Abstract
We propose a pump-probe differential Lidar technique to remotely map the ability of the atmosphere to undergo particle condensation, which depends on the concentration of both pre-existing nanoparticles and condensable species or their precursors. Besides its interest for improving short-time, local weather forecast, this technique could provide information on atmospheric parameters such as the concentration of condensable species and physical parameters including the temperature and relative humidity.
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References
H.R. Pruppacher, J.D. Klett, Microphysics of Clouds and Precipitation (Kluwer Academic Publishers 1997)
J.H. Seinfeld, S.N. Pandis, Atmospheric Chemistry and Physics—From Air Pollution to Climate Change, 2nd edn. (Wiley, Hoboken, 2006)
P. Rohwetter, J. Kasparian, K. Stelmaszczyk, Z. Hao, S. Henin, N. Lascoux, W.M. Nakaema, Y. Petit, M. Queißer, R. Salamé, E. Salmon, L. Wöste, J.-P. Wolf, Laser-induced water condensation in air. Nat. Photonics 4, 451 (2010)
S. Henin, Y. Petit, P. Rohwetter, K. Stelmaszczyk, Z.Q. Hao, W.M. Nakaema, A. Vogel, T. Pohl, F. Schneider, J. Kasparian, K. Weber, L. Wöste, J.P. Wolf, Field measurements reveal mechanism of laser-assisted water condensation. Nat. Commun. 2, 456 (2011)
J. Kasparian, M. Rodriguez, G. Méjean, J. Yu, E. Salmon, H. Wille, R. Bourayou, S. Frey, Y.-B. André, A. Mysyrowicz, R. Sauerbrey, J.-P. Wolf, L. Wöste, Science 301, 61 (2003)
A. Couairon, A. Mysyrowicz, Phys. Rep. 44, 47 (2007)
L. Bergé, S. Skupin, R. Nuter, J. Kasparian, J.-P. Wolf, Rep. Prog. Phys. 70, 1633 (2007)
J. Kasparian, J.-P. Wolf, Opt. Express 16, 466 (2008)
S.L. Chin, S.A. Hosseini, W. Liu, Q. Luo, F. Théberge, N. Aközbek, A. Becker, V.P. Kandidov, O.G. Kosareva, H. Schröder, Can. J. Phys. 83, 863 (2005)
H. Saathoff, S. Henin, K. Stelmaszczyk, M. Petrarca, R. Delagrange, Z. Hao, J. Lüder, O. Möhler, Y. Petit, P. Rohwetter, M. Schnaiter, J. Kasparian, T. Leisner, J.-P. Wolf, L. Wöste, Laser filament-induced aerosol formation. Atmos. Chem. Phys. 13, 4593 (2013)
J. Kasparian, P. Rohwetter, L. Wöste, J.-P. Wolf, Laser-assisted water condensation in the atmosphere: a step towards modulating precipitation? J. Phys. D Appl. Phys. 45, 293001 (2012)
A.M. Chekalyuk, F.E. Hoge, C.W. Wright, R.N. Swift, Short-pulse pump-and-probe technique for airborne laser assessment of Photosystem II. photochemical characteristic. Photosynth. Res. 66, 33–44 (2000)
R.M. Measures Laser Remote Sensing–Fundamentals and Applications (Wiley, 1984)
F.A. Theopold, J.-P. Wolf, L. Wöste Dial Revisited: Belinda and White-Light Femtosecond Lidar, Range-Resolved Optical Sensing of the Atmosphere (Springer, 2005)
C.F. Bohren, D.R. Huffman Absorption and Scattering of Light by Small Particles (Wiley, 1983)
Acknowledgments
We acknowledge technical assistance of Nicolas Berti in programming the numerical simulations, as well as Jean-Pierre Wolf for fruitful discussions.
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Chagas, J.C.S., Leisner, T. & Kasparian, J. Pump-probe differential Lidar to quantify atmospheric supersaturation and particle-forming trace gases. Appl. Phys. B 117, 667–672 (2014). https://doi.org/10.1007/s00340-014-5881-3
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DOI: https://doi.org/10.1007/s00340-014-5881-3