl. Data Sheets, 114, 751 (2013).

    Article  ADS  Google Scholar 

  12. B. Singh, M. Basunia, M. Martin, et al., “Nuclear data sheets for A = 218,” Nucl. Data Sheets, 160, 405 (2019).

    Article  ADS  Google Scholar 

  13. A. Knight, E. Eitheim, A. Nelson, and M. Schultz, “A simple rapid method to separate uranium, thorium, and protactinium for U-series age-dating of materials,” J. Environ. Radioact., 134, 66–74 (2014).

    Article  Google Scholar 

  14. B. Singh, J. Tuli, and E. Browne, “Nuclear data sheets for A = 233,” Nucl. Data Sheets, 170, 499 (2020).

    Article  ADS  Google Scholar 

Download references

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Correspondence to T. Yu. Malamut.

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Translated from Atomnaya Énergiya, Vol. 132, No. 5, pp. 279–282, May, 2022.

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Smirnov, A.A., German, M.N., Zagryadsky, V.A. et al. 230U Yield Measurement on 3,4He-Irradiated ThO2 Targets. At Energy 132, 294–297 (2022). https://doi.org/10.1007/s10512-023-00952-1

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  • DOI: https://doi.org/10.1007/s10512-023-00952-1

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