Abstract
Field measurement campaigns were conducted at a Chinese municipal solid waste landfill to investigate variation of non-methane organic compounds (NMOCs) when migrating through an intermediate soil cover. Flux change ratio (FCR) was introduced to indicate quantitative variation of NMOCs between two depths through the soil cover. FCR of NMOCs showed a positive correlation with methane oxidation fraction (99 % confidence level), indicating the synergistic effects of methane oxidation and NMOCs mitigation in soil cover. Emission reduction indicator (ERI), ozone-forming potential reduction indicator (ORI), and toxicity reduction indicator (TRI) of halogenated hydrocarbons were calculated to evaluate the environmental effects of intermediate soil cover for NMOCs control and reached up to 7.85 mg m−2 day−1, 20.8 mg m−2day−1 and 7.27 µg m−2 day−1, respectively. Enhancement of methane oxidation in landfill covers could be an effective way to reduce NMOCs emission and decrease its environmental effects, which would give guidance on landfill management.
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References
Scheutz C, Kjeldsen P (2003) Capacity for biodegradation of CFCs and HCFCs in a methane oxidative counter-gradient laboratory system simulating landfill soil covers. Environ Sci Technol 37:5143–5149. doi:10.1021/es026464+
Allen MR, Braithwaite A, Hills CC (1997) Trace organic compounds in landfill gas at seven UK waste disposal sites. Environ Sci Technol 31:1054–1061. doi:10.1021/es9605634
Dincer F, Odabasi AM, Muezzinoglu A (2006) Chemical characterization of odorous gases at a landfill site by gas chromatography-mass spectrometry. J Chromatogr A 1122:222–229. doi:10.1016/j.chroma.2006.04.075
Hodson EL, Martin D, Prinn RG (2010) The municipal solid waste landfill as a source of ozone-depleting substances in the United States and United Kingdom. Atmos Chem Phys 10:1899–1910. doi:10.5194/acp-10-1899-2010
Wagner P, Kuttler W (2013) Biogenic and anthropogenic isoprene in the near-surface urban atmosphere—a case study in Essen, Germany. Sci Total Environ 475:104–115. doi:10.1016/j.scitotenv.2013.12.026
Liu WT, Chen SP, Chang CC, Ouyang CF, Liao WC, Su YC, Wu YC, Wang CH, Wang JL (2014) Assessment of carbon monoxide (CO) adjusted non-methane hydrocarbon (NMHC) emissions of a motor fleet—a long tunnel study. Atmos Environ 89:403–414. doi:10.1016/j.atmosenv.2014.01.002
Sadasivam BY, Reddy KR (2014) Landfill methane oxidation in soil and bio-based cover systems: a review. Rev Environ Sci Bio 13:79–107. doi:10.1007/s11157-013-9325-z
Mor S, Visscher AD, Ravindra K, Dahiya RP, Chandra A, Van Cleemput O (2006) Induction of enhanced methane oxidation in compost: temperature and moisture response. Waste Manage 26:381–388. doi:10.1016/j.wasman.2005.11.005
Scheutz C, Kjeldsen P (2005) Biodegradation of trace gases in simulated landfill soil cover systems. J Air Waste Manage 55:878–885. doi:10.1080/10473289.2005.10464693
Schuetz C, Bogner J, Chanton J, Blake D, Morcet M, Kjeldsen P (2003) Comparative oxidation and net emissions of methane and selected mon-methane organic compounds in landfill cover soils. Environ Sci Technol 37:5150–5158. doi:10.1021/es034016b
Scheutz C, Bogner J, Chanton JP, Blake D, Morcet M, Aran C, Kjeldsen P (2008) Atmospheric emissions and attenuation of non-methane organic compounds in cover soils at a French landfill. Waste Manage 28:1892–1908. doi:10.1016/j.wasman.2007.09.010
Kjeldsen P, Dalager A, Broholm K (1997) Attenuation of methane and nonmethane organic compounds in landfill gas affected soils. J Air Waste Manage 47:1268–1278. doi:10.1080/10473289.1997.10464072
Duan ZH, Lu WJ, Li D, Wang HT (2014) Temporal variation of trace compound emission on the working surface of a landfill in Beijing. Atmos Environ 88:230–238. doi:10.1016/j.atmosenv.2014.01.051
Yue DB, Han B, Sun Y, Yang T (2014) Sulfide emissions from different areas of a municipal solid waste landfill in China. Waste Manag 34:1041–1044. doi:10.1016/j.wasman.2013.07.020
Abichou T, Powelson D, Chanton J, Escoriaza S, Stern J (2006) Characterization of methane flux and oxidation at a solid waste landfill. J Environ Eng 132:220–228. doi:10.1061/(ASCE)0733-9372(2006)132:2(220)
Stern JC, Chanton J, Abichou T, Powelson D, Yuan L, Escoriza S, Bogner J (2007) Use of a biologically active cover to reduce landfill methane emissions and enhance methane oxidation. Waste Manage 27:1248–1258. doi:10.1016/j.wasman.2006.07.018
Yang T, Yue DB, Han B, Sun Y (2014) Field methane oxidation efficiency at municipal solid waste landfills located in the north of China. Adv Mater Res 878:812–820. doi:10.4028/www.scientific.net/AMR.878.812
US Environmental Protection Agency (2012) Quantifying methane abatement efficiency at three municipal solid waste landfills. EPA/600/R-12/033. ARCADIS US, Inc, Durham
Saquing JM, Chanton JP, Yazdani R, Barlaz MA, Scheutz C, Blake DR, Imhoff PT (2014) Assessing methods to estimate emissions of non-methane organic compounds from landfills. Waste Manage 34:2260–2270. doi:10.1016/j.wasman.2014.07.007
Kucera CL, Kirkham DR (1971) Soil respiration studies in tallgrass prairie in Missouri. Ecology 52:912–915. doi:10.2307/1936043
Gebert J, Rower IU, Scharff H, Roncato CDL, Cabral AR (2011) Can soil gas profiles be used to assess microbial CH4 oxidation in landfill covers? Waste Manag 31:987–994. doi:10.1016/j.wasman.2010.10.008
Carter WPL, Heo G (2012) Development of revised SPARC aromatics mechanisms. Final report to california air resources board contracts No. 07-730 and 08-326
Thomas CL, Barlaz MA (1999) Production of non-methane organic compounds during refuse decomposition in a laboratory-scale landfill. Waste Manage Res 17:205–211. doi:10.1034/j.1399-3070.1999.00030.x
Chanton J, Abichou T, Ford C, Harter G, Green R, Goldsmith D, Swan N (2011) Landfill methane oxidation across climate types in the U.S. Environ Sci Technol 45:313–319. doi:10.1021/es101915r
Spokas KA, Bogner JE (2011) Limits and dynamics of methane oxidation in landfill cover soils. Waste Manag 31:823–832. doi:10.1016/j.wasman.2009.12.018
Barlaz MA, Green RB, Chanton JP, Goldsmith CD, Hater GR (2004) Evaluation of a biologically active cover for mitigation of landfill gas emissions. Environ Sci Technol 38:4891–4899. doi:10.1021/es049605b
Majumdar D, Ray S, Chakraborty S, Rao PS, Akolkar AB, Chowdhury M (2014) Emission, speciation, and evaluation of impacts of non-methane volatile organic compounds from open dump site. J Air Waste Manage 64:834–845. doi:10.1080/10962247.2013.873747
Scheutz C, Kjeldsen P, Bogner JE, Visscher AD, Gebert J, Hilger HA, Huber-Humer M, Spokas K (2009) Microbial methane oxidation processes and technologies for mitigation of landfill gas emissions. Waste Manage Res 27:409–455. doi:10.1177/0734242X09339325
Yao YJ, Su Y, Wu Y, Liu WP, He R (2015) An analytical model for estimating the reduction of methane emission through landfill cover soils by methane oxidation. J Hazard Mater 283:871–879. doi:10.1016/j.jhazmat.2014.10.035
Hrad M, Huber-Humer M, Reichenauer BW (2012) Design of top covers supporting aerobic in situ stabilization of old landfills-an experimental simulation in lysimeters. Inst Waste Manag 32:2324–2335. doi:10.1016/j.wasman.2012.06.004
Scheutz C, Pedersen RB, Petersen PH, Jorgensen JHB, Ucendo IMB, Monster JG (2014) Mitigation of methane emission from an old unlined landfill in Klintholm, Denmark using a passive biocover system. Waste Manag 34:1179–1190. doi:10.1016/j.wasman.2014.03.015
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This project is supported by Special Fund of Environmental Protection Research for Public Welfare of China (No. 201509055) and Tsinghua University Initiative Scientific Research Program (No. 2012Z02128).
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Wang, X., Yue, D., Zhao, K. et al. Mitigation of non-methane organic compounds through landfill soil cover and its environmental implications. J Mater Cycles Waste Manag 17, 616–625 (2015). https://doi.org/10.1007/s10163-015-0403-x
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DOI: https://doi.org/10.1007/s10163-015-0403-x