Abstract
A new approach for quantitative mixture fraction imaging in the turbulent mixing of a fuel jet and a high temperature oxidizer co-flow was developed by means of planar laser-induced fluorescence of nitric oxide (NO-PLIF). Unlike existing strategies, the new approach is based on seeding NO in the oxidizer stream. The method was first evaluated during the laminar mixing of methane in air and \(\hbox {CH}_4/\hbox {CO}_2\) blends (synthetic biogas) in air, at room temperature. Mixture fraction measurements were validated against Rayleigh scattering imaging. Then, the measurements were extended to the turbulent mixing of a cold fuel jet issuing into a NO-seeded, hot air co-flow. By seeding the NO in the air stream, high signal-to-noise ratios were achieved at locations around the stoichiometric mixture fraction. Additionally, a stable in situ calibration region is available at every measurement location, which contributes to reduce the uncertainty. Results showed that the approach is not suitable for CH\(_4\)/air mixtures due to the lack of sensitivity of the fluorescence signal to the mixture fraction. For biogas/air mixtures, the addition of CO\(_2\) increased the response of the fluorescence signal to the mixture fraction, making the measurements feasible. The stoichiometric mixture fraction can be fully resolved for each biogas blend. Two-dimensional instantaneous mixture fraction measurements were feasible with an acceptable uncertainty. The high spatial resolution of the measurement was of the same order of the smallest scale in the concentration field (i.e., Batchelor scale).
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Arndt CM, Papageorge MJ, Fuest F, Sutton JA, Meier W, Aigner M (2016) The role of temperature, mixture fraction, and scalar dissipation rate on transient methane injection and auto-ignition in a jet in hot coflow burner. Combust Flame 167:60–71. https://doi.org/10.1016/j.combustflame.2016.02.027
Arndt CM, Papageorge MJ, Fuest F, Sutton JA, Meier W (2018) Experimental investigation of the auto-ignition of a transient propane jet-in-hot-coflow. Proc Combust Ins. https://doi.org/10.1016/j.proci.2018.06.195
Bedoya ID, Saxena S, Cadavid FJ, Dibble RW (2011) Exploring strategies for reducing high intake temperature requirements and allowing optimal operational conditions in a biogas fueled HCCI engine for power generation. In: Proceedings of the ASME 2011 internal combustion engine division fall technical conference, ASME. https://doi.org/10.1115/ICEF2011-60198
Bessler WG, Schulz C, Sick V, Daily JW (2003) A versatile modeling tool for nitric oxide LIF spectra. In: Proceedings of third joint meeting of the US Sections of Combust Inst paper PI05. http://www.lifsim.com
Bessler WG, Schulz C, Lee T, Jeffries JB, Hanson RK (2002) Strategies for laser-induced fluorescence detection of nitric oxide in high-pressure flames. I. A–X(0,0) excitation. Appl Opt 41(18):3547–3557
Buch KA, Dahm WJA (1998) Experimental study of the fine-scale structure of conserved scalar mixing in turbulent shear flows. Part 2. Sc ≈ 1. J Fluid Mech 364:129. https://doi.org/10.1017/S0022112098008726
Charogiannis A, Beyrau F (2013) Laser induced phosphorescence imaging for the investigation of evaporating liquid flows. Exp Fluids 54(5):1518. https://doi.org/10.1007/s00348-013-1518-2
Dunn MJ, Masri AR, Bilger RW (2007) A new piloted premixed jet burner to study strong finite-rate chemistry effects. Combust Flame 151(1):46–60. https://doi.org/10.1016/j.combustflame.2007.05.010
Eitel F, Pareja J, Geyer D, Johchi A, Michel F, Elsäßer W, Dreizler A (2015) A novel plasma heater for auto-ignition studies of turbulent non-premixed flows. Exp Fluids 56(10):186. https://doi.org/10.1007/s00348-015-2059-7
Fielding J, Schaffer AM, Long MB (1998) Three-scalar imaging in turbulent non-premixed flames of methane. Symp (Int) Combust 27(1):1007–1014. https://doi.org/10.1016/S0082-0784(98)80500-6
Frank JH, Kaiser SA (2010) High-resolution imaging of turbulence structures in jet flames and non-reacting jets with laser Rayleigh scattering. Exp Fluids 49(4):823–837. https://doi.org/10.1007/s00348-010-0931-z
Frank J, Kaiser S, Long M (2005) Multiscalar imaging in partially premixed jet flames with argon dilution. Combust Flame 143(4):507–523
Gordon RL, Heeger C, Dreizler A (2009) High-speed mixture fraction imaging. Appl Phys B 96(4):745–748. https://doi.org/10.1007/s00340-009-3637-2
Hosseini SE, Wahid MA (2013) Biogas utilization: experimental investigation on biogas flameless combustion in lab-scale furnace. Energy Convers Manag 74:426–432. https://doi.org/10.1016/j.enconman.2013.06.026
Hsu A, Narayanaswamy V, Clemens N, Frank J (2011) Mixture fraction imaging in turbulent non-premixed flames with two-photon LIF of krypton. Proc Combust Inst 33(1):759–766. https://doi.org/10.1016/j.proci.2010.06.051
Kelman JB, Masri AR, Stråner SH, Bilger RW (1994) Wide-field conserved scalar imaging in turbulent diffusion flames by a raman and Rayleigh method. Symp (Int) Combust 25(1):1141–1147. https://doi.org/10.1016/S0082-0784(06)80752-6
Macfarlane A, Dunn M, Juddoo M, Masri A (2017) Stabilisation of turbulent auto-igniting dimethyl ether jet flames issuing into a hot vitiated coflow. Proc Combust Inst 36(2):1661–1668. https://doi.org/10.1016/j.proci.2016.08.028
Mansour MS (2003) Stability characteristics of lifted turbulent partially premixed jet flames. Combust Flame 133(3):263–274. https://doi.org/10.1016/S0010-2180(02)00566-7
Mastorakos E (2009) Ignition of turbulent non-premixed flames. Prog Energy Combust Sci 35(1):57–97
Namazian M, Kelly J, Schefer R (1994) Twenty-fifth symposium (international) on combustion 25(1):1149–1157
Papageorge M, Arndt C, Fuest F, Meier W, Sutton JA (2014) High-speed mixture fraction and temperature imaging of pulsed, turbulent fuel jets auto-igniting in high-temperature, vitiated co-flows. Exp Fluids 55(7):1–20
Patton RA, Gabet KN, Jiang N, Lempert WR, Sutton JA (2012) Multi-kHz mixture fraction imaging in turbulent jets using planar Rayleigh scattering. Appl Phys B 106(2):457–471. https://doi.org/10.1007/s00340-011-4658-1
Paul PH, Carter CD, Gray JA, Durant JL JR, Thoman JW, Furlanetto MR (1995) Correlations for the NO A\(^2\sigma ^+ (v^{\prime }=0)\) electronic quenching cross-section. Sandia National Laboratory Sandia Report pp SAND94-8237
Paul P (1997) Calculation of transition frequencies and rotational line strengths in the \(\gamma \)-bands of nitric oxide. J Quan Spectrosc Radiat Transf 57(5):581–589. https://doi.org/10.1016/S0022-4073(96)00158-6
Paul PH, Gray JA, Durant JL, Thoman JW (1993) A model for temperature-dependent collisional quenching of NO A\(^2\Sigma ^+\). Appl Phys B 57(4):249–259. https://doi.org/10.1007/BF00325203
Peters N (2000) Turbulent combustion. Cambridge University Press, Cambridge
Sadanandan R, Schießl RA, Markus D, Maas U (2011) 2D mixture fraction studies in a hot-jet ignition configuration using NO-LIF and correlation analysis. Flow Turbul Combust 86(1):45–62. https://doi.org/10.1007/s10494-010-9285-0
Sadanandan R, Fleck J, Meier W, Griebel P, Naumann C (2012) 2D mixture fraction measurements in a high pressure and high temperature combustion system using NO tracer-LIF. Appl Phys B 106(1):185–196
Schulz C, Sick V (2005) Tracer-LIF diagnostics: quantitative measurement of fuel concentration, temperature and fuel/air ratio in practical combustion systems. Prog Ener Combust Sci 31(1):75–121. https://doi.org/10.1016/j.pecs.2004.08.002
Schulz C, Dreizler A, Ebert V, Wolfrum J (2007) Combustion diagnostics. Springer, Berlin, pp 1241–1315 10.1007/978-3-540-30299-5\_20
Settersten TB, Patterson BD, Gray JA (2006) Temperature- and species-dependent quenching of NO A\(^2\Sigma ^+(v^{\prime }=0)\) probed by two-photon laser-induced fluorescence using a picosecond laser. J Chem Phys 124(23):234308. https://doi.org/10.1063/1.2206783
Skalska K, Miller JS, Ledakowicz S (2010) Kinetics of nitric oxide oxidation. Chem Pap 64(2):269–272. https://doi.org/10.2478/s11696-009-0105-8
Su LK, Clemens NT (2003) The structure of fine-scale scalar mixing in gas-phase planar turbulent jets. J Fluid Mech 488:129. https://doi.org/10.1017/S002211200300466X
Su LK, Han D, Mungal M (2000) Measurements of velocity and fuel concentration in the stabilization region of lifted jet diffusion flames. Proc Combust Inst 28(1):327–334. https://doi.org/10.1016/S0082-0784(00)80227-1
Sutton JA, Driscoll JF (2006) A method to simultaneously image two-dimensional mixture fraction, scalar dissipation rate, temperature and fuel consumption rate fields in a turbulent non-premixed jet flame. Exp Fluids 41(4):603–627
Tamura M, Berg PA, Harrington JE, Luque J, Jeffries JB, Smith GP, Crosley DR (1998) Collisional quenching of CH(A), OH(A), and NO(A) in low pressure hydrocarbon flames. Combust Flame 114(3–4):502–514. https://doi.org/10.1016/S0010-2180(97)00324-6
Tsurikov M, Clemens N (2002) The structure of dissipative scales in axisymmetric turbulent gas-phase jets. In: 40th AIAA aerospace sciences meeting and exhibit, aerospace sciences meetings, American Institute of Aeronautics and Astronautics. https://doi.org/10.2514/6.2002-164
van Breda IG (1992) Halation in image intensifiers. Mon Not R Astron Soc 257(3):415–418. https://doi.org/10.1093/mnras/257.3.415
Wang GH, Clemens NT (2004) Effects of imaging system blur on measurements of flow scalars and scalar gradients. Exp Fluids 37(2):194–205. https://doi.org/10.1007/s00348-004-0801-7
Acknowledgements
The authors acknowledge the funding by the Deutsche Forschungsgemeinschaft (DFG) through SFB-Transregio 129. Ayane Johchi for the funding of the Alexander von Humboldt Foundation. Andreas Dreizler is grateful for the support by the Gottfried Wilhelm Leibniz program of DFG.
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Johchi, A., Pareja, J., Böhm, B. et al. Quantitative mixture fraction imaging of a synthetic biogas turbulent jet propagating into a NO-vitiated air co-flow using planar laser-induced fluorescence (PLIF). Exp Fluids 60, 82 (2019). https://doi.org/10.1007/s00348-019-2723-4
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DOI: https://doi.org/10.1007/s00348-019-2723-4