Skip to main content
Log in

Variation of indoor radon concentration and ambient dose equivalent rate in different outdoor and indoor environments

  • Original Article
  • Published:
Radiation and Environmental Biophysics Aims and scope Submit manuscript

Abstract

Subject of this study is an investigation of the variations of indoor radon concentration and ambient dose equivalent rate in outdoor and indoor environments of 40 dwellings, 31 elementary schools and five kindergartens. The buildings are located in three municipalities of two, geologically different, areas of the Republic of Macedonia. Indoor radon concentrations were measured by nuclear track detectors, deployed in the most occupied room of the building, between June 2013 and May 2014. During the deploying campaign, indoor and outdoor ambient dose equivalent rates were measured simultaneously at the same location. It appeared that the measured values varied from 22 to 990 Bq/m3 for indoor radon concentrations, from 50 to 195 nSv/h for outdoor ambient dose equivalent rates, and from 38 to 184 nSv/h for indoor ambient dose equivalent rates. The geometric mean value of indoor to outdoor ambient dose equivalent rates was found to be 0.88, i.e. the outdoor ambient dose equivalent rates were on average higher than the indoor ambient dose equivalent rates. All measured can reasonably well be described by log-normal distributions. A detailed statistical analysis of factors which influence the measured quantities is reported.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7

Similar content being viewed by others

References

  • Almgren S, Isaksson M, Barregard L (2008) Gamma radiation doses to people living in Western Sweden. J Environ Radioact 99:394–403

    Article  Google Scholar 

  • Antovic N, Vukotic P, Zekic R, Svrkota R, Ilic R (2007) Indoor radon concentrations in urban settlements on the Montenegrin Coast. Radiat Meas 42:1573–1579

    Article  Google Scholar 

  • Bochicchio F, Zunic SZ, Carpentieri C, Antignani S, Venoso G, Carelli V, Cordedda C, Veselinovic N, Tollefsen T, Bossew P (2014) Radon in indoor air of primary schools: a systematic survey to evaluate factors affecting radon concentration levels and their variability. Indoor Air 24:315–326

    Article  Google Scholar 

  • Bossew P, Stojanovska Z, Zunic ZS, Ristova M (2013) Prediction of indoor radon risk from radium concentration in soil: Republic of Macedonia case study. Rom J Phys 58S:S29–S43

    Google Scholar 

  • Bossew P, Zunic ZS, Stojanovska Z, Tollefsen T, Carpentieri C, Veselinovic N, Komatina S, Vaupotic J, Simovic R, Antignani S, Bochicchio F (2014) Geographical distribution of the annual mean radon concentrations in primary schools of Southern Serbia and application of geostatistical methods. J Environ Radioact 127:141–148

    Article  Google Scholar 

  • Carpentieri C, Zunic SZ, Carelli V, Cordedda C, Ferrigno G, Veselinovic N, Bossew P, Tollefsen T, Cuknic O, Vojinovic Z, Bochicchio F (2011) Assessment of long-term radon concentration measurement precision in field conditions (Serbian schools) for a survey carried out by an international collaboration. Radiat Prot Dosim 145:305–311

    Article  Google Scholar 

  • Clouvas A, Xanthos S, Antonopoulos-Domis M (2003) A combination study of indoor radon and in situ gamma spectrometry measurements in Greek dwellings. Radiat Prot Dosim 103:363–366

    Article  Google Scholar 

  • Clouvas A, Takoudis G, Xanthos S, Potiriadis C, Kolovou M (2009) Indoor radon measurements in areas of northern Greece with relatively high indoor radon concentrations. Radiat Prot Dosim 136:127–131

    Article  Google Scholar 

  • Curguz Z, Zunic ZS, Tollefsen T, Jovanovic P, Nikezic D, Kolarz P (2013) Active and passive radon concentration measurements and first-step mapping in schools of Banja Luka, Republic of Srpska. Rom J Phys 58S:S90–S98

    Google Scholar 

  • Curguz Z, Stojanovska Z, Zunic ZS, Kolarz P, Ischikawa T, Omori Y, Mishra R, Sapra B, Vaupotic J, Ujic P, Bossew P (2015) Long-term measurements of radon, thoron and their airborne progeny in 25 schools in Republic of Srpska. J Environ Radioact 148:163–169

    Article  Google Scholar 

  • Darby S, Hill D, Auvinen A, Barros-Dios JM, Baysson H, Bochicchio F, Deo H, Falk R, Forastiere F, Hakama M, Heid I, Kreienbrock L, Kreuzer M, Lagarde F, Mäkeläinen I, Muirhead C, Oberaigner W, Pershagen G, Ruano-Ravina A, Ruosteenoja E, Rosario AS, Tirmarche M, Tomásek L, Whitley E, Wichmann HE, Doll R (2005) Radon in homes and risk of lung cancer: collaborative analysis of individual data from 13 European case-control studies. BMJ 330:223–226

    Article  Google Scholar 

  • Dumurdzanov N, Serafimovski T, Burchfiel CB (2004) Evolution of the Neogene-Pleistocene basins of Macedonia geological. Society of America digital map and chart series 1. http://www.geosociety.org/maps/2004-dumurdzanov-macedonia/dmc001.pdf

  • Gulan L, Milic G, Bossew P, Omori Y, Ishikawa T, Mishra R, Mayya Y, Stojanovska Z, Nikezic D, Vuckovic B, Zunic ZS (2012) Field experience on indoor radon, thoron and their progenies with solid state detectors in a survey of Kosovo and Metohija. Radiat Prot Dosim 152:189–197

    Article  Google Scholar 

  • Gulan L, Bochicchio F, Carpentieri C, Milic G, Stajic J, Krstic D, Stojanovska Z, Nikezic D, Zunic ZS (2013) High annual radon concentration in dwellings and natural radioactivity content in nearby soil in some rural areas of Kosovo and Metohija. Nucl Technol Radiat 28:60–67

    Article  Google Scholar 

  • Harrison JD, Marsh JW (2012) Effective dose from inhaled radon and its progeny. Ann ICRP 41:378–388

    Article  Google Scholar 

  • Ivanova K, Stojanovska Z, Badulin V, Kunovska B (2013) Pilot survey of indoor radon in the dwellings of Bulgaria. Radiat Prot Dosim 157:594–599

    Article  Google Scholar 

  • Ivanova K, Stojanovska Z, Tsenova M, Badulin V, Kunovska B (2014) Measurement of indoor radon concentration in kindergartens in Sofia, Bulgaria. Radiat Prot Dosim 162:163–166

    Article  Google Scholar 

  • Karajovanovik M, Hadži-Mitrova S (1975) Explanatory note of the General Geological Map of SFRJ, Sheet of Titov Veles (K 34–80), scale 1:100 000. Geological institute Skopje, Federal geological institute, Beograd

    Google Scholar 

  • Karajovanovik M, Hristov S (1976) Explanatory note of the general geological map of SFRJ for the map sheets of Kratovo (K 34–69) and Kystendil (K 34–70), scale 1:100 000. Geological institute Skopje, Federal geological institute, Beograd

    Google Scholar 

  • Kropat G, Bochud F, Jaboyedoff M, Laedermann JP, Murith C, Palacios M, Baechler S (2014) Major influencing factors of indoor radon concentrations in Switzerland. J Environ Radioact 129:7–22

    Article  Google Scholar 

  • Milic G, Jakupi B, Tokonami S, Trajkovic R, Ishikawa T, Celikovic I, Ujic P, Cuknic O, Yarmoshenko I, Kosanovic K, Adrovic F, Sahoo S, Veselinovic N, Zunic ZS (2010) The concentrations and exposure doses of radon and thoron in residences of the rural areas of Kosovo and Metohija. Radiat Meas 45:118–121

    Article  Google Scholar 

  • Milic G, Yarmoshenko I, Jakupi B, Kovacevic M, Zunic ZS (2011) Indoor radon measurements in Kosovo and Metohija over the period 1995–2007. Radiat Meas 46:141–144

    Article  Google Scholar 

  • Műllerová M, Kozak K, Kovács T, Smetanová I, Csordás A, Grzadziel D, Holý K, Mazur J, Moravcsík A, Neznal M, Neznal M (2016) Indoor radon survey in Visegrad countries. Appl Radiat Isot 110:124–128

    Article  Google Scholar 

  • Negi MS, Prasad Y, Prasad G, Gusain GS, Badoni M, Ramola RC (2009) Gamma radiation dose rate in indoor, outdoor and underground atmosphere around Tehridam project, Uttarakhand, India. Indian J Phys 83:1209–1214

    Article  ADS  Google Scholar 

  • Nikolopoulos D, Kottou S, Louizi A, Petraki E, Vogiannis E, Yannakopoulos P (2014) Factors affecting indoor radon concentrations of Greek dwellings through multivariate statistics-first approach. J Phys Chem Biophys 4:145

    Google Scholar 

  • Onischenko A, Zhukovsky M, Veselinovic N, Zunic ZS (2010) Radium-226 concentration in spring water sampled in high radon regions. Appl Radiat Isot 68:825–827

    Article  Google Scholar 

  • Rakikevnik T, Dumurdžanov N, Petkovski P (1976) Explanatory note of the general geological map of SFRJ, sheet of Štip (K 34–81), scale 1:100 000. Geological institute Skopje, Federal geological institute, Beograd

    Google Scholar 

  • Stajic MJ, Milenkovic B, Nikezic D (2015) Radon concentrations in schools and kindergartens in Kragujevac City, Central Serbia. CLEAN Soil Air Water 43:1361–1365

    Article  Google Scholar 

  • Stojanovska Z, Januseski J, Bossew P, Zunic Z, Tollefsen T, Ristova M (2011) Seasonal indoor radon concentration in FYR of Macedonia. Radiat Meas 46:602–610

    Article  Google Scholar 

  • Stojanovska Z, Januseski J, Boev B, Ristova M (2012) Indoor exposure of population to radon in The FYR of Macedonia. Radiat Prot Dosim 148:162–167

    Article  Google Scholar 

  • Stojanovska Z, Zunic ZS, Bossew P, Bochicchio F, Carpentieri C, Venoso G, Mishra R, Rout R, Sapra B, Burghele B, Cucos-Dinu A, Boev B, Cosma C (2014) Results from time integrated measurements of indoor radon, thoron and their decay product concentrations in schools in the Republic of Macedonia. Radiat Prot Dosim 162:152–156

    Article  Google Scholar 

  • Szabó Z, Jordan G, Szabó C, Horváth Á, Holm Ó, Kocsy G, Csige I, Szabó P, Homoki Z (2013) Radon and thoron levels, their spatial and seasonal variations in adobe dwellings: a case study at the great Hungarian plain. Isot Environ Health Stud 50:211–225

    Article  Google Scholar 

  • Tushe KB, Bylyku E, Xhixha G, Dhoqina P, Daci B, Cfarku F, Xhixha MK, Strati V (2015) First step towards the geographical distribution of indoor radon in dwellings in Albania. Radiat Prot Dosim. doi:10.1093/rpd/ncv494

    Google Scholar 

  • United Nations Scientific Committee on the Effects of Atomic Radiation (2000) Sources and effects of ionizing radiation. Report to the General Assembly with Scientific Annexes (Vol I Annex B) (NY: UN)

  • United Nations Scientific Committee on the Effects of Atomic Radiation (2008) Sources and effects of ionizing radiation. Report to the General Assembly with Scientific Annexes (Vol I Annex B) (NY: UN)

  • Yarmoshenko I, Vasilyev A, Malinovsky G, Bossew P, Žunić ZS, Onischenko A, Zhukovsky M, Onischenko A, Zhukovsky M (2016) Variance of indoor radon concentration: major influencing factors. Sci Total Environ 541:155–160

    Article  Google Scholar 

  • Yoshimura E, Da Silva A, Dos Anjos R, Umisedo N, Rizzotto M, Velasco H, Valladares D (2015) Radon concentration in air and external gamma dose rate: is there a correlation? J Radioanal Nucl Chem 307:787–792

    Article  Google Scholar 

  • Zhukovsky M, Termechikova R (2005) Exposure to radon in the northern part of the Republic of Kyrgyzstan. In: McLaughlin JP, Simopoulos SE, Steinhausler F (eds) Radioactivity in the environment, vol 7., The Natural Radiation Environment VIIElsevier, Amsterdam, pp 706–714

    Google Scholar 

  • Zunic ZS, McLaughlin JP, Walsh C, Birovljev A, Simopoulos SE, Jakupi B, Gordanic V, Demajo M, Trotti F, Falk R, Vanmarcke H, Paridaens J, Fujimoto K (2001) Integrated natural radiation exposure studies in stable Yugoslav rural communities. Sci Total Environ 272:253–259

    Article  Google Scholar 

  • Zunic ZS, Celikovic I, Tokonami S, Ishikawa T, Ujic P, Onischenko A, Zhukovsky M, Milic G, Jakupi B, Cuknic O, Veselinovic N, Fujimoto K, Sahoo S, Yarmoshenko I (2010a) Collaborative investigations on thoron and radon in some rural communities of Balkans. Radiat Prot Dosim 141:346–350

    Article  Google Scholar 

  • Zunic ZS, Veselinovic N, Bochicchio F, Carelli V, Vaupotic J, Cuknic O, Simovic R, Vojinovic Z, Kisic D, Tollefsen T (2010b) The indoor radon survey in Serbian schools: can it also reflect the general population exposure? Nukleonika 55:419–427

    Google Scholar 

  • Zunic ZS, Carpentieri C, Stojanovska Z, Antignani S, Veselinovic N, Tollefsen T, Carelli V, Cordedda C, Cuknic O, Filipovic J, Bossew P, Bochicchio F (2013) Some results of a radon survey in 207 Serbian schools. Rom J Phys 58S:S320–S327

    Google Scholar 

  • Zunic ZS, Ujic P, Nad L, Yarmoshenko IV, Radanovic SB, Komatina Petrovic S, Celikovic I, Komatina M, Bossew P (2014) High variability of indoor radon concentrations in uraniferous bedrock areas in the Balkan region. Appl Radiat Isot 94:328–337

    Article  Google Scholar 

Download references

Acknowledgments

The authors highly appreciate the enthusiasm of Mr. Eric Hulbert, Ph.D. from Radosys Company, Budapest, Hungary, who supported this project by donating the RSKS detectors. The authors would also like to express their gratitude to the mayors, schools directors, and the owners of the dwellings in Sveti Nikole, Kratovo, and Probistip municipalities for collaboration during this survey. This survey was funded by the research fund of the Goce Delcev University, Stip, Republic of Macedonia. The Gamma 1 detectors were provided within the Project P-41028 of the Ministry of Education, Science and Technological Development of the Republic of Serbia.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Zdenka Stojanovska.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Stojanovska, Z., Boev, B., Zunic, Z.S. et al. Variation of indoor radon concentration and ambient dose equivalent rate in different outdoor and indoor environments. Radiat Environ Biophys 55, 171–183 (2016). https://doi.org/10.1007/s00411-016-0640-y

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s00411-016-0640-y

Keywords

Navigation