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The influence of electrolyte on photocatalytic activity of PEO coatings with incorporated Ce-ZSM5 formed on aluminum

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Abstract

The preparation and characterization of oxide coatings made by plasma electrolytic oxidation (PEO) process on aluminum in two different electrolyte solutions of opposite pH values with addition of Ce-enriched ZSM-5 zeolite are investigated in this paper. The first selected electrolyte solution is highly acidic pH < 3, prepared with tungstosilicic acid (H4O40SiW12), while the second one is made with sodium tungstate (Na2WO4) creating highly alkaline PEO environment with pH > 12. Phase structure, chemical composition, morphology, photoluminescent properties, and photocatalytic activity of deposited oxide coatings are discussed. Properties of PEO coatings are analyzed against processing time revealing dynamics of PEO under defined conditions. Both sets of oxide coatings have similar chemical composition and morphology, but the photocatalytic activity is considerably higher for oxide coatings made in alkaline environment.

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Funding

This work is supported by the Ministry of Education, Science, and Technological Development of the Republic of Serbia, contract numbers: 451–03-68/2022–14/200162 and 451–03-68/2022–14/200146, and by the European Union Horizon 2020 research and innovation program under the Marie Sklodowska-Curie grant agreement no. 823942 (FUNCOAT).

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Authors and Affiliations

  1. University of Belgrade, Faculty of Physics, Studentski Trg 12-16, 11000, Belgrade, Serbia

    Nikola Božović, Kristina Mojsilović, Stevan Stojadinović & Rastko Vasilić

  2. Directorate of Measures and Precious Metals, Mike Alasa 14, 11000, Belgrade, Serbia

    Nikola Božović

  3. University of Belgrade, Faculty of Physical Chemistry, Studentski Trg 12-16, 11000, Belgrade, Serbia

    Srna Stojanović & Ljiljana Damjanović-Vasilić

Authors
  1. Nikola Božović
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  2. Kristina Mojsilović
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  3. Srna Stojanović
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  4. Ljiljana Damjanović-Vasilić
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  5. Stevan Stojadinović
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  6. Rastko Vasilić
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Contributions

The manuscript was written through contributions of all authors. All authors have given approval to the final version of the manuscript. Nikola Božović: investigation, data curation, and writing; Kristina Mojsilović: investigation, data curation, visualization, and writing—reviewing and editing; Srna Stojanović: investigation; Ljiljana Damjanović-Vasilić: conceptualization and writing; Stevan Stojadinović: methodology; Rastko Vasilić: conceptualization, supervision, and writing—reviewing and editing.

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Correspondence to Rastko Vasilić.

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Božović, N., Mojsilović, K., Stojanović, S. et al. The influence of electrolyte on photocatalytic activity of PEO coatings with incorporated Ce-ZSM5 formed on aluminum. J Solid State Electrochem 27, 1945–1953 (2023). https://doi.org/10.1007/s10008-023-05455-4

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  • DOI: https://doi.org/10.1007/s10008-023-05455-4

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