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Investigation of Plasma-Chemical Synthesis of Complex Oxide Compositions for Dispersed Uranium-Plutonium Mixed Fuel

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Atomic Energy Aims and scope

The central problems of using ceramic nuclear fuel fabricated from uranium dioxide enriched in uranium-235 are low thermal conductivity, high disposal costs, and limited natural reserves of uranium-235. A potential direction for the further development of nuclear power in Russia is the use of mixed uranium-plutonium dispersion fuel consisting of fissile materials (uranium and plutonium dioxides) uniformly distributed in a matrix of metal oxides, which have a high thermal conductivity and a low neutron absorption cross section. The methods used to obtain complex oxide compositions (sol-gel, separate preparation, mechanical mixing, and others) are multi-stage, do not provide a uniform distribution of phases, and are characterized by high energy and labor costs. This article proposes a plasma-chemical method of synthesizing nanosized complex oxide compositions in an air-plasma flow from dispersed water-organic nitrate solutions, which provides a significant reduction in energy consumption, a uniform distribution of phases, and the required phase composition.

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References

  1. D. M. Skorov, Yu. F. Bychkov, and A. M. Dashkovskii, Reactor Materials Science, Atomizdat, Moscow (1979).

    Google Scholar 

  2. A. G. Samoilov, A. I. Kashtanov, and V. S. Volkov, Dispersion Fuel Elements of Nuclear Reactors, Atomizdat, Moscow (1965).

    Google Scholar 

  3. S. V. Alekseev, V. A. Zaitsev, and S. S. Tolstoukhov, Dispersion Nuclear Fuel, Technosfera, Moscow (2015).

    Google Scholar 

  4. Yu. N. Tumanov, Plasma and High-Frequency Processes for Obtaining and Processing Materials in the Nuclear Fuel Cycle: Present and Future, Fizmatlit, Moscow (2003).

    Google Scholar 

  5. A. G. Karengin, A. A. Karengin, I. Yu. Novoselov, and N. V. Tundeshev, “Calculation and optimization of plasma utilization process of infl ammable wastes after spent nuclear fuel recycling,” Adv. Mater. Res., 1040, 433–436 (2014).

    Article  Google Scholar 

  6. I. Yu. Novoselov, A. G, Karengin, and R. G. Babaev, “Simulation of uranium and plutonium oxides compounds obtained in plasma,” ITMA-2017, Tomsk, Russia, Sept. 18–22, 2017, in: AIP Conf. Proc., 1938 (2018), p. 020016.

  7. I. Yu. Novoselov, A. G. Karengin, I. V. Shamanin, et al., “Plasmachemical synthesis of nanopowders of yttria and zirconia from dispersed water–salt–organic mixtures,” ibid. p. 020010.

  8. V. F. Myshkin, V. A. Khan, M. Tichy, et al., “Particularities of Cu and Zn nanoparticles formation in a magnetic field,” ITMA-2018, Tomsk, Russia, Nov. 19–23, 2018, in: AIP Conf. Proc., 2101 (2019), p. 020023.

  9. I. V. Shamanin, A. G. Karengin, I. Yu. Novoselov, et al. “Plasmachemical synthesis and evaluation of the thermal conductivity of metal–oxide compounds for prospective nuclear fuel,” PFSD-2018, Tomsk, Russia, April 24–27, 2018, in: J. Phys. Conf. Ser., 1145 (2019), Art. 012057, pp. 1–7.

  10. I. V. Shamanin, A. G. Karengin, I. Yu. Novoselov, et al., “Plasmachemical synthesis and the assessment of the thermal conductivity of fuel compounds UO2–MgO,” ITMA-2018, Tomsk, Russia, Nov. 19–23, 2018, in: AIP Conf. Proc., 2101 (2019), p. 020017.

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Correspondence to I. V. Shamanin.

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Translated from Atomnaya Énergiya, Vol. 131, No. 3, pp. 134–138, September, 2021.

I. V. Shamanin is deceased

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Shamanin, I.V., Karengin, A.G., Karengin, A.A. et al. Investigation of Plasma-Chemical Synthesis of Complex Oxide Compositions for Dispersed Uranium-Plutonium Mixed Fuel. At Energy 131, 135–139 (2022). https://doi.org/10.1007/s10512-022-00854-8

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  • DOI: https://doi.org/10.1007/s10512-022-00854-8

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