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Absorption properties of urban/suburban aerosols in China

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Abstract

The broadband diffuse radiation method is improved to retrieve the aerosol refractive index imaginary part (AIP) and broadband (400–1000 nm mean) single scattering albedo (SSA). In this method, four sets of SSA selection criteria are proposed for quality control. The method is used to retrieve AIP, SSA and absorptive optical thickness (AbOT) from routine bourly-exposed pyrheliometer and paranometer measurements over 11 sites (meteorological observatories) in China during 1998–2003. Apart from one suburban site (Ejin Qi), the other urban sites are all located around big or medium cities. As shown in the retrieval results, annual mean SSA during 1998–2003 changes from 0.941 (Wuhan) to 0.849 (Lanzhou), and AIP from 0.0054 to 0.0203. The 11-site average annual mean SSA and AIP are 0.898 and 0.0119, respectively. SSA during winter is smaller for most sites. There is an evidently positive correlation between SSA and aerosol optical thickness (AOT) for all sites. There is also a positive correlation between SSA and relative humidity for most sites, but a negative correlation for a few sites, such as Kashi and Ürümqi in Northwest China.

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References

  • Bengtsson, L., E. Roeckner, and M. Stendel, 1999: Why is the global warming proceeding much slower than expected. J. Geophys. Res., 104, 3865–3878.

    Article  Google Scholar 

  • Charlson, R. J., S. E. Schwartz, J. M. Hales, R. D. Cess, J. A. Coakley, Jr. J. E. Hansen, and D. J. Hofmann, 1992: Climate forcing by anthropogenic aerosols. Science, 255, 423–429.

    Article  Google Scholar 

  • CMA (China Meteorological Administration), 1996: Meteorological Radiation Observation Method. China Meteorological Press, Beijing, 165pp.

    Google Scholar 

  • Dubovik, O., B. N. Holben, T. F. Eck, A. Smirnov, Y. J. Kaufman, M. D. King, D. Tanre, and I. Slutsker, 2002: Variability of absorption and optical properties of key aerosol types observed in worldwide locations. J. Atmos. Sci., 59, 590–608.

    Article  Google Scholar 

  • Eck, T. F., and Coauthors, 2005: Columnar aerosol optical properties of AERONET sites in central eastern Asia and aerosol transport to the tropical mid-Pacific. J. Geophys. Res., 110, D06202, doi:10,1029/2004JD005274.

  • Hartley, W. S., P. V. Hobbs, J. L. Ross, P. B. Ressell, and J. M. Livingston, 2000: Properties of aerosol aloft relevant to direct radiative forcing off the mid-Atlantic coast of the United States. J. Geophys. Res., 105, 9859–9885.

    Article  Google Scholar 

  • Herman, B. M., S. R. Browning, and J. J. De Luisi, 1975: Determination of the effective imaginary term of the complex refractive index of atmospheric dust by remote sensing: The Diffuse-Direct radiation method. J. Atmos. Sci., 32, 918–925.

    Article  Google Scholar 

  • Holben, B. N., and Coauthors, 1998: AERONET—A federated instrument network and data archive for aerosol characterization. Remote Sens. Environ., 66, 1–16.

    Article  Google Scholar 

  • Kaufman, Y. J., and Coauthors, 1997: Passive remote sensing of tropospheric aerosol and atmospheric correction for the aerosol effect. J. Geophys. Res., 102, 16815–16830.

    Article  Google Scholar 

  • Kiehl, J. T., and B. P. Briegleb, 1993: The radiative role of sulfate aerosols and greenhouse gases in climate forcing. Science, 260, 311–314.

    Article  Google Scholar 

  • Menon, S., J. Hansen, L., Nazarenko, and Y. Luo, 2002: Climate effects of black carbon aerosols in China and India. Science, 297, 2250–2253.

    Article  Google Scholar 

  • Nakajima, T., T. Hayasaka, A. Higrashi, G. Hashida, N. Moharram-Nejad, N. Yahya, and V. Hamzeh, 1996: Aerosol optical properties in the Iranian region obtained by ground-based solar radiation measurements in the summer of 1991. J. Appl. Meteor., 35, 1265–1278.

    Article  Google Scholar 

  • Paltridge, G. W., and C. M. R. Platt, 1976: Radiative Processes in Meteorology and Climatology. Elsevier Science, 318pp.

  • Penner, J. E., and Coauthors, 1994: Quantifying and minimizing uncertainty of climate forcing by anthropogenic aerosols. Bull. Amer. Meteor. Soc., 75, 375–400.

    Article  Google Scholar 

  • Qiu, J., 2001: Broadband extinction method to determine atmospheric aerosol optical properties. Tellus, 53B, 72–82.

    Google Scholar 

  • Qiu, J., 2003: Broadband extinction method to determine aerosol optical depth from accumulated solar direct radiation. J. Appl. Meteor., 42, 1611–1625.

    Article  Google Scholar 

  • Qiu, J., 2006: Broadband diffuse radiation method to retrieve radiation-weighted mean aerosol single scattering albedo. Chinese J. Atmos. Sci., 30, 767–777. (in Chinese)

    Google Scholar 

  • Qiu, J., L. Yang, and X. Zhang, 2004: Characteristics of imaginary part and single scattering albedo of urban aerosol in northern China. Tellus, 56B, 276–284.

    Google Scholar 

  • Qiu, J., X. Zong, and X. Zhang, 2005: A study of the scaling height of the tropospheric aerosol and its extinction coefficient profilre. Journal of Aerosol Science, 36, 361–371.

    Article  Google Scholar 

  • Taylor, K. E., and J. E. Penner, 1994: Response of the climate system to atmospheric aerosols and greenhouse gases. Nature, 369, 734–737.

    Article  Google Scholar 

  • Tegen, I., A. A. Lasis, and I. Fung, 1996: The influence of mineral aerosols from disturbed soils on the global radiation budget. Nature, 380, 419–422.

    Article  Google Scholar 

  • Wei, D., and J. Qiu, 1998: Wideband method to retrieve the imaginary part of complex refractive index of atmospheric aerosols, Part I: Theory. Chinese J. Atmos. Sci., 22, 677–685. (in Chinese)

    Google Scholar 

Download references

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Correspondence to Qiu Jinhuan  (邱金恒).

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Qiu, J., Yang, J. Absorption properties of urban/suburban aerosols in China. Adv. Atmos. Sci. 25, 1–10 (2008). https://doi.org/10.1007/s00376-008-0001-0

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  • DOI: https://doi.org/10.1007/s00376-008-0001-0

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