A mathematical model of the diffusion of radionuclides through engineered safety barriers is developed for 14C in order to determine the long-term safety conditions and characteristics of a decommissioned commercial uranium-graphite reactor. Dry and wet mixtures and concrete are used as the barrier materials. Diffusion is studied as the dominant mechanism for the transport of the radionuclides. The 14C concentration at the boundary between the radwaste storage site and the environment is determined computationally and the effect of the modeling conditions on the specific activity of the radionuclide is analyzed. The decomposition sequence of the safety barriers for which the 14C concentration is much lower than the admissible value is determined.
Similar content being viewed by others
References
P. M. Gavrilov, A. A. Ustinov, M. V. Antonenko, et al., “Validation of the decommissioning of commercial uranium graphite reactor (PUGR) at the unitary enterprise GKHK according to the on-site disposal variant,” Abstr. AtomEko-2011, Moscow, pp. 49–55.
P. V. Amosov, A. V. Naumov, and N. V. Novozhilova, “Investigation of the diffusion transfer of long-lived radionuclides in the engineered barriers of objects of long-term storage of spent nuclear fuel and disposal of radwastes,” Vest. MGTU, 10, No. 4, 123–129 (2007).
RB-011–2000, Safety Evaluation of Surface Repositories for Radwastes, Gosatomnadzor, Moscow (2001).
A. D. Sakharov, “Radioactive carbon from nuclear explosions and zero-threshold biological effects,” At. Énerg., 4, No. 6, 576–580 (1958).
A. A. Germanskaia, “Natural background radioactive carbon and the natural death rate of people,” Rejuven. Res., 9, No. 2, 302–308 (2006).
NP-055–04, Disposal of Radwastes: Principles, Criteria, and Basic Safety Requirements, Rostekhnadzor, Moscow (2005).
A. A. Abramzon, Surface-Active Substances: Properties and Applications, Moscow (1981).
NRB 99/2009, Radiation Safety Norms, Russ. Sci. Commiss. Radiol. Prot. RAMN, Moscow (2009).
Author information
Authors and Affiliations
Additional information
Translated from Atomnaya Énergiya, Vol. 118, No. 5, pp. 278–281, May, 2015.
Rights and permissions
About this article
Cite this article
Antonenko, M.V., Chubreev, D.O. & Kuznetsov, G.V. Modeling of 14C Diffusion from the Core of the Decommissioned ad Reactor. At Energy 118, 346–350 (2015). https://doi.org/10.1007/s10512-015-0005-7
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10512-015-0005-7