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Laser-based measurements of pressure broadening and pressure shift coefficients of combustion-relevant absorption lines in the near-infrared region

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Abstract

A set of high-resolution absorption spectrometers based on TDLAS was used to determine the impact of combustion-relevant gases on the pressure shift and broadening of H2O, CO2, C2H2 and CH4 absorption lines in the near-infrared spectral region. In particular, self- and foreign-broadening coefficients induced by CO2, N2, O2, air, C2H2 and CH4 were measured. The absorption lines under investigation are suitable to measure the respective species in typical combustion environments via laser absorption spectroscopy. Additionally, species-dependent self- and foreign-induced pressure shift coefficients were measured and compared to the literature. The experiments were performed in two specifically designed absorption cells over a wide pressure range from 5 to 180 kPa. Different sources of uncertainty were identified and quantified to achieve relative measurement uncertainties of 0.7–1.5% for broadening coefficients and 0.6–1.6% for pressure shift coefficients.

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Acknowledgements

The authors thank the Deutsche Forschungsgemeinschaft for its support through CRC/Transregio 150 “Turbulent, chemically reactive multi-phase flows near walls”.

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  1. Reactive Flows and Diagnostics, Technische Universität Darmstadt, Darmstadt, Germany

    Sebastian Bürkle, Nicole Walter & Steven Wagner

  2. High Temperature Process Diagnostics, Technische Universität Darmstadt, Darmstadt, Germany

    Steven Wagner

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  1. Sebastian Bürkle
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Correspondence to Steven Wagner.

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Bürkle, S., Walter, N. & Wagner, S. Laser-based measurements of pressure broadening and pressure shift coefficients of combustion-relevant absorption lines in the near-infrared region. Appl. Phys. B 124, 121 (2018). https://doi.org/10.1007/s00340-018-6993-y

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