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On the Reaction between 1-Aza-1,3-dienes and Push-Pull Olefins of the Acyloxymethylidene-malononitrile Type

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Summary.

 The reaction between push-pull olefins of the acyloxymethylidene-malononitrile type and α, β-unsaturated hydrazones affords selectively 5-alkyl-2-cyano-6-(N′,N′-dimethylhydrazono)-hexa-2,4-dienenitriles. No [4+2]-cycloaddition products were detected. The structure elucidation of the obtained compounds and possible reaction mechanisms are discussed.

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Authors and Affiliations

  1.  Department of Organic Chemistry, Faculty of Pharmacy, Medical University of Gdansk, PL-80416 Gdansk, Poland, , , , , , PL

    Czeslawa Orlewska

  2.  Chemistry Department, Faculty of Science, Minia University, El-Minia, Egypt, , , , , , EG

    Rafat M. Shaker

  3.  Institute of Pharmacy, Pharmaceutical/Medicinal Chemistry, University of Greifswald, D-17487 Greifswald, Germany, , , , , , DE

    Martin Dees & Hans-Hartwig Otto

Authors
  1. Czeslawa Orlewska
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  2. Rafat M. Shaker
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  3. Martin Dees
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  4. Hans-Hartwig Otto
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Additional information

Received March 9, 2000. Accepted March 20, 2000

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Orlewska, C., Shaker, R., Dees, M. et al. On the Reaction between 1-Aza-1,3-dienes and Push-Pull Olefins of the Acyloxymethylidene-malononitrile Type. Monatshefte fuer Chemie 131, 889–893 (2000). https://doi.org/10.1007/s007060070066

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  • DOI: https://doi.org/10.1007/s007060070066

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