Skip to main content
Log in

Pretreatment of nonbiodegradable landfill leachate by air stripping coupled with agitation as ammonia stripping and coagulation–flocculation processes

  • Original Paper
  • Published:
Clean Technologies and Environmental Policy Aims and scope Submit manuscript

Abstract

A combination process has developed as a pretreatment of non biodegradable leachate. The processes consist of air stripping coupled with agitation as a modified of ammonia stripping followed by coagulation–flocculation processes. The main aims of these processes are reducing a concentration of NH3-N and organic matter as well as enhancing the biodegradability of landfill leachate. Ammonia stripped by the airflow rate of 10 L min−1 at pH 11 for 3 h, while the agitation process applied to air stripping effluent for 2 h at the pH of 11.5 in 150 s−1 gradient velocity. NH3-N was removed at 96 % as removal ratio by the modified ammonia stripping in 5 h stripping time. Ferric sulfate, poly ferric sulfate and aluminum poly chloride was tested as a coagulant material in the coagulation process. Chemical oxygen demand (COD), suspended solids (SS), turbidity as well as the sludge ratios were discovered for each material operated under optimum condition of pH and dosage. The overall removal of NH3-N, COD, biochemical oxygen demand, total organic carbon, and SS obtained by these processes were 96.5, 71.5, 56.5, 48.5, and 96.5 %, respectively, at the corresponding biodegradable ratio was modified from 0.20 to 0.31.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4

Similar content being viewed by others

References

  • Aguilar MI, Liorens M, Soler A, Ortuno JF (2002) Nutrient removal and sludge production in the coagulation–flocculation process. Water Res 36:2910–2919

    Article  CAS  Google Scholar 

  • Amokrane A, Comel C, Veron J (1997) Landfill leachates pretreatment by coagulation–flocculation. Water Res 31:2775–2782

    Article  CAS  Google Scholar 

  • APHA (2005) Standard methods for the examination of water and wastewater, 21st edn. American Public Health Association, Washington, DC

  • Atmaca E (2009) Treatment of landfill leachate by using electro-Fenton method. J Hazard Mater 163:109–114

    Article  CAS  Google Scholar 

  • Bonmati A, Flotats X (2003) Air stripping of ammonia from pig slurry: characterisation and feasibility as a pre-or post-treatment to mesophilic anaerobic digestion. Waste Manage 23:261–272

    Article  CAS  Google Scholar 

  • Calace N, Liberatori A, Petronio BM, Pietroletti M (2001) Characteristics of different molecular weight fractions of organic matter in landfill leachate and their role in soil sorption of heavy metals. Environ Pollut 113:331–339

    Article  CAS  Google Scholar 

  • Cheng RC, Liang S, Wang HC, Beuhler MD (1994) Enhanced coagulation for arsenic removal. J Am Water Works Assoc 86:79–90

    CAS  Google Scholar 

  • Cheung KC, Chu LM, Wong MH (1997) Ammonia stripping as a pretreatment for landfill leachate. Water Air Soil Pollut 94:209–221

    CAS  Google Scholar 

  • Collivignarelli C, Bertanza G, Baldi M, Avezzu F (1998) Ammonia stripping from MSW landfill leachate in bubble reactors: process modeling and optimization. Waste Manage Res 16:455–466

    Article  CAS  Google Scholar 

  • Cortez S, Teixeira P, Oliveira R, Mota M (2011) Evaluation of Fenton and ozone-based advanced oxidation processes as mature landfill leachate pre-treatments. J Environ Manage 92:749–755

    Article  CAS  Google Scholar 

  • Guo JS, Abbas AA, Chen YP, Liu ZP, Fang F, Chen P (2010) Treatment of landfill leachate using a combined stripping, Fenton, SBR, and coagulation process. J Hazard Mater 178:699–705

    Article  CAS  Google Scholar 

  • Hasar H, Unsal SA, Ipek U, Karatas S, Cinar O, Yaman C, Kinace C (2009) Stripping/flocculation/membrane bioreactor/reverse osmosis treatment of municipal landfill leachate. J Hazard Mater 171:309–317

    Article  CAS  Google Scholar 

  • Hermosilla D, Cortijo M, Huang CP (2009) Optimizing the treatment of landfill leachate by conventional Fenton and photo-Fenton processes. Sci Total Environ 407:3473–3481

    Article  CAS  Google Scholar 

  • Kang KH, Shin HS, Park H (2002) Characterization of humic substances present in landfill leachates with different landfill ages and its implications. Water Res 36:4023–4032

    Article  CAS  Google Scholar 

  • Kilic MY, Kestioglu K, Yonar T (2007) Landfill leachate treatment by the combination of physicochemical methods with adsorption process. J Biol Environ Sci 1:37–43

    Google Scholar 

  • Li W, Hua T, Zhou Q, Zhang S, Li F (2010) Treatment of stabilized landfill leachate by the combined process of coagulation/flocculation and powder activated carbon adsorption. Desalination 264:56–62

    Article  CAS  Google Scholar 

  • Maranon E, Castrillon L, Fernandez-Nava Y, Fernandez-Mendez A, Fernandez-Sanchez A (2008) Coagulation–flocculation as a pretreatment process at a landfill leachate nitrification-denitrification plant. J Hazard Mater 156:538–544

    Article  CAS  Google Scholar 

  • Marttinen SK, Kettunen RH, Sormunen KM, Soimasuo RM, Rintala JA (2002) Screening of physical–chemical methods for removal of organic material, nitrogen and toxicity from low strength landfill leachates. Chemosphere 46:851–858

    Article  CAS  Google Scholar 

  • Neczaj E, Okoniewska E, Kacprzak M (2005) Treatment of landfill leachate by sequencing batch reactor. Desalination 185:357–362

    Article  CAS  Google Scholar 

  • Ntampou X, Zouboulis AI, Samaras P (2006) Appropriate combination of physico-chemical methods (coagulation/flocculation and ozonation) for the efficient treatment of landfill leachates. Chemosphere 62:722–730

    Article  CAS  Google Scholar 

  • Ozturk I, Altinbas M, Koyuncu I, Arikan O, Gomec-Yangin C (2003) Advanced physico-chemical treatment experiences on young municipal landfill leachates. Waste Manage 23:441–446

    Article  CAS  Google Scholar 

  • Pi KW, Li Z, Wan DJ, Gao LX (2009) Pretreatment of municipal landfill leachate by a combined process. Process Saf Environ Prot 87:191–196

    Article  CAS  Google Scholar 

  • Silva AC, Dezotti M, SantaAnna GL (2004) Treatment and detoxification of a sanitary landfill leachate. Chemosphere 55:207–214

    Article  CAS  Google Scholar 

  • Stephenson RJ, Duff SJB (1996) Coagulation and precipitation of a mechanical pulping effluent: I. Removal of carbon, colour and turbidity. Water Res 30:781–792

    Article  CAS  Google Scholar 

  • Tatsi AA, Zouboulis AI, Matis KA, Samaras P (2003) Coagulation–flocculation pretreatment of sanitary landfill leachates. Chemosphere 53:737–744

    Article  CAS  Google Scholar 

  • Uygur A, Kargi F (2004) Biological nutrient removal from pre-treated landfill leachate in a sequencing batch reactor. J Environ Manage 71:9–14

    Article  Google Scholar 

  • Wang F, Smith DW, El-Din MG (2003) Application of advanced oxidation methods for landfill leachate treatment: a review. J Environ Eng Sci 2:413–427

    Article  CAS  Google Scholar 

  • Wang Q, Matsufuji Y, Dong L, Huang Q, Hirano F, Tanaka A (2006) Research on leachate recirculation from different types of landfills. Waste Manage 26:815–824

    Article  Google Scholar 

  • Wang X, Chen S, Gu X, Wang K (2009) Pilot study on the advanced treatment of landfill leachate using a combined coagulation, fenton oxidation and biological aerated filter process. Waste Manage 29:1354–1358

    Article  CAS  Google Scholar 

  • Wichitsathian B, Sindhuja S, Visvanathan C, Ahn KH (2005) Landfill leachate treatment by yeast and bacteria based membrane bioreactors. J Environ Sci Heal A 39:2391–2404

    Article  Google Scholar 

  • Wu JJ, Wu CC, Ma HW, Chang CC (2004) Treatment of landfill leachate by ozone-based advanced oxidation processes. Chemosphere 54:997–1003

    Article  CAS  Google Scholar 

  • Yilmaz T, Apaydin S, Berktay A (2010) Coagulation–flocculation and air stripping as a pretreatment of young landfill leachate. Open Environ Eng J 3:42–48

    Article  CAS  Google Scholar 

  • Zgajnar Gotvajn A, Zagorc-Koncan J, Cotman M (2011) Fenton’s oxidative treatment of municipal landfill leachate as an alternative to biological process. Desalination 275:269–275

    Article  CAS  Google Scholar 

  • Zhang H, Choi HJ, Huang CP (2006a) Treatment of landfill leachate by Fenton’s reagent in a continuous stirred tank reactor. J Hazard Mater 136:618–623

    Article  CAS  Google Scholar 

  • Zhang H, Zhang D, Zhou J (2006b) Removal of COD from landfill leachate by electro-Fenton method. J Hazard Mater 135:106–111

    Article  CAS  Google Scholar 

  • Zhang T, Ding L, Ren H (2009) Pretreatment of ammonium removal from landfill leachate by chemical precipitation. J Hazard Mater 166:911–915

    Article  CAS  Google Scholar 

Download references

Acknowledgments

This study was financially supported by the Hubei Provincial Science and Technology Department with grant No. 2006AA305A05. Mr Alkhafaji R. Abood thanks the Ministry of Higher Education and Thi-Qar University in Iraq for enabling him to purse a higher degree. He is also grateful to the China Scholarship Council (CSC) and China University of Geosciences (CUG) for the financial support of this research.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Jianguo Bao.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Abood, A.R., Bao, J., Abudi, Z.N. et al. Pretreatment of nonbiodegradable landfill leachate by air stripping coupled with agitation as ammonia stripping and coagulation–flocculation processes. Clean Techn Environ Policy 15, 1069–1076 (2013). https://doi.org/10.1007/s10098-012-0575-1

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10098-012-0575-1

Keywords

Navigation