Abstract
Data from a field experiment performed over a period of 16 years at the testing site of the Moscow Scientific and Industrial Association Radon, studying intermediate-level activity K-26 glass with surface storage, are analyzed. The average 137Cs leach rate was 2.2·10−7 g/(cm2·day) over 16 years of testing. The effective mutual diffusion coefficient of cesium was found to be 5·10−21 m2/sec and the rate of hydrolysis of the glass framework was found to be 0.1 µm/yr. The calculation showed that the maximum possible amount of leached radionuclides from glass does not exceed 20 kBq over 300 yr.
Similar content being viewed by others
REFERENCES
P. McGrail, D. Bacon, P. Meyer, et al., “New developments in field studies of low activity waste glass corrosion and contaminant transport,” in: Res. Soc. Symp. Proc., 2003, Vol. 757, pp. 211–213.
J. Sheng, K. Choi, and M.-J. Song, “Vitrification of liquid wastes from nuclear power plants,” J. Nucl. Mater., 297, 7–13 (2001).
F. Lifanov, I. Sobolev, S. Dmitriev, et al., “Vitrification of low and intermediate level waste: technology and glass performance,” in: Proc. WM’04 Conference, Tucson, Arizona (2004), p. 10.
I. A. Sobolev, O. G. Batyukhnova, T. D. Shcherbatova, et al., “Corrosion of vitrified intermediate level wastes under open storage conditions,” At. Energ., 81, No.5, 353–364 (1996).
D. Bacon, M. Ojovan, P. McGrail, et al., “Vitrified waste corrosion rates from field experiment and reactive transport modeling,” in: Proc. ICEM’03, Oxford, England (2003), p. 7.
I. A. Sobolev, F. A. Lifanov, S. V. Stefanovskii, et al., “Reprocessing of radioactive wastes from nuclear power plants on a pilot system with an electric bath furnace,” At. Energ., 69, No.4, 233–236 (1990).
M. Ojovan, N. Ojovan, I. Startseva, et al., “Waste glass behavior in a loamy soil of a wet repository site,” J. Nucl. Mater., 298, 174–179 (2001).
A. A. Belyustin and M. M. Shul’ts, “Interdiffusion of cations and accompanying processes in surface layers of alkaline-silicate glasses treated with water solutions,” Fiz. Khim. Stekla, 9, 3–26 (1983).
T. Richter, G. Frischat, G. Borshart, and S. Scherer, “Short time leaching of a soda-lime glass in H2O and D2O,” Phys. Chem. Glasses, 26, 208–212 (1985).
L. I. Anisimova, V. V. Kulichenko, N. V. Krylova, et al., “Estimate of the degree of contamination of water during storage of vitrified radioactive wastes in geological formations,” At. Energ., 60, No.6, 413–414 (1980).
M. Aertensen, K. Lemmens, and P. van Iseghem, “Fitting elemental profiles for predicting glass dissolution rates in synthetic interstitial clay water,” in: Res. Soc. Symp. Proc., 2003, Vol. 757, pp. 581–588.
K. Knauss, W. Bourcier, K. McKeegan, et al., “Dissolution of a simple analogue nuclear waste glass as a function of pH, time and temperature,” in: Res. Soc. Symp. Proc., 1997, Vol. 176, pp. 371–381.
Author information
Authors and Affiliations
Additional information
__________
Translated from Atomnaya Energiya, Vol. 98, No. 3, pp. 206–211, March, 2005.
Rights and permissions
About this article
Cite this article
Dmitriev, S.A., Barinov, A.S., Ozhovan, N.V. et al. Results of 16 Years of Testing of Vitrified Intermediate-Level Wastes from the Kursk Nuclear Power Plant. At Energy 98, 196–201 (2005). https://doi.org/10.1007/s10512-005-0193-7
Received:
Issue Date:
DOI: https://doi.org/10.1007/s10512-005-0193-7