Skip to main content
Log in

Gas–liquid flow stability and bubble formation in non-Newtonian fluids in microfluidic flow-focusing devices

  • Short Communication
  • Published:
Microfluidics and Nanofluidics Aims and scope Submit manuscript

Abstract

This communication describes the gas–liquid two-phase flow patterns and the formation of bubbles in non-Newtonian fluids in microfluidic flow-focusing devices. Experiments were conducted in two different polymethyl methacrylate (PMMA) square microchannels of, respectively, 600 × 600 and 400 × 400 μm. N2 bubbles were generated in non-Newtonian polyacrylamide (PAAm) solutions of different concentrations. Slug bubble, missile bubble, annular and intermittent flow patterns were observed at the cross-junction by varying gas and liquid flow rates. Gas and liquid flow rates, concentration of PAAm solutions, and channel size were varied to investigate their effect on the mechanism of bubble formation. The bubble size was proportional to the ratio of gas/liquid flow rate for slug bubbles and could be scaled with the ratio of gas/liquid flow rate as a power–law relationship for missile bubbles under wide experimental conditions.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6

References

  • Anna SL, Bontoux N, Stone HA (2003) Formation of dispersions using “flow focusing” in microchannels. Applied Physics Letters 82:364–366

    Article  Google Scholar 

  • Arratia PE, Gollub JP, Durian DJ (2008) Polymeric filament thinning and breakup in microchannels. Physical Review E 77:036309

    Article  Google Scholar 

  • Burton JC, Waldrep R, Taborek P (2005) Scaling and instability in bubble pinch-off. Phys Rev Lett 94:184502

    Article  Google Scholar 

  • Chhabra RP (2007) Bubbles, drops, and particles in non-Newtonian fluids. CRC Press, Boca Raton

    Google Scholar 

  • Chhabra RP, Richardson JF (1984) Prediction of flow pattern for the co-current flow of gas and non-newtonian liquid in horizontal pipes. The Canadian Journal of Chemical Engineering 62:449–454

    Article  Google Scholar 

  • Cubaud T, Tatineni M, Zhong X, Ho CM (2005) Bubble dispenser in microfluidic devices. Physical Review E. 72: 037302

    Google Scholar 

  • de Menech M, Garstecki P, Jousse F, Stone HA (2008) Transition from squeezing to dripping in a microfluidic T-shaped junction. J Fluid Mech 595:141–161

    MATH  Google Scholar 

  • Dollet B, van Hoeve W, Raven J-P, Marmottant P, Versluis M (2008) Role of the channel geometry on the bubble pinch off in flow focusing devices. Phys Rev Lett 100:034504

    Article  Google Scholar 

  • Frank X, Li HZ (2005) Complex flow around a bubble rising in a non-Newtonian fluid. Physical Review E 71:036309

    Article  Google Scholar 

  • Frank X, Li HZ (2006) Negative wake behind a sphere rising in viscoelastic fluids: A lattice Boltzmann investigation. Physical Review E 74:056307

    Article  Google Scholar 

  • Fu T, Funfschilling D, Ma Y, Li HZ (2010) Scaling the formation of slug bubbles in microfluidic flow-focusing devices. Microfluid Nanofluid 8:467–475

    Article  Google Scholar 

  • Gañán-Calvo AM, Gordillo JM (2001) Perfectly monodisperse microbubbling by capillary flow focusing. Phys Rev Lett 87:274501

    Article  Google Scholar 

  • Garstecki P, Gitlin I, DiLuzio W, Whitesides G, Kumacheva EM, Stone HA (2004) Formation of monodisperse bubbles in a microfluidic flow-focusing device. Applied Physics Letters 85:2649–2651

    Article  Google Scholar 

  • Garstecki P, Stone HA, Whitesides GM (2005) Mechanism for flow-rate controlled breakup in confined geometries: A route to monodisperse emulsions. Phys Rev Lett 94:164501

    Article  Google Scholar 

  • Groisman A, Enzelberger M, Quake SR (2003) Microfluidic memory and control devices. Science 300:955–958

    Article  Google Scholar 

  • Husny J, Cooper-White JJ (2006) The effect of elasticity on drop creation in T-shaped microchannels. J Non-Newton Fluid Mech 137:121–136

    Article  Google Scholar 

  • Li HZ (1999) Bubbles in non-Newtonian fluids: Formation, interactions and coalescence. Chem Eng Sci 54:2247–2254

    Article  Google Scholar 

  • Pillapakkam SB, Singh P, Blackmore D, Aubry N (2007) Transient and steady state of a rising bubble in a viscoelastic fluid. J Fluid Mech 589:215–252

    Article  MATH  MathSciNet  Google Scholar 

  • Qiu D, Silva L, Tonkovich AL, Arora R (2010) Micro-droplet formation in non-Newtonian fluid in a microchannel. Microfluid Nanofluid 8:531–548

    Article  Google Scholar 

  • Sang L, Hong Y, Wang F (2009) Investigation of viscosity effect on droplet formation in T-shaped microchannels by numerical and analytical methods. Microfluid Nanofluid 6:621–635

    Article  Google Scholar 

  • Skurtys O, Bouchon P, Aguilera JM (2008) Formation of bubbles and foams in gelatine solutions within a vertical glass tube. Food hydrocolloids 22:706–714

    Article  Google Scholar 

  • Sullivan MT, Stone HA (2008) The role of feedback in microfluidic flow-focusing devices. Philosophical Transactions of The Royal Society A 366:2131–2143

    Article  Google Scholar 

  • Utada AS, Lorenceau E, Link DR, Kaplan PD, Stone HA, Weitz DA (2005) Monodisperse double emulsions generated from a microcapillary device. Science 308:537–541

    Article  Google Scholar 

  • Whitesides GM (2006) The origins and the future of microfluidics. Nature 442:368–373

    Article  Google Scholar 

  • Zhang J (2010) Lattice Boltzmann method for microfluidics: models and applications. Microfluid Nanofluid. doi:10.1007/s10404-010-0624-1

Download references

Acknowledgments

We gratefully acknowledge the financial support for this project from the National Natural Science Foundation of China (No. 20876107), the aid of Opening Project of State Key Laboratory of Chemical Engineering (Grant No. SKL-ChE-08B06) and the Program of Introducing Talents of Discipline to Universities (Grant No. B06006). Taotao Fu appreciates the financial aid from both the China Scholarship Council and the French Embassy in China.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Huai Z. Li.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Fu, T., Ma, Y., Funfschilling, D. et al. Gas–liquid flow stability and bubble formation in non-Newtonian fluids in microfluidic flow-focusing devices. Microfluid Nanofluid 10, 1135–1140 (2011). https://doi.org/10.1007/s10404-010-0741-x

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10404-010-0741-x

Keywords

Navigation